Experimental determination of single molecule toroic behaviour in a Dy single molecule magnet.

The enhancement of toroic motifs through coupling toroidal moments within molecular nanomagnets is a new, interesting and relevant approach for both fundamental research and potential quantum computation applications. We investigate a Dy8 molecular cluster and discover it has a antiferrotoroic ground state with slow magnetic relaxation. The experimental characterization of the magnetic anisotropy axes of each magnetic center and their exchange interactions represents a considerable challenge due to the non-magnetic nature of the toroidal motif.

Transport evidence for a sliding two-dimensional quantum electron solid.

Ignited by the discovery of the metal-insulator transition, the behaviour of low-disorder two-dimensional (2D) electron systems is currently the focus of a great deal of attention. In the strongly interacting limit, electrons are expected to crystallize into a quantum Wigner crystal, but no definitive evidence for this effect has been obtained despite much experimental effort over the years. Here, studying the insulating state of a 2D electron system in silicon, we have found two-threshold voltage-current characteristics with a dramatic increase in noise between the two threshold voltages.

Onset of a propagating self-sustained spin reversal front in a magnetic system.

The energy released in a magnetic material by reversing spins as they relax toward equilibrium can lead to a dynamical instability that ignites self-sustained rapid relaxation along a deflagration front that propagates at a constant subsonic speed. Using a trigger heat pulse and transverse and longitudinal magnetic fields, we investigate and control the crossover between thermally driven magnetic relaxation and magnetic deflagration in single crystals of Mn(12)-acetate.

Critical behavior of a strongly interacting 2D electron system.

With decreasing density n(s) the thermopower S of a low-disorder two-dimensional electron system in silicon is found to exhibit a sharp increase by more than an order of magnitude tending to a divergence at a finite disorder-independent density n(t) consistent with the critical form (-T/S) is proportional to (n(s)-n(t))(x) with x=1.0±0.1 (T is the temperature).

Propagation of avalanches in Mn12-acetate: magnetic deflagration.

Local time-resolved measurements of fast reversal of the magnetization of single crystals of Mn12-acetate indicate that the magnetization avalanche spreads as a narrow interface that propagates through the crystal at a constant velocity that is roughly 2 orders of magnitude smaller than the speed of sound. We argue that this phenomenon is closely analogous to the propagation of a flame front (deflagration) through a flammable chemical substance.

Distribution of tunnel splittings in Mn(12) acetate.

In magnetic fields applied parallel to the anisotropy axis, the relaxation of the magnetization of Mn(12)-acetate measured for different sweep rates collapses onto a single scaled curve. The form of the scaling implies that the dominant symmetry-breaking process responsible for tunneling is a locally varying second-order transverse anisotropy, forbidden by tetragonal symmetry in the perfect crystal, which gives rise to a broad distribution of tunnel splittings in a real crystal of Mn(12) acetate. Different forms applied to even- and odd-numbered steps provide a clear distinction between even resonances (associated with crystal anisotropy) and odd resonances (which require a transverse magnetic field).

Scaling of the magnetoconductivity of silicon MOSFETs: evidence for a quantum phase transition in two dimensions.

For a broad range of electron densities n and temperatures T, the in-plane magnetoconductivity of the two-dimensional system of electrons in silicon MOSFETs can be scaled onto a universal curve with a single parameter H(sigma)(n,T), where H(sigma) obeys the empirical relation H(sigma) = A(n) [Delta(n)(2)+T2](1/2). The characteristic energy k(B)Delta associated with the magnetic field dependence of the conductivity decreases with decreasing density, and extrapolates to 0 at a critical density n(0), signaling the approach to a zero-temperature quantum phase transition. We show that H(sigma) = AT for densities near n(0).

Small-angle shubnikov-de haas measurements in a 2D electron system: the effect of a strong In-plane magnetic field.

Measurements in magnetic fields applied at small angles relative to the electron plane in silicon MOSFETs indicate a factor of 2 increase of the frequency of Shubnikov-de Haas oscillations at H>H(sat). This signals the onset of full spin polarization above H(sat), the parallel field above which the resistivity saturates to a constant value. For H View Article and Find Full Text PDF

Novel phenomena in dilute electron systems in two dimensions.

For the past two decades, all two-dimensional systems of electrons were believed to be insulating in the limit of zero temperature. Recent experiments provide evidence for an unexpected transition to a conducting phase at very low electron densities. The nature of this phase is not understood and is currently the focus of intense theoretical and experimental attention.