A novel device structure for thermally activated delayed fluorescence (TADF) top emission organic light-emitting diodes (TEOLEDs) that improves the viewing angle characteristics and reduces the efficiency roll-off is presented. Furthermore, we describe the design and fabrication of a cavity-suppressing electrode (CSE), Ag (12 nm)/WO (65 nm)/Ag (12 nm) that can be used as a transparent cathode. While the TADF-TEOLED fabricated using the CSE exhibits higher external quantum efficiency (EQE) and improved angular dependency than the device fabricated using the microcavity-based Ag electrode, it suffers from low color purity and severe efficiency roll-off.
View Article and Find Full Text PDFParameters such as electrode work function (WF), optical reflectance, electrode morphology, and interface roughness play a crucial role in optoelectronic device design; therefore, fine-tuning these parameters is essential for efficient end-user applications. In this study, amorphous carbon-silver (C-Ag) nanocomposite hybrid electrodes are proposed and fully characterized for solar photovoltaic applications. Basically, the WF, sheet resistance, and optical reflectance of the C-Ag nanocomposite electrode are fine-tuned by varying the composition in a wide range.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2018
Light extraction of microscale light-emitting diodes (μLEDs) is fundamentally limited by p-type metal electrodes for current injection due to the small pixel size of the LEDs. We propose Cr/Ni-doped silicon oxide (CN-SiO) films as p-type contact electrodes for blue μLEDs to increase the light-output power under the same emitting areas. The conductivity of CN-SiO electrode originates from the diffusion of top Cr/Ni atoms via electric-field-induced doping treatments, which allows for effective hole injection into the active layer.
View Article and Find Full Text PDFMicrolight-emitting diodes (µLEDs) are emerging solutions for both high-quality displays and lighting technologies. However, the overall light output power density of these devices is low, as the emission area is shielded by the p-electrodes required for current injection. In this study, instead of the more conventionally used indium tin oxide (ITO), an AlN thin film with nanoscale conducing filaments (CFs) is used, referred to as CF-AlN, as a transparent conducting electrode (TCE), to enhance the output power density from the same emission area.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2017
Many studies have set out to develop electrodes that are both highly conductive and transparent across a wide spectral region, from visible to deep UV (DUV). However, few solutions have been proposed because these two properties are mutually exclusive. In this paper, an AlN-based glass electrode film with a conducting filament formed by the application of an ac pulse is proposed as a solution, which exhibits a high transmittance in the DUV region (over 95.
View Article and Find Full Text PDFWe report the enhancement of deep ultraviolet emissions from AlGaN-based quantum wells (QWs) using energy-matched localized surface plasmons (LSPs) in platinum (Pt) nanoring arrays. The peak resonances of the extinction spectra were shifted to the red spectral region as the nanoring diameters increased, and the Pt nanorings with a diameter of 325 nm exhibited strong photoluminescence (PL) resonance at 279 nm. The emission enhancement ratio was calculated to be 304% in peak PL intensity when compared to that of the bare AlGaN QWs; this is attributed to the strong coupling of QWs with LSPs from the Pt nanorings.
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