We demonstrate the successful implementation of an artificial neural network (ANN) to eliminate detrimental spectral shifts imposed in the measurement of laser absorption spectrometers (LASs). Since LASs rely on the analysis of the spectral characteristics of biological and chemical molecules, their accuracy and precision is especially prone to the presence of unwanted spectral shift in the measured molecular absorption spectrum over the reference spectrum. In this paper, an ANN was applied to a scanning grating-based mid-infrared trace gas sensing system, which suffers from temperature-induced spectral shifts.
View Article and Find Full Text PDFQuantum optics largely relies on the fundamental concept that the diffraction and interference patterns of a multi-partite state are determined by its de Broglie wavelength. In this paper we show that this is still true for a mixed state with one sub-system being in a classical coherent state and one being in entangled state. We demonstrate the quantum-classical light discrimination using de Broglie wavelength for the states with all classical parameters being the same.
View Article and Find Full Text PDFWe report ultra-low phase-noise microwave generation at a 9.6 GHz carrier frequency from optical frequency combs based on diode-pumped solid-state lasers emitting at telecom wavelength and referenced to a common cavity-stabilized continuous-wave laser. Using a novel fibered polarization-maintaining pulse interleaver, a single-oscillator phase-noise floor of -171 dBc/Hz at 10 MHz offset frequency has been measured with commercial PIN InGaAs photodiodes, constituting a record for this type of detector.
View Article and Find Full Text PDFDisordered photonic materials can diffuse and localize light through random multiple scattering, offering opportunities to study mesoscopic phenomena, control light-matter interactions, and provide new strategies for photonic applications. Light transport in such media is governed by photonic modes characterized by resonances with finite spectral width and spatial extent. Considerable steps have been made recently towards control over the transport using wavefront shaping techniques.
View Article and Find Full Text PDFCdSe semiconductor nanocrystal quantum dots are assembled into nanowire-like arrays employing microtubule fibers as nanoscale molecular "scaffolds." Spectrally and time-resolved energy-transfer analysis is used to assess the assembly of the nanoparticles into the hybrid inorganic biomolecular structure. Specifically, we demonstrate that a comprehensive study of energy transfer between quantum dot pairs on the biotemplate and, alternatively, between quantum dots and molecular dyes embedded in the microtubule scaffold comprises a powerful spectroscopic tool for evaluating the assembly process.
View Article and Find Full Text PDFWe demonstrate the nonresonant magnetic interaction at optical frequencies between a photonic crystal microcavity and a metallized near-field microscopy probe. This interaction can be used to map and control the magnetic component of the microcavity modes. The metal coated tip acts as a microscopic conductive ring, which induces a magnetic response opposite to the inducing magnetic field.
View Article and Find Full Text PDFOptical properties of InAs/GaAs quantum dots in micropillar cavities emitting at 1.3 microm are studied by time-resolved microphotoluminescence. The Purcell effect is observed with an enhancement of the decay rate by a factor of two for quantum dots in resonance with the cavity mode.
View Article and Find Full Text PDFNanocomposite materials provide the possibility for multifunctional properties in contrast with their more-limited single-component counterparts. Here, we report the synthesis and characterization of the first all-inorganic core/shell hybrid magnetic-optical nanoparticle, cobalt/cadmium selenide. The core/shell nanocrystals are prepared in a facile one-pot reaction, and their microstructure is analyzed using low- and high-resolution transmission electron microscopy.
View Article and Find Full Text PDF