We report for the first time to our knowledge optical waveguiding in an organic crystalline waveguide produced by ion implantation. Using H+ ions a refractive index barrier suitable for waveguiding has been realized in the highly nonlinear optical organic crystal 4-N, N-dimethylamino-4'-N'-methyl-stilbazolium tosylate (DAST). The refractive index changes in the waveguiding region as a function of the distance from the surface have been measured.
View Article and Find Full Text PDFWe show that high-temperature reduction in a CO-CO(2) atmosphere increases the photorefractive sensitivity of KNbO(3):Rh at 860nm by 4 orders of magnitude compared with that of the as-grown crystal. The effective trap density is increased by a factor of 3, and the photoconductivity by a factor of 30, and the photorefractive response at a grating spacing of 0.15 mu;m is accelerated by a factor of 400.
View Article and Find Full Text PDFThe photorefractive properties of stoichiometric LiNbO(3) crystals with a small number of defect densities grown by the double-crucible Czochralski method are investigated and compared with the defect densities of commercially available congruent Fe-doped LiNbO(3) crystals. Two-wave-mixing experiments show that novel stoichiometric crystals exhibit larger photorefractive gain and considerably faster response times than congruent ones. The results indicate that the nonstoichiometry defect control of photorefractive crystals is of key importance for the improvement of their properties.
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