Amplification-free GW-level, 150 W, 14 MHz, and 8 fs thin-disk laser based on compression in multipass cells.

We report an amplification-free thin-disk laser system delivering 0.9 GW peak power. The 120 fs pulses, at 14 MHz, centered around 1 µm, containing 12.

Free-space quasi-phase matching.

We report a new, to the best of our knowledge, approach to phase matching of nonlinear materials based on the free-space multipass cells. This technique is applicable to noncentrosymmetric nonlinear crystals, including crystals that cannot be birefringent phase-matched or quasi-phase matched by periodic poling. Notably, by using this approach, the crystalline quartz is quasi-phase matched with the demonstrated increase of the second harmonic generation efficiency by a factor of 40.

110 MW thin-disk oscillator.

A compact Kerr-lens mode-locked thin-disk oscillator reproducibly delivering 110 MW output peak power, the highest among all oscillators, is reported. This simple and stable femtosecond oscillator delivering a unique combination of high average power (202 W) and peak power, is an ideal driver and an important milestone for the development of extreme ultraviolet transportable frequency comb sources.

Spectral broadening in convex-concave multipass cells.

Since its first demonstration in 2016, the multi-pass spectral broadening technique has covered impressive ranges of pulse energy (3 µJ - 100 mJ) and peak power (4 MW - 100 GW). Energy scaling of this technique into the joule-level is currently limited by phenomena such as optical damage, gas ionization and spatio-spectral beam inhomogeneity. These limitations can be overcome by the novel multi-pass convex-concave arrangement, which exhibits crucial properties such as large mode size and compactness.

Few-cycle pulse compression and white light generation in cascaded multipass cells.

We report supercontinuum generation and pulse compression in two stacked multipass cells based on dielectric mirrors. The 230 fs pulses at 1 MHz containing 12 µJ are compressed by a factor of 33 down to 7 fs, corresponding to 1.0 GW peak power and overall transmission of 84%.

Scalable high-repetition-rate sub-half-cycle terahertz pulses from spatially indirect interband transitions.

Intense phase-locked terahertz (THz) pulses are the bedrock of THz lightwave electronics, where the carrier field creates a transient bias to control electrons on sub-cycle time scales. Key applications such as THz scanning tunnelling microscopy or electronic devices operating at optical clock rates call for ultimately short, almost unipolar waveforms, at megahertz (MHz) repetition rates. Here, we present a flexible and scalable scheme for the generation of strong phase-locked THz pulses based on shift currents in type-II-aligned epitaxial semiconductor heterostructures.

Dual-comb thin-disk oscillator.

Dual-comb spectroscopy (DCS) normally operates with two independent, relatively low power and actively synchronized laser sources. This hinders the wide adoption for practical implementations and frequency conversion into deep UV and VUV spectral ranges. Here, we report a fully passive, high power dual-comb laser based on thin-disk technology and its application to direct frequency comb spectroscopy.

Multipass spectral broadening and compression in the green spectral range.

Multipass spectral broadening and compression around 515 nm are experimentally demonstrated. A nonlinear multipass cell with a bulk medium is used to compress 250-fs pulses down to 38 fs. The same input pulses create a sufficient bandwidth for sub-20-fs pulse generation in a multipass cell with gaseous media.

Field-resolved infrared spectroscopy of biological systems.

The proper functioning of living systems and physiological phenotypes depends on molecular composition. Yet simultaneous quantitative detection of a wide variety of molecules remains a challenge. Here we show how broadband optical coherence opens up opportunities for fingerprinting complex molecular ensembles in their natural environment.

Intra-pulse difference-frequency generation of mid-infrared (2.7-20 μm) by random quasi-phase-matching.

We present a mid-infrared (MIR) source based on intra-pulse difference-frequency generation under the random quasi-phase-matching condition. The scheme enables the use of non-birefringent materials whose crystal orientations are not perfectly and periodically poled, widening the choice of media for nonlinear frequency conversion. With a 2 μm driving source based on a Ho:YAG thin-disk laser, together with a polycrystalline ZnSe element, an octave-spanning MIR continuum (2.

All-solid-state multipass spectral broadening to sub-20 fs.

In this work, we present a nonlinear spectral broadening and compression scheme based on self-phase modulation in bulk media inside a Herriott-type multipass cell. With this reliable approach, we achieved a spectral broadening factor of 22 while maintaining an efficiency of over 60% at an average input power of 100 W, and an excellent output beam quality with M=1.2.

Efficient High-Power Ultrashort Pulse Compression in Self-Defocusing Bulk Media.

Peak and average power scalability is the key feature of advancing femtosecond laser technology. Today, near-infrared light sources are capable of providing hundreds of Watts of average power. These sources, however, scarcely deliver pulses shorter than 100 fs which are, for instance, highly beneficial for frequency conversion to the extreme ultraviolet or to the mid- infrared.

Kerr effect in multilayer dielectric coatings.

We report the utilization of the optical Kerr effect in multilayer dielectric coatings, previously discussed only theoretically. We present the design and realization of multilayer dielectric optical structures with layer-specific Kerr nonlinearities, which permit tailoring of the intensity-dependent effects. The modulation depth in reflectance reaches up to 6% for the demonstrated examples of dielectric nonlinear multilayer coatings.

Highly-dispersive mirrors reach new levels of dispersion.

A highly-dispersive mirror with the unprecedented group delay dispersion of -10000 fs in the wavelength range of 1025-1035 nm is reported. Reproducible production of a coating with such a high dispersion was possible due to the recently developed robust synthesis technique. Successful employment of the new highly-dispersive mirror in an oscillator is demonstrated.