Coherent Control of the Rotational Degree of Freedom of a Two-Ion Coulomb Crystal.

We demonstrate the preparation and coherent control of the angular momentum state of a two-ion crystal. The ions are prepared with an average angular momentum of 7850ℏ freely rotating at 100 kHz in a circularly symmetric potential, allowing us to address rotational sidebands. By coherently exciting these motional sidebands, we create superpositions of states separated by up to four angular momentum quanta.