Using a rigorous, rate-based model and a validated economic model, we investigated the technoeconomic performance of an aqueous NH-based CO capture process integrated with a 650-MW coal-fired power station. First, the baseline NH process was explored with the process design of simultaneous capture of CO and SO to replace the conventional FGD unit. This reduced capital investment of the power station by US$425/kW (a 13.
View Article and Find Full Text PDFUsing a rate-based model, we assessed the technical feasibility and energy performance of an advanced aqueous-ammonia-based postcombustion capture process integrated with a coal-fired power station. The capture process consists of three identical process trains in parallel, each containing a CO2 capture unit, an NH3 recycling unit, a water separation unit, and a CO2 compressor. A sensitivity study of important parameters, such as NH3 concentration, lean CO2 loading, and stripper pressure, was performed to minimize the energy consumption involved in the CO2 capture process.
View Article and Find Full Text PDFEnviron Sci Technol
February 2015
The gas-liquid membrane contactor generally used as a nonselective gas absorption enhancement device is innovatively proposed as a condenser for heat recovery in liquid-absorbent-based carbon capture. The membrane condenser is used as a heat exchanger to recover the latent heat of the exiting vapor from the desorber, and it can help achieve significant energy savings when proper membranes with high heat-transfer coefficients are used. Theoretical thermodynamic analysis of mass and heat transfer in the membrane condensation system shows that heat recovery increases dramatically as inlet gas temperature rises and outlet gas temperature falls.
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