A New Approach for the Determination of Dose Rate and Radioactivity for Detected Gamma Nuclides Using an Environmental Radiation Monitor Based on an NaI(Tl) Detector.

To expand the application of dose rate spectroscopy to the environment, the method using an environmental radiation monitor (ERM) based on a 3' × 3' NaI(Tl) detector was used to perform real-time monitoring of the dose rate and radioactivity for detected gamma nuclides in the ground around an ERM. Full-energy absorption peaks in the energy spectrum for dose rate were first identified to calculate the individual dose rates of Bi, Ac, Tl, and K distributed in the ground through interference correction because of the finite energy resolution of the NaI(Tl) detector used in an ERM. The radioactivity of the four natural radionuclides was then calculated from the in situ calibration factor-that is, the dose rate per unit curie-of the used ERM for the geometry of the ground in infinite half-space, which was theoretically estimated by Monte Carlo simulation.

Combustion/absorption process for the separation of C and H in radwastes released from nuclear power plants and their analysis.

Radioactivities of H and C in spent radioactive ion exchange resins and spent radioactive lubricant oils released from nuclear power plants, has been determined using a combustion and sorption method (combustion method). The liquid scintillation counting (LSC) spectra showed that the interference of other radionuclides has not significantly affected the determination of radioactivities of H and C in the radwaste samples. The chemical structure of CO, which originated from the combustion of radwastes, trapped C sorbent has been investigated using Fourier transform infrared spectroscopy (FT-IR).

Analysis and evaluation for consumer goods containing NORM in Korea.

We analyzed the consumer goods containing NORM by ICP-MS and evaluated the external dose. To evaluate the external dose, we assumed the small room model as irradiation scenario and calculated the specific effective dose rate using MCNPX code. The external doses for twenty goods are less than 1 mSv considering the specific effective dose rates and usage quantities.

Simultaneous Determination of the Depth of an Embedded Source and its Radioactivity in the Medium.

The simultaneous determination of the depth of an embedded source and its radioactivity in the medium at the environmental surveys is a very useful and advisable method for an in-situ gamma-ray measurement with respect to the time and cost constraint. An algorithm for the determination of the source depth and its radioactivity in the medium was developed using the information on the uncollided photon fluences and measured net count rates, which mean not scattered fluences and background subtracted count rate, at the detector positions. Uncollided photon fluences were calculated at several source depths in the medium as well as at detector positions from the Monte Carlo N-Particle (MCNP) simulation.

Validation of a procedure for the analysis of Ra in naturally occurring radioactive materials using a liquid scintillation counter.

An analytical procedure for detecting Ra in naturally occurring radioactive materials (NORMs) using a liquid scintillation counter (LSC) was developed and validated with reference materials (zircon matrix, bauxite matrix, coal fly ash, and phosphogypsum) that represent typical NORMs. The Ra was released from samples by a fusion method and was separated using sulfate-coprecipitation. Next, a Rn-emanation technique was applied for the determination of Ra.

Analytical evaluation of natural radionuclides and their radioactive equilibrium in raw materials and by-products.

An investigation into the distribution of natural radionuclides and radioactive secular equilibrium in raw materials and by-products in a domestic distribution was conducted to deduce the optimum conditions for the analytical evaluation of natural radionuclides for (238)U, (226)Ra, and (232)Th using a gamma-ray spectrometer and inductively coupled plasma mass spectrometer (ICP-MS). The range of the specific activities of natural radionuclides was first evaluated by analyzing (228)Ac and (214)Bi, which are (232)Th and (226)Ra indicators, respectively, in about 100 samples of raw materials and by-products through a gamma-ray spectrometer. From further experiments using several samples selected based on the results of the distribution of natural radionuclides, the validation of their analytical evaluations for the indirect measurements using a gamma-ray spectrometer and direct measurements using ICP-MS was assured by comparing their results.

Design and performance of an automated radionuclide separator: its application on the determination of ⁹⁹Tc in groundwater.

A modular automated radionuclide separator for (99)Tc (MARS Tc-99) has been developed for the rapid and reproducible separation of technetium in groundwater samples. The control software of MARS Tc-99 was developed in the LabView programming language. An automated radiochemical method for separating (99)Tc was developed and validated by the purification of (99m)Tc tracer solution eluted from a commercial (99)Mo/(99m)Tc generator.

Vertical distribution and characteristics of soil humic substances affecting radionuclide distribution.

The humic substances extracted from different soil depths are separated into humic (HA) and fulvic (FA) acids, and characterized for their chemical composition, proton exchange capacity, spectroscopic characteristics and binding properties to the europium ion. The chemical and spectroscopic results show that FA compared to HA has a relatively high O/C ratio, high acidic functional group contents and low aromatic contents. The synchronous fluorescence spectroscopic results show that the stability constant (K) of the soil humic substances with Eu(III) ion tends to increase as the soil depth becomes deeper, and HA has a slightly stronger binding ability than FA.

An anticoincidence-shielded gamma-ray spectrometer for analysis of low level environmental radionuclides.

We developed an ultralow-level background gamma-ray spectrometer, using active and passive shield devices at the same time. Cosmic-ray-induced background is suppressed by means of active shield devices consisting of plastic scintillating plates of 50mm thick and anti-coincidence electronic system. The observed background rate was 0.