Expression of concern for 'Surface modification engineering of two-dimensional titanium carbide for efficient synergistic multitherapy of breast cancer' by Lei Bai , , 2020, , 6402-6417, https://doi.org/10.1039/D0TB01084G.
View Article and Find Full Text PDFMaterials (Basel)
June 2024
With the wide application of laser weapons, the requirements of laser protection technology are becoming more and more strict. Therefore, it is important to find ideal optical limiting (OL) materials to protect human eyes and detectors. In this work, the nonlinear optical responses of gold nanoparticles/porous carbon (Au NPs/PC) nanocomposites prepared by the reduction method were studied using the nanosecond Z-scan technique.
View Article and Find Full Text PDFTwo-dimensional molybdenum disulfide (MoS) has been proven to be a candidate in photodetectors, and MoS/lead sulfide (PbS) quantum dots (QDs) heterostructure has been used to expand the optical response wavelength of MoS. Time-resolved pump-probe transient absorption measurements are performed to clarify the carrier transfer dynamics in the MoS/PbS heterostructure. By comparing the carrier dynamics in MoS and MoS/PbS under different pump wavelengths, we found that the excited electrons in PbS QDs can transfer rapidly (<100 fs) to MoS, inducing its optical response in the near-infrared region, although the pump light energy is lower than the bandgap of MoS.
View Article and Find Full Text PDFApplications of the type-I fiber Bragg gratings (FBGs) written through the coating (TTC) in strain sensing and tunable distributed Bragg reflector (DBR) fiber lasers were demonstrated. We reported the principle of selecting the distance between the fiber and the phase mask when writing type-I TTC FBGs. Type-I TTC FBGs written in commercially available acrylate-coated fibers with various geometries and their strain responses were demonstrated.
View Article and Find Full Text PDFAll-inorganic lead halide perovskite nanocrystals (NCs) have been widely applied in optoelectronic devices owing to their excellent photoluminescence (PL) properties. However, poor stability upon exposure to water, UV light or heat strongly limits their practical application. Herein, CsPbBr@Pb-MOF composites with exceptional stability against water, UV light, and heat are synthesized by ultrasonic processing the precursors of lead-based MOF (Pb-MOF), oleylammonium bromide (OAmBr) and cesium oleate (Cs-OA) solutions at room temperature.
View Article and Find Full Text PDFWe demonstrate a single longitudinal mode distributed Bragg reflection (DBR) fiber laser by directly fabricating fiber Bragg gratings (FBGs) on an ytterbium-doped fiber (YDF) using a femtosecond laser. A simple optical self-injection feedback method was used to effectively compress the linewidth and reduce relative intensity noise (RIN) of a single longitudinal mode DBR fiber laser. Further, we investigated the effect of self-injection feedback cavity length and reflectivity on linewidth compression and determined that the linewidth tends to decrease with the increase of the external cavity photon lifetime.
View Article and Find Full Text PDFWith the wide application of intense lasers, the protection of human eyes and detectors from laser damage is becoming more and more strict. In this paper, we study the nonlinear optical limiting (OL) properties of porous carbon with a super large specific surface area (2.9 × 10 m/g) using the nanosecond Z-scan technique.
View Article and Find Full Text PDFBy controlling the 800 nm fs laser energy and applying an isopropyl alcohol environment, controlled sub-diffraction limited lithography with a characteristic structure of approximately 30 nm was achieved on the surface of diamond films, and diamond gratings with a period of 200 nm were fabricated. The fabrication of single grooves with a feature size of 30 nm demonstrates the potential for patterning periodic or nonperiodic structures, and the fabrication of 200 nm periodic grating structures demonstrates the ability of the technique to withstand laser proximity effects. This enhances the technology of diamond film nanofabrication and broadens its potential applications in areas such as optoelectronics and biology.
View Article and Find Full Text PDFEnergy transfer has been proven to be an effective method to optimize optoelectronic conversion efficiency by improving light absorption and mitigating nonradiative losses. We prepared 2D/3D CsPbBr3 hybrid assemblies at different reaction temperatures using the hot injection method and found that the photoluminescence quantum yields (PLQYs) of these hybrids were greatly enhanced from 53.4% to 72.
View Article and Find Full Text PDFPhotoinduced excited-state carriers can affect both the absorption coefficient and refractive index of materials and influence the performance of photoelectric devices. Femtosecond time-resolved pump-probe transient absorption (TA) spectroscopy is usually used to detect carrier dynamics and excited-state absorption coefficients; however, measurements of transient refractive-index change are still difficult. We propose a method for determining the excited-state refractive-index change using TA microscopy.
View Article and Find Full Text PDFWe demonstrated a new method of fabricating a stretchable antenna by injecting liquid metal (LM) into a femtosecond-laser-ablated embedded hydrogel microchannel, and realized miniaturization of a stretchable dipole antenna based on hydrogel substrate. Firstly, symmetrical microchannels with two equal and linear branches were formed by a femtosecond laser in the middle of a hydrogel substrate, and then were filled with LM by use of a syringe needle. Using this method, a stretchable LM-dipole antenna with each dimension of 24 mm × 0.
View Article and Find Full Text PDFLead halide perovskites (LHPs) have excellent semiconductor properties. They have been used in many applications such as solar cells. Recently, the hot carrier dynamics in this type of material have received much attention as they are useful for enhancing the performance of optoelectrical devices fabricated from it.
View Article and Find Full Text PDFThe advancement of carbon-based electronics is reliant on the development of semiconducting carbon nanotubes with high purity and yield. We developed a new extraction strategy to efficiently sort SWCNTs with superior yields and purity. The approach uses two polymers, poly[N-(1-octylnonyl)-9H-carbazol-2,7-diyl](PCz) and poly(9,9-n-dihexyl-2,7-fluorene-alt-9-phenyl-3,6-carbazole)(PDFP), and two sonication processes to eliminate surface polymer contamination.
View Article and Find Full Text PDFWe studied the application of the fiber Bragg grating (FBG) temperature sensing method based on support vector regression optimized by a genetic algorithm (GA-SVR) for constant and decreasing external ambient temperature cases by simulation. The external ambient temperature could be retrieved from both the transient FBG wavelength and its corresponding change rate using GA-SVR, before the FBG temperature sensor reached the thermal equilibrium state with the external ambient temperature. FBG wavelengths and their corresponding change rates in the cases of FBG sensor temperatures higher and lower than the external ambient temperature were studied and used to construct the training data set.
View Article and Find Full Text PDF"Naked" ferroferric-oxide nanoparticles (FONPs) synthesized by a femtosecond laser ablation on a bulk stainless steel in liquid were applied to the Nd: YVO laser to achieve passive Q-switched pulse laser output. Without the pollution of ligand, the inherent light characteristic of "naked" FONPs was unaffected. The analysis of the morphological characteristics, dominant chemical elements, and phase composition of the FONPs showed that they were mainly composed of FeO, which was spherical with an average diameter of 40 nm.
View Article and Find Full Text PDFIn this study, the time-spatial evolution of single-pulse femtosecond laser-induced plasma in sapphire is studied by using femtosecond time-resolved pump-probe shadowgraphy. Laser-induced sapphire damage occurred when the pump light energy was increased to 20 µJ. Based on its shadowgraphy image, the threshold electron density can be estimated to be about 2.
View Article and Find Full Text PDFUltrafast fiber lasers combining high peak power and excellent beam quality in the 1-µm wavelength range have been explored to applications in industry, medicine and fundamental science. Here, we report generation of a high-energy sub 300 fs polarization maintaining fiber chirped pulse amplification (CPA) system by using a Yb-doped large mode area tapered polarization maintaining (PM) optical fiber with the core/cladding diameters of 35/250 µm at the thin end and 56/400 µm at the thick end. The taper fiber design features a confined core for selective gain amplification and multi-layer cladding for enhanced suppression of higher order modes.
View Article and Find Full Text PDFWe propose an ultra-high-temperature sensing method using a fiber Bragg grating (FBG) and demodulation technique based on support vector regression optimized by a genetic algorithm (GA-SVR). A type-I FBG inscribed by a femtosecond laser in a silica fiber was packaged with a tube and used as a temperature sensor. The external ambient temperature was retrieved from the transient FBG wavelength and its increase rate in reaching thermal equilibrium of the FBG with the external environment using GA-SVR.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2022
The electromagnetic induced transparency (EIT) effect originates from the destructive interference in an atomic system, which contributes to the transparency window in its response spectrum. The implementation of EIT requires highly demanding laboratory conditions, which greatly limits its acceptance and application. In this paper, an improved harmonic spring oscillation (HSO) model with four oscillators is proposed as a classical analog for the tunable triple-band EIT effect.
View Article and Find Full Text PDFNanomaterials (Basel)
October 2022
The excellent performance of InP/ZnSe/ZnS core/shell/shell quantum dots (CSS-QDs) in light-emitting diodes benefits from the introduction of a ZnSe midshell. Understanding the changes of ultrafast carrier dynamics caused by the ZnSe midshell is important for their optoelectronic applications. Herein, we have compared the ultrafast carrier dynamics in CSS-QDs and InP/ZnS core/shell QDs (CS-QDs) using femtosecond transient absorption spectroscopy.
View Article and Find Full Text PDFNonlinear optical limiting (OL) properties of carboxyl-functionalized TiC nanosheets (COOH-MXene) were studied using the nanosecond laser Z-scan technology. COOH-MXene showed excellent broadband OL properties with OL thresholds of 0.34 J/cm at 532 nm and 0.
View Article and Find Full Text PDFA simple method of fabricating (- (PMN-PT) deep grooves with high aspect ratios using an 800-nm femtosecond laser with chemical-selective etching is demonstrated. The 567-µm-deep grooves with aspect ratios of approximately 35 were obtained with no cracks or thermal affected zone. The morphologies and chemical compositions of grooves were analyzed by a scanning electron microscope with an energy dispersive x-ray spectrometer.
View Article and Find Full Text PDFInP/ZnS core/shell quantum dots have shown extraordinary application potential in photocatalysis. In this work, we demonstrated by ultrafast spectroscopy that the electron transfer ability of InP/ZnSe/ZnS core/shell/shell quantum dots was better than that of InP/ZnS quantum dots, because the introduction of ZnSe midshell resulted in improved passivation and greater exciton delocalization. The temperature-dependent PL spectra indicate that the exciton-phonon coupling strength and exciton binding energy of InP/ZnSe/ZnS quantum dots are smaller than those of InP/ZnS quantum dots.
View Article and Find Full Text PDFCoronavirus disease (COVID-19) is a pandemic that has caused thousands of casualties and impacts all over the world. Most countries are facing a shortage of COVID-19 test kits in hospitals due to the daily increase in the number of cases. Early detection of COVID-19 can protect people from severe infection.
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