On-demand generation of soliton molecules through evolutionary algorithm optimization.

Combining evolutionary algorithm optimization with ultrafast fiber laser technology, we report on the self-generation of stable two-soliton molecules with controllable temporal separation. A fiber laser setup including an adjustable virtual saturable absorber achieved through nonlinear polarization evolution and an intracavity pulse shaper is used to generate two-soliton molecules with a user-defined 3-8 ps internal delay.

Ultrafast background-free ro-vibrational fs/ps-CARS thermometry using an Yb:YAG crystal-fiber amplified probe.

A novel laser system for ro-vibrational spectroscopy using coherent anti-Stokes Raman Scattering in hybrid fs/ps regime is presented. A single Yb:KGW laser source is used as a master laser to generate the three CARS laser beams, namely the pump and Stokes femtosecond pulses and a 58 ps probe pulse. Master oscillator power amplifier (MOPA) architecture is implemented to increase the probe output power using a custom two stage free space linear amplifier.

Fully phase-stabilized quantum cascade laser frequency comb.

Miniaturized frequency comb sources across hard-to-access spectral regions, i.e. mid- and far-infrared, have long been sought.

Rovibrational hybrid fs/ps CARS using a volume Bragg grating for N₂ thermometry.

Coherent anti-Stokes Raman scattering (CARS) spectra of N2 in the hybrid femtosecond/picosecond regime have been recorded with 0.7  cm(-1) resolution. The Q-branch rovibrational structure has been resolved, making it suitable for gas-phase simultaneous rotational and vibrational thermometry applications.