Giant non-linear susceptibility of hydrogenic donors in silicon and germanium.

Implicit summation is a technique for the conversion of sums over intermediate states in multiphoton absorption and the high-order susceptibility in hydrogen into simple integrals. Here, we derive the equivalent technique for hydrogenic impurities in multi-valley semiconductors. While the absorption has useful applications, it is primarily a loss process; conversely, the non-linear susceptibility is a crucial parameter for active photonic devices.

Silicon carbide--a high-transparency nonlinear material for THz applications.

Optical properties of 4H-SiC were measured using time-domain and Fourier transform spectroscopy in the range of 0.1-20 THz. A high-transparency region was found between <0.

Broadband two-stage frequency conversion of CO laser in AgGaSe(2) crystal.

For the first time, to the best of our knowledge, a broadband two-stage frequency conversion of multiline CO laser radiation was theoretically and experimentally demonstrated in a single AgGaSe crystal. The first stage is sum frequency generation of CO laser radiation. The second stage is concurrent difference frequency generation within 4.

Dispersion properties of sulfur doped gallium selenide crystals studied by THz TDS.

High optical quality nonlinear crystals of solid solution GaSe(1-x)S(x), x=0, 0.05, 0.11, 0.

Terahertz time-domain spectroscopy for textile identification.

A range of natural and artificial textiles are examined using terahertz time-domain spectroscopy. Different types of textiles are shown to have different terahertz optical properties, which may be employed for textile identification and to combat textile counterfeiting.

Cascaded carbon monoxide laser frequency conversion into the 4.3-4.9 μm range in a single ZnGeP2 crystal.

Collinear cascaded mid-IR frequency conversion in a single nonlinear optical crystal was accomplished. Concurrent collinear generation of the sum frequency of multiline fundamental band carbon monoxide laser radiation as a first frequency conversion cascade resulted in collinear difference frequency generation within the 4.3 to 4.

Optimal Te-doping in GaSe for non-linear applications.

Centimeter-sized Te-doped GaSe ingots were grown from the charge compositions of GaSe with nominals 0.05, 0.1, 0.

Widely linear and non-phase-matched optical-to-terahertz conversion on GaSe:Te crystals.

We demonstrate the widely linear and broadband terahertz (THz) generation on GaSe:Te crystals by femtosecond laser pulses. It was found that the dopant, Te atoms, in GaSe crystals significantly enhances the efficiency of THz generation, and its central frequency can be tuned by varying the crystal thickness through non-phase-matched optical rectification. Moreover, the wide-ranging linearity for the optical-to-THz conversion and central-frequency-tunable THz generation promise for GaSe:Te crystals to be potential materials for high-power (>1.

SHG in doped GaSe:In crystals.

Optical transmission range and phase matching (PM) conditions for second harmonic generation (SHG) of Er3+:YSGG and CO2 laser in indium doped GaSe:In(0.1, 1.23, 2.

SHG phase matching in GaSe and mixed GaSe1(1-x)S(x), x < or =0.412, crystals at room temperature.

The optical properties of p-type GaSe and mixed GaSe(1-x)S(x), x=0.04, 0.023, 0.

Wide-tunable, high-energy AgGaS(2) optical parametric oscillator.

Nanosecond AgGaS(2) type-I singly resonant optical parametric oscillator pumped by a Q-switched 1.064 mum Nd:YAG laser is demonstrated experimentally. Continuously tunable 2.

Acceptable composition-ratio variations of a mixed crystal for nonlinear laser device applications.

A theory is developed to predict some crucial parameters that optimize the performance of mixed nonlinear crystals in nonlinear devices. These include acceptable variations of the composition ratio of the parent crystals and the optimal as well as acceptable interaction lengths for any interaction. The theory is successfully applied to make necessary predictions for the newly developed LiIn(Se(x)S(1-x))2 crystal for second-harmonic and optical parametric generation.