In situ monitoring of the electrochemically induced phase transition of thermodynamically metastable 1T-MoS at nanoscale.

1T-MoS2 is widely used in the hydrogen evolution reaction (HER) due to its abundant active sites and good conductivity. However, 1T-MoS2 is thermodynamically metastable due to the distorted crystal structure. Recently, researchers have detected the J1 and A1g Raman peaks after the HER process and confirmed that the 2H-1T phase possesses good stability.