Publications by authors named "Linhan Lin"

Fano resonances in photonics arise from the coupling and interference between two resonant modes in structures with broken symmetry. They feature an uneven and narrow and tunable lineshape and are ideally suited for optical spectroscopy. Many Fano resonance structures have been suggested in nanophotonics over the last ten years, but reconfigurability and tailored design remain challenging.

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Laser-induced crystallization through optical trapping offers precise and spatiotemporal control of crystallization kinetics at the microscale region. Here, we demonstrate the optical trapping-induced crystallization of various amino acids, including glycine, l-cysteine, and l-alanine, by focusing a 532 nm continuous-wave laser in amino acid/HO solution. The coordinated effect of optical forces and heat-driven molecular delivery improves the local molecular concentration, leading to nucleation and subsequent crystal growth.

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The emitter-cavity strong coupling manifests crucial significance for exploiting quantum technology, especially in the scale of individual emitters. However, due to the small light-matter interaction cross-section, the single emitter-cavity strong coupling has been limited by its harsh requirement on the quality factor of the cavity and the local density of optical states. Herein, we present a strategy termed waveguide-assisted energy quantum transfer (WEQT) to improve the single emitter-cavity coupling strength by extending the interaction cross-section.

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Crystallization is a fundamental phenomenon which describes how the atomic building blocks such as atoms and molecules are arranged into ordered or quasi-ordered structure and form solid-state materials. While numerous studies have focused on the nucleation behavior, the precise and spatiotemporal control of growth kinetics, which dictates the defect density, the micromorphology, as well as the properties of the grown materials, remains elusive so far. Herein, we propose an optical strategy, termed optofluidic crystallithography (OCL), to solve this fundamental problem.

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3D printing of inorganic materials with nanoscale resolution offers a different materials processing pathway to explore devices with emergent functionalities. However, existing technologies typically involve photocurable resins that reduce material purity and degrade properties. We develop a general strategy for laser direct printing of inorganic nanomaterials, as exemplified by more than 10 semiconductors, metal oxides, metals, and their mixtures.

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Non-invasive and rapid imaging technique at subcellular resolution is significantly important for multiple biological applications such as cell fate study. Label-free refractive-index (RI)-based 3D tomographic imaging constitutes an excellent candidate for 3D imaging of cellular structures, but its full potential in long-term spatiotemporal cell fate observation is locked due to the lack of an efficient integrated system. Here, a long-term 3D RI imaging system incorporating a cutting-edge white light diffraction phase microscopy module with spatiotemporal stability, and an acoustofluidic device to roll and culture single cells in a customized live cell culture chamber is reported.

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Excitons are quasi-particles composed of electron-hole pairs through Coulomb interaction. Due to the atomic-thin thickness, they are tightly bound in monolayer transition metal dichalcogenides (TMDs) and dominate their optical properties. The capability to manipulate the excitonic behavior can significantly influence the photon emission or carrier transport performance of TMD-based devices.

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Three-dimensional (3D) laser nanoprinting allows maskless manufacturing of diverse nanostructures with nanoscale resolution. However, 3D manufacturing of inorganic nanostructures typically requires nanomaterial-polymer composites and is limited by a photopolymerization mechanism, resulting in a reduction of material purity and degradation of intrinsic properties. We developed a polymerization-independent, laser direct writing technique called photoexcitation-induced chemical bonding.

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The development of high-temperature photodetectors can be beneficial for numerous applications, such as aerospace engineering, military defence and harsh-environments robotics. However, current high-temperature photodetectors are characterized by low photoresponsivity (<10 A/W) due to the poor optical sensitivity of commonly used heat-resistant materials. Here, we report the realization of h-BN-encapsulated graphite/WSe2 photodetectors which can endure temperatures up to 700 °C in air (1000 °C in vacuum) and exhibit unconventional negative photoconductivity (NPC) at high temperatures.

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Precise patterning with microscale lateral resolution and widely tunable heights is critical for integrating colloidal nanocrystals into advanced optoelectronic and photonic platforms. However, patterning nanocrystal layers with thickness above 100 nm remains challenging for both conventional and emerging direct photopatterning methods, due to limited light penetration depths, complex mechanical and chemical incompatibilities, and others. Here, we introduce a direct patterning method based on a thermal mechanism, namely, the thermally activated ligand chemistry (or TALC) of nanocrystals.

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Article Synopsis
  • Optical systems are explored as a new way to study Bloch oscillations, focusing on how different polarizations affect their propagation.
  • The research uses advanced 3D laser writing to create a unique waveguide array that reveals polarization-dependent behaviors in Bloch oscillations.
  • Findings present a novel method for understanding two-dimensional optical Bloch modes, emphasizing how optical polarization influences these oscillations, potentially uncovering more complex phenomena within a single structure.
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The optical manipulation of tiny objects is significant to understand and to explore the unknown in the microworld, which has found many applications in materials science and life science. Physically speaking, these technologies arise from direct or indirect optomechanical coupling to convert incident optical energy to mechanical energy of target objects, while their efficiency and functionalities are determined by the coupling behavior. Traditional optical tweezers stem from direct light-to-matter momentum transfer, and the generation of an optical gradient force requires high optical power and rigorous optics.

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Remote manipulation of a micromachine under an external magnetic field is significant in a variety of applications. However, magnetic manipulation requires that either the target objects or the fluids should be ferromagnetic or superparamagnetic. To extend the applicability, we propose a versatile optical printing technique termed femtosecond laser-directed bubble microprinting (FsLDBM) for on-demand magnetic encoding.

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Optical manipulation of micro/nanoscale objects is of importance in life sciences, colloidal science, and nanotechnology. Optothermal tweezers exhibit superior manipulation capability at low optical intensity. However, our implicit understanding of the working mechanism has limited the further applications and innovations of optothermal tweezers.

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It has been well established that thermoelectric (TE) field can arise from different Soret coefficients of salt ions in the aqueous solution under constant temperature gradient. Despite their high relevance to cellular biology and particle manipulations, understanding and controlling of TE field in complex colloidal systems that involve micro/nanoparticles, salt ions and molecules have remained challenging. In such colloidal systems, the challenge arises from the thermal interactions with charged micro/nanoparticles that distort the TE field around the particles.

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Inspired by the "run-and-tumble" behaviours of Escherichia coli () cells, we develop opto-thermoelectric microswimmers. The microswimmers are based on dielectric-Au Janus particles driven by a self-sustained electrical field that arises from the asymmetric optothermal response of the particles. Upon illumination by a defocused laser beam, the Janus particles exhibit an optically generated temperature gradient along the particle surfaces, leading to an opto-thermoelectrical field that propels the particles.

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The rapid development in materials science and engineering requests the manufacturing of materials in a more rational and designable manner. Beyond traditional manufacturing techniques, such as casting and coating, digital control of material morphology, composition, and structure represents a highly integrated and versatile approach. Digital manufacturing systems enable users to fabricate freeform materials, which lead to new functionalities and applications.

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Optomechanics arises from the photon momentum and its exchange with low-dimensional objects. It is well known that optical radiation exerts pressure on objects, pushing them along the light path. However, optical pulling of an object against the light path is still a counter-intuitive phenomenon.

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Constructing colloidal particles into functional nanostructures, materials, and devices is a promising yet challenging direction. Many optical techniques have been developed to trap, manipulate, assemble, and print colloidal particles from aqueous solutions into desired configurations on solid substrates. However, these techniques operated in liquid environments generally suffer from pattern collapses, Brownian motion, and challenges that come with reconfigurable assembly.

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Chirality is a ubiquitous phenomenon in the natural world. Many biomolecules without inversion symmetry such as amino acids and sugars are chiral molecules. Measuring and controlling molecular chirality at a high precision down to the atomic scale are highly desired in physics, chemistry, biology, and medicine, however, have remained challenging.

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Light-based manipulation of colloidal particles holds great promise in fabrication of functional devices. Construction of complex colloidal superstructures using traditional optical tweezers is limited by high operation power and strong heating effect. Herein, we demonstrate low-power opto-thermophoretic manipulation and construction of colloidal superstructures in photocurable hydrogels.

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Article Synopsis
  • Recent advancements in chemical sciences allow for customizable synthesis of colloidal particles, enabling control over their composition, size, shape, and properties.
  • Optical nanoprinting emerges as a powerful technique, enabling precise arrangement of colloidal particles into desired configurations for creating functional materials and devices.
  • This review highlights recent developments in optical nanoprinting, detailing various techniques and their potential applications in fields like nanophotonics, energy, microelectronics, and nanomedicine.
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The response of colloidal particles to a light-controlled external temperature field can be harnessed for opto-thermophoretic manipulation of the particles. The thermoelectric effect is regarded as the driving force for thermophoretic trapping of particles at the light-irradiated hot region, which is thus limited to ionic liquids. Herein, we achieve opto-thermophoretic manipulation of colloidal particles in various non-ionic liquids, including water, ethanol, isopropyl alcohol and 1-butanol, and establish the physical mechanism of the manipulation at the molecular level.

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Opto-thermophoretic manipulation is an emerging field, which exploits the thermophoretic migration of particles and colloidal species under a light-controlled temperature gradient field. The entropically favorable photon-phonon conversion and widely applicable heat-directed migration make it promising for low-power manipulation of variable particles in different fluidic environments. By exploiting an optothermal substrate, versatile opto-thermophoretic manipulation of colloidal particles and biological objects can be achieved via optical heating.

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Lipid vesicles are important biological assemblies, which are critical to biological transport processes, and vesicles prepared in the lab are a workhorse for studies of drug delivery, protein unfolding, biomolecular interactions, compartmentalized chemistry, and stimuli-responsive sensing. The current method of using optical tweezers for holding lipid vesicles in place for single-vesicle studies suffers from limitations such as high optical power, rigorous optics, and small difference in the refractive indices of vesicles and water. Herein, we report the use of plasmonic heating to trap vesicles in a temperature gradient, allowing long-range attraction, parallel trapping, and dynamic manipulation.

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