Publications by authors named "Lennart J de Vreede"

Article Synopsis
  • - This paper introduces a method for creating fused silica chips for low-noise sensing without using masks, involving techniques like femtosecond laser modification and low-pressure chemical vapor deposition of silicon nitride (SiN).
  • - The resulting chips feature a robust SiN window attached to a fused silica support, showing durability during cleaning processes and allowing for controlled creation of nanopores using advanced techniques.
  • - Fused silica nanopore chips outperform silicon chips significantly, improving signal-to-noise ratios and capture rates for proteins, with notably reduced noise, which benefits experiments combining electrical and optical measurements.
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We found that gold nanoparticles, when heated to close to their melting point on substrates of amorphous SiO2 or amorphous Si3N4, move perpendicularly into the substrate. Dependent on applied temperatures, particles can become buried or leave nanopores of extreme aspect ratio (diameter ≅ 25 nm, length up to 800 nm). The process can be understood as driven by gold evaporation and controlled by capillary forces and can be controlled by temperature programming and substrate choice.

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The strong demand for renewable energy promotes research on novel methods and technologies for energy conversion. Microfluidic systems for energy conversion by streaming current are less known to the public, and the relatively low efficiencies previously obtained seemed to limit the further applications of such systems. Here we report a microdroplet-based electrostatic generator operating by an acceleration-deceleration cycle ('ballistic' conversion), and show that this principle enables both high efficiency and compact simple design.

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In this contribution, we present for the first time the experimental results of energy conversion from the streaming current when a polymer is added to the working solution. We added polyacrylic acid (PAA) in concentrations of 200 ppm to 4000 ppm to a KCl solution. By introducing PAA, the input power, which is the product of volumetric flow rate and the applied pressure, reduced rapidly as compared to the case of using only a normal viscous electrolyte KCl solution.

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