Manipulating the polarization of spin current is essential for understanding the mechanism of charge-to-spin conversion and achieving efficient electrically driven magnetization switching. Here, a novel exchange-spring magnetic structure is introduced formed by the coupling of perpendicular magnetic anisotropy (PMA) CoTb and in-plane magnetic anisotropy (IMA) Co films. When a spin current with the polarization along the y-direction flows through this exchange-spring (x-z plane) structure, the interaction between the y-spin and the local exchange field with a non-collinear spatial distribution gives rise to substantial unconventional spin polarizations in the x- and z-directions, enabling field-free spin-orbit torque driven perpendicular magnetization switching at room temperature.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
October 2024
High-voltage ultrahigh-Ni cathodes (LiNiCoMnO, x≥0.9) can significantly enhance the energy density and cost-effectiveness of Li-ion batteries beyond current levels. However, severe Li-Ni antisite defects and their undetermined dynamic evolutions during high-voltage cycling limit the further development of these ultrahigh-Ni cathodes.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2024
Increasing the charging cutoff voltage is a viable approach to push the energy density limits of LiCoO and meet the requirements of the rapid development of 3C electronics. However, an irreversible oxygen redox is readily triggered by the high charging voltage, which severely restricts practical applications of high-voltage LiCoO. In this study, we propose a modification strategy via suppressing surface ligand-to-metal charge transfer to inhibit the oxygen redox-induced structure instability.
View Article and Find Full Text PDFAll-Mn-based Li-rich cathodes Li MnO have attracted extensive attention because of their cost advantage and ultrahigh theoretical capacity. However, the unstable anionic redox reaction (ARR), which involves irreversible oxygen releases, causes declines in cycling capacity and intercalation potential, thus hindering their practical applications. Here, it is proposed that introducing stacking-fault defects into the Li MnO can localize oxygen lattice evolutions and stabilize the ARR, eliminating oxygen releases.
View Article and Find Full Text PDFIEEE Trans Neural Netw Learn Syst
September 2023
Exponential function is a basic form of temporal signals, and how to fast acquire this signal is one of the fundamental problems and frontiers in signal processing. To achieve this goal, partial data may be acquired but result in severe artifacts in its spectrum, which is the Fourier transform of exponentials. Thus, reliable spectrum reconstruction is highly expected in the fast data acquisition in many applications, such as chemistry, biology, and medical imaging.
View Article and Find Full Text PDFChem Commun (Camb)
October 2021
By using temperature-dependent neutron powder diffraction combined with maximum entropy method analysis, a previously unreported Li lattice site was discovered in the argyrodite LiPSCl solid-state electrolyte. This new finding enables a more complete description of the Li diffusion model in argyrodites, providing structural guidance for designing novel high-conductivity solid-state electrolytes.
View Article and Find Full Text PDFDynamic nuclear polarization (DNP) can provide a powerful means to amplify neutron diffraction from biological crystals by 10-100-fold, while simultaneously enhancing the visibility of hydrogen by an order of magnitude. Polarizing the neutron beam and aligning the proton spins in a polarized sample modulates the coherent and incoherent neutron scattering cross-sections of hydrogen, in ideal cases amplifying the coherent scattering by almost an order of magnitude and suppressing the incoherent background to zero. This chapter describes current efforts to develop and apply DNP techniques for spin polarized neutron protein crystallography, highlighting concepts, experimental design, labeling strategies and recent results, as well as considering new strategies for data collection and analysis that these techniques could enable.
View Article and Find Full Text PDFSheng Wu Yi Xue Gong Cheng Xue Za Zhi
April 2017
The present study was carried out with the surface electromyography signal of subjects during the time when subjects did the exercises of the 6 core stability trainings. We analyzed the different activity level of surface electromyography signal, and finally got various fatigue states of muscles in different exercises. Thirty subjects completed exercises of 6 core stability trainings, which were prone bridge, supine bridge, unilateral bridge (divided into two trainings, the left and right sides alternatively) and bird-dog (divided into two trainings, the left and right sides alternatively), respectively.
View Article and Find Full Text PDFEzrin is a member of the ezrin-radixin-moesin family (ERM) of adapter proteins that are localized at the interface between the cell membrane and the cortical actin cytoskeleton, and they regulate a variety of cellular functions. The structure representing a dormant and closed conformation of an ERM protein has previously been determined by x-ray crystallography. Here, using contrast variation small angle neutron scattering, we reveal the structural changes of the full-length ezrin upon binding to the signaling lipid phosphatidylinositol 4,5-bisphosphate (PIP(2)) and to F-actin.
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