Coherent Bichromatic Force Deflection of Molecules.

We demonstrate the effect of the coherent optical bichromatic force on a molecule, the polar free radical strontium monohydroxide (SrOH). A dual-frequency retroreflected laser beam addressing the X[over ˜]^{2}Σ^{+}↔A[over ˜]^{2}Π_{1/2} electronic transition coherently imparts momentum onto a cryogenic beam of SrOH. This directional photon exchange creates a bichromatic force that transversely deflects the molecules.