Advancements in photonics technologies have significantly enhanced their capability to facilitate experiments involving quantum light, even at room temperature. Nevertheless, fully integrating photonic chips that include quantum light sources, effective manipulation and transport of light minimizing losses, and appropriate detection systems remains an ongoing challenge. Topological photonic systems have emerged as promising platforms to protect quantum light properties during propagation, beyond merely preserving light intensity.
View Article and Find Full Text PDFJ Chem Theory Comput
March 2024
We report on a theoretical study of a Cs molecule illuminated by two lasers and show how this can result in novel quantum dynamics. We reveal that these interactions facilitate the bypass of the non-crossing rule, forming light-induced conical intersections and modifiable avoided crossings. Our findings show how laser field orientation and strength, along with initial phase differences, can control molecular-state transitions, especially on the scale.
View Article and Find Full Text PDFWe report on the effects of electron-phonon interaction in materials such as graphene, showing that it enables the formation of a gap bridged by unique edge states. These states exhibit a distinctive locking among propagation direction, valley, and phonon mode, allowing for the generation of electron-phonon entangled states whose parts can be easily split. We discuss the effect of the chiral atomic motion in the zone boundary phonons leading to this effect.
View Article and Find Full Text PDFUnlike the chirality of electrons, the intrinsic chirality of phonons has only surfaced in recent years. Here, we report on the effects of the interaction between electrons and chiral phonons in two-dimensional materials by using a nonperturbative solution. We show that chiral phonons introduce inelastic Umklapp processes resulting in copropagating edge states that coexist with a continuum.
View Article and Find Full Text PDFHarnessing the unique features of topological materials for the development of a new generation of topological based devices is a challenge of paramount importance. Using Floquet scattering theory combined with atomistic models we study the interplay among laser illumination, spin, and topology in a two-dimensional material with spin-orbit coupling. Starting from a topological phase, we show how laser illumination can selectively disrupt the topological edge states depending on their spin.
View Article and Find Full Text PDFFloquet theory combined with a realistic description of the electronic structure of illuminated graphene and graphene nanoribbons is developed to assess the emergent non-adiabatic and non-perturbative effects on the electronic properties. Here we introduce an efficient computational scheme and illustrate its use by applying it to graphene nanoribbons in the presence of both linear and circular polarization. The interplay between confinement due to the finite sample size and laser-induced transitions is shown to lead to sharp features in the average conductance and density of states.
View Article and Find Full Text PDFThis review deals with the role of electron-phonon (e-ph) coupling in quantum transport of carbon nanotubes. First, the case of low-energy phonons and weak localization phenomena is addressed, followed by a summary of inelastic scattering lengths within the Fermi golden rule. A second part outlines the contribution of high-energy optic phonon modes, and discusses the applicability limits of semi-classical transport theory.
View Article and Find Full Text PDFPhys Rev Lett
August 2006
We report on a theoretical study of inelastic quantum transport in (3m,0) carbon nanotubes. By using a many-body description of the electron-phonon interaction in Fock space, a novel mechanism involving optical phonon emission (absorption) is shown to induce an unprecedented energy-gap opening at half the phonon energy, variant Planck's over 2piomega0/2, above (below) the charge neutrality point. This mechanism, which is prevented by Pauli blocking at low bias voltages, is activated at bias voltages on the order of variant Planck's over 2piomega0.
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