Publications by authors named "Laurent C Chapon"

Transition-metal dichalcogenides (TMDs) offer an ideal platform to experimentally realize Dirac fermions. However, typically these exotic quasiparticles are located far away from the Fermi level, limiting the contribution of Dirac-like carriers to the transport properties. Here we show that NiTe hosts both bulk Type-II Dirac points and topological surface states.

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The analysis of three-dimensional neutron spin polarization vectors, using a technique referred to as spherical neutron polarimetry (SNP), is a very powerful means of determining complex magnetic structures in magnetic materials. However, the requirement to maintain neutrons in a highly polarized state has made it difficult to use this technique in conjunction with extreme experimental conditions. We have developed a high pressure cell made completely of nonmagnetic materials and having no effect on neutron polarizations.

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(ND)[FeCl(DO)] represents a promising example of the hybrid molecular/inorganic approach to create materials with strong magneto-electric coupling. Neutron spherical polarimetry, which is directly sensitive to the absolute magnetic configuration and domain population, has been used in this work to unambiguously prove the multiferroicity of this material. We demonstrate that the application of an electric field upon cooling results in the stabilization of a single-cycloidal magnetic domain below 6.

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The coupling of magnetic chiralities to the ferroelectric polarization in multiferroic RbFe(MoO4)2 is investigated by neutron spherical polarimetry. Because of the axiality of the crystal structure below T(c)=190   K, helicity and triangular chirality are symmetric-exchange coupled, explaining the onset of the ferroelectricity in this proper-screw magnetic structure--a mechanism that can be generalized to other systems with ferroaxial distortions in the crystal structure. With an applied electric field, we demonstrate control of the chiralities in both structural domains simultaneously.

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The incommensurate-commensurate phases reported in cupric oxide below 230 K are shown theoretically to realize an inverted sequence of symmetry-breaking mechanisms with respect to the usual sequence occurring in low-temperature multiferroic compounds. The sequence inversion results from a strong triggering-coupling mechanism between two antiferromagnetic order parameters inducing a first-order transition to the multiferroic phase. Such mechanism is favored by the large antiferromagnetic superexchange interactions, responsible of the high-T(N) temperature, and implies a preeminence of these interactions on the magnetocrystalline anisotropy.

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Article Synopsis
  • The study utilized high-resolution neutron powder diffraction to determine the magnetic and crystal structures of alpha-NaMnO2.
  • The material features a frustrated triangular spin lattice with two-dimensional spin correlations occurring below 200 K.
  • A structural phase transition at 45 K leads to a three-dimensional antiferromagnetic state with a specific propagation vector k=(1/2,1/2,0).
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The reaction of hydrogen gas with magnesium metal, which is important for hydrogen storage purposes, is enhanced significantly by the addition of catalysts such as Nb and V and by using nanostructured powders. In situ neutron diffraction on MgNb(0.05) and MgV(0.

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