J Phys Chem Lett
February 2020
Lead halide perovskites have been promising candidates in spintronics applications; however, the mechanism of spin relaxation is still unclear. Here, we compare the temperature-dependent spin dynamics of four perovskite films (XPbY) with different compositions (X = CHNH, Cs; Y = I, Br). The room-temperature net spin lifetime is found to increase as the molar mass decreases, indicating the dominant role of spin orbital coupling in their spin relaxation.
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