Efficient Decoupled Electrolytic Water Splitting in Acid through Pseudocapacitive TiO.

Water electrolysis remains a key component in the societal transition to green energy. Membrane electrolyzers are the state-of-the-art technology for water electrolysis, relying on 80 °C operation in highly alkaline electrolytes, which is undesirable for many of the myriad end-use cases for electrolytic water splitting. Herein, an alternative water electrolysis process, decoupled electrolysis, is described which performed in mild acidic conditions with excellent efficiencies.