The pure beta emitter Sr (T = 28.8y) is a typical contaminant released by nuclear accidents and nuclear explosions. In the event of a nuclear disaster, it is crucial to identify radioactive pollutants quickly, to expedite the public's awareness of radiation exposure.
View Article and Find Full Text PDFSr and Cs activity concentrations were determined by radiometric methods in 76 soil samples (soil, litter, rain gutter deposit, and roadside sediment samples) affected by the Fukushima Dai-ichi Nuclear Power Station (FDNPS) accident and collected from the Fukushima exclusion zone. The Sr and Cs activity concentrations were in the range of 3 to 1050 Bq kg (median 82 Bq·kg) and 0.7 to 6770 kBq·kg (median 890 kBq·kg), respectively (decay correction date: March 15, 2011).
View Article and Find Full Text PDFRadiostrontium (r-Sr: Sr) is one of the primary fission products in nuclear power plants and generates liquid radioactive waste when intermixed to the aqueous matrix. Therefore, separation or preconcentration of r-Sr from the aqueous matrices is necessary for environmental monitoring or nuclear forensics. The solid-phase extraction (SPE) approach is prevalently used for r-Sr isolation and to design matrix-specific methods, while generalized SPE-assisted operating protocols are not proposed by far.
View Article and Find Full Text PDFInt J Environ Res Public Health
August 2021
Radon passive monitors based on solid state nuclear track detectors (SSNTD), especially CR-39, are widely used in radon and thoron studies. They may be subjected to the influence of external factors, like changing of temperature, humidity, and pressure, both before and during the measurement. Evaluation of the exposed detectors involves chemical processing, whose conditions also influence the measurement results.
View Article and Find Full Text PDFVarious radionuclides including fission products and heavy nuclides were released into the environment during the Fukushima Daiichi Nuclear Power Station (FDNPS) accident. The dissolution followed by migration of deposited radionuclides of Cs, Sr and U on soils could take place to the local environment. Therefore, it is necessary to determine sorption-desorption coefficients of U in soil-water system around the FDNPS from a migration viewpoint.
View Article and Find Full Text PDFIn the present study, Cs and U activity concentrations, U/U activity ratio, and U/U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg with a mean of 2007 kBq kg.
View Article and Find Full Text PDFThe Kanyakumari coastal area in the southernmost part of Tamil Nadu, India is a well-known natural high background radiation area due to the abundance of monazite in beach placer deposits. In the present study, the concentrations of major oxides, rare earth elements (REEs), Th and U were measured to understand geochemical characteristics of these monazite sands. Based on the ambient dose rate, 23 locations covering an area of about 60 km along the coast were selected for sample collection.
View Article and Find Full Text PDFThere has been tritium groundwater leakage to the land side of Fukushima Dai-ichi nuclear power plants since 2013. Groundwater was continuously collected from the end of 2013 to 2019, with an average tritium concentration of approximately 20 Bq/L. Based on tritium data published by Tokyo Electric Power Company Holdings (TEPCO) (17,000 points), the postulated source of the leakage was (1) leaks from a contaminated water tank that occurred from 2013 to 2014, or (2) a leak of tritium that had spread widely over an impermeable layer under the site.
View Article and Find Full Text PDFA novel method for the determination of ultra-trace level Sr has been recently developed applying thermal ionization mass spectrometry (TIMS). The method includes the chemical separation of Zr (isobaric interference of Zr) from the samples followed by determination of Sr/Sr abundance sensitivity (2.1 × 10).
View Article and Find Full Text PDFRadiat Prot Dosimetry
October 2019
In order to estimate occupational exposure of workers in a therapeutic radon spa facility, radon concentration in the workplace air was investigated at Markhot Ferenc Hospital, Eger, Hungary. The investigated balneotherapeutic facility and its natural hot spa water are used for treatments and rehabilitations of rheumatic patients. Radon concentration, radon decay products at a bathhouse, treatment rooms and a consultation room were continuously measured in August and September 2018.
View Article and Find Full Text PDFThe main contribution to population exposure is due to radon and thoron progenies and not radon itself. The aim of this study was therefore to estimate annual effective dose using the results of Direct Radon and Thoron Progeny Sensors were exposed in 69 selected schools and 319 dwellings in several regions of Balkans: in Serbia: regions of Sokobanja and Kosovo and Metohija, Republic of Macedonia, Republic of Srpska and Slovenia. Obtained average total effective doses are in the range from 0.
View Article and Find Full Text PDFIn this work, a new Sr analysis method was developed using the Isotopx Ltd., Phoenix X62 thermal ionization mass spectrometer (TIMS). Excellent ion beam sensitivity was demonstrated with the detection of 1 mBq (0.
View Article and Find Full Text PDFIn this study, radiocesium and K analysis were accomplished for samples of riverbed sediments and floodplain deposits collected from five rivers in the vicinity (<20 km) of the damaged Fukushima Daiichi Nuclear Power Plant after seven years of the accident. Sediment particle size distribution and major oxide content were determined also for six selected samples to understand the retention and migration process of radiocesium in river environments. The radiocesium activity concentration varied from 103 ± 6 Bq·kg to 22,000 ± 500 Bq·kg in riverbed sediments and from 92 ± 5 Bq·kg to 117,000 ± 2000 Bq·kg in floodplain deposits.
View Article and Find Full Text PDFThe radioactive fission product (90)Sr has a long biological half-life (˜18 y) in the human body. Due to its chemical similarity to calcium it accumulates in bones and irradiates the bone marrow, causing its high radio-toxicity. Assessing (90)Sr is therefore extremely important in case of a nuclear disaster.
View Article and Find Full Text PDFRadon and thoron as well as their short-lived progenies are decay products of the radium and thorium series decays. They are the most important radionuclide elements with respect to public exposure. To utilize the semiconductor pixel radiation Timepix chip for the measurement of active and real-time alpha particles from radon, thoron and their progenies, it is necessary to check the registration and visualization of the chip.
View Article and Find Full Text PDFRadiat Prot Dosimetry
November 2015
A method based on liquid scintillation counting system has been developed for the measurement of (90)Sr in Fukushima soil samples due to contamination of (134)Cs and (137)Cs. Three soil samples were collected within 30 km radius from the Fukushima Daiichi Nuclear Power Plant (FDNPP). Activity concentration of (134)Cs and (137)Cs were measured using a gamma spectroscopy system with high-purity germanium detector.
View Article and Find Full Text PDFDuring a one-year long measurement period, radon and thoron data obtained by two different passive radon-thoron discriminative monitors were compared at subsurface workplaces in Hungary, such as mines (bauxite and manganese ore) and caves (medical and touristic). These workplaces have special environmental conditions, such as, stable and high relative humidity (100%), relatively stable temperature (12°C-21°C), low or high wind speed (max. 2.
View Article and Find Full Text PDFInhalation of radon ((222)Rn) and its short-lived decay products and of products of the thoron ((220)Rn) series accounts for more than half of the effective dose from natural radiation sources. At this time, many countries have begun large-scale radon and thoron surveys and many different measurement methods and instruments are used in these studies. Consequently, it is necessary to improve and standardize technical methods of measurements and to verify quality assurance by intercomparisons between laboratories.
View Article and Find Full Text PDFExposing the Raduet Rn-Tn solid-state nuclear track detectors, radon (Rn: (222)Rn) and thoron (Tn: (220)Rn) activity concentrations have been measured in 7 kindergartens and 18 elementary schools in Slovenia. Diurnal variations of both gases were monitored using a Rad7 device. The Rn concentration was in the range from 145 to 794 Bq m(-3) in kindergartens and from 70 to 770 Bq m(-3) in schools, and the Tn concentration was in the range from 21 to 73 Bq m(-3) in kindergartens and from 4 to 91 Bq m(-3) in schools.
View Article and Find Full Text PDFRadiat Prot Dosimetry
November 2012
A new thoron ((220)Rn) experimental room (TER) was established at National Institute of Radiological Sciences in 2011 to respond to the appearance of new passive devices for (220)Rn and its progeny ((212)Pb, (212)Bi) measurement. The room volume is 21.7 m(3) with a low air exchange rate, 0.
View Article and Find Full Text PDFAt the lowest point along the tourist route in the Postojna Cave, the activity concentration of radon ((222)Rn) short-lived decay products and number concentration and size distribution of background aerosol particles in the size range of 10-1100 nm were measured. In the warm yearly season, aerosol concentration was low (52 cm(-3)) with 21 % particles smaller than 50 nm, while in the cold season, it was higher (1238 cm(-3)) with 8 % of <50 nm particles. Radon activity concentrations were 4489 and 1108 Bq m(-3), and fractions of unattached radon decay products were 0.
View Article and Find Full Text PDFRadiat Prot Dosimetry
November 2012
Radon and thoron exhalation rates and gamma-ray dose rate in different places in Hiroshima Prefecture were measured. Exhalation rates were measured using an accumulation chamber method. The radon exhalation rate was found to vary from 3 to 37 mBq m(-2) s(-1), while the thoron exhalation rate ranged from 40 to 3330 mBq m(-2) s(-1).
View Article and Find Full Text PDFOne of the essential parameters influencing of the dose conversion factor is the ratio of unattached short-lived radon progeny. This may differ from the value identified for indoor conditions when considering special workplaces such as mines. Inevitably, application of the dose conversion factors used in surface workplaces considerably reduces the reliability of dose estimation in the case of mines.
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