Time-domain observation of interlayer exciton formation and thermalization in a MoSe/WSe heterostructure.

Vertical heterostructures of transition metal dichalcogenides (TMDs) host interlayer excitons with electrons and holes residing in different layers. With respect to their intralayer counterparts, interlayer excitons feature longer lifetimes and diffusion lengths, paving the way for room temperature excitonic optoelectronic devices. The interlayer exciton formation process and its underlying physical mechanisms are largely unexplored.

Impact of Optically Pumped Nonequilibrium Steady States on Luminescence Emission of Atomically Thin Semiconductor Excitons.

The interplay of the nonequivalent corners in the Brillouin zone of transition metal dichalcogenides (TMDCs) has been investigated extensively. While experimental and theoretical works contributed to a detailed understanding of the relaxation of selective optical excitations and the related relaxation rates, only limited microscopic descriptions of stationary experiments are available so far. Here we present microscopic calculations for the nonequilibrium steady state properties of excitons during continuous wave pumping exemplary for monolayer MoSe_{2}.

Extended Spatial Coherence of Interlayer Excitons in MoSe_{2}/WSe_{2} Heterobilayers.

We report on the spatial coherence of interlayer exciton ensembles as formed in MoSe_{2}/WSe_{2} heterostructures and characterized by point-inversion Michelson-Morley interferometry. Below 10 K, the measured spatial coherence length of the interlayer excitons reaches values equivalent to the lateral expansion of the exciton ensembles. In this regime, the light emission of the excitons turns out to be homogeneously broadened in energy with a high temporal coherence.

Using Matrix-Product States for Open Quantum Many-Body Systems: Efficient Algorithms for Markovian and Non-Markovian Time-Evolution.

This paper presents an efficient algorithm for the time evolution of open quantum many-body systems using matrix-product states (MPS) proposing a convenient structure of the MPS-architecture, which exploits the initial state of system and reservoir. By doing so, numerically expensive re-ordering protocols are circumvented. It is applicable to systems with a Markovian type of interaction, where only the present state of the reservoir needs to be taken into account.