Organic-inorganic halide perovskite solar cells (PSCs) have attracted significant attention in photovoltaic research, owing to their superior optoelectronic properties and cost-effective manufacturing techniques. However, the unbalanced charge carrier diffusion length in perovskite materials leads to the recombination of photogenerated electrons and holes. The inefficient charge carrier collecting process severely affects the power conversion efficiency (PCE) of the PSCs.
View Article and Find Full Text PDFDynamic optimization of the quantum-well (QW) width distribution in quasi-2D halide perovskite thin films is an effective approach for tuning the properties of photoelectric devices. Here, that the QWs width distribution in quasi-2D perovskite films can be controlled only by using hydroiodic acid (HI) as an additive is demonstrated. A uniform distribution of the colloidal particle size in the quasi-2D perovskite precursor solution is achieved through the formation of soluble iodoplumbate coordination complexes, PbI from the reaction of HI with PbI , resulting in an improved phase purity in the final film.
View Article and Find Full Text PDFSurface trap as intrinsic defects-mediated non-radiative charge recombination is a major obstacle to achieving the reliable fabrication of high-efficiency and large-area perovskite photovoltaics. Here a CS vapor-assisted passivation strategy is proposed for perovskite solar module, aiming to passivate the iodine vacancy and uncoordinated Pb caused by ion migration. Significantly, this method can avoid the disadvantages of inhomogeneity film caused by spin-coating-assisted passivation and reconstruction of perovskite surface from solvent.
View Article and Find Full Text PDFPaper is ubiquitous in the daily life and has been widely used for writing and drawing because of their low-cost, widely accessible, and degradable properties. However, simple ways to fabricate paper-based optoelectronic devices remain a great challenge. In this work, we report a facile method to fabricate high-quality perovskite films and optoelectronic devices on paper by direct pen-writing.
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