Publications by authors named "Jingkai Qin"

Featuring the capabilities of self-power, low dark current, and broadband response, photothermoelectric (PTE) detection demonstrates great potential for application in the military and civilian fields. The development of materials with an intrinsically high efficiency for PTE energy conversion and the in-depth study of its thermoelectric properties on the device performance are of great significance. Here, we reported a quasi-one-dimensional (quasi-1D) van der Waals (vdW) TaSe crystal as a promising material candidate for PTE detection.

View Article and Find Full Text PDF

Intelligent neuromorphic hardware holds considerable promise in addressing the growing demand for massive real-time data processing in edge computing. Resistive switching materials with intrinsic anisotropy and a compact design of non-volatile memory devices with the capability of handling spatiotemporally reconstructed data is crucial to perform sophisticated tasks in complex application scenarios. In this study, an anisotropic resistive switching cell with a planar configuration based on lithiated NbSe nanosheets is demonstrated.

View Article and Find Full Text PDF

Perovskite thin-film transistors (TFTs) simultaneously possessing exceptional carrier transport capabilities, nonvolatile memory effects, and photosensitivity have recently attracted attention in fields of both complementary circuits and neuromorphic computing. Despite continuous performance improvements through additive and composition engineering of the channel materials, the equally crucial dielectric/channel interfaces of perovskite TFTs have remained underexplored. Here, it is demonstrated that engineering the dielectric/channel interface in 2D tin perovskite TFTs not only enhances the performance and operational stability for their utilization in complementary circuits but also enables efficient synaptic behaviors (optical information sensing and storage) under an extremely low operating voltage of -1 mV at the same time.

View Article and Find Full Text PDF
Article Synopsis
  • A high vacuum flavor extraction (HVE) device was developed to overcome the drawbacks of traditional extraction methods, which can take a long time and create unwanted by-products at high temperatures.
  • The HVE method showed reliable results in quantitative tests, achieving a mean relative standard deviation of 11.60% and a recovery rate of 90.55%, indicating its precision and effectiveness.
  • When comparing HVE to other methods like solvent-assisted flavor evaporation (SAFE) and simultaneous distillation-extraction (SDE), HVE was found to be superior in extracting key flavor compounds, with sensory evaluations revealing it produced odor profiles most similar to the original fried tilapia sample.
View Article and Find Full Text PDF

A two-dimensional (2D) ferroelectric semiconductor, which is coupled with photosensitivity and room-temperature ferroelectricity, provides the possibility of coordinated conductance modulation by both electric field and light illumination and is promising for triggering the revolution of optoelectronics for monolithic multifunctional integration. Here, we report that semiconducting SnPS crystals can be achieved in a 2D morphology using a chemical vapor transport approach with the assistant of space confinement and experimentally demonstrate the robust ferroelectricity in atomic-thin SnPS nanosheet at room temperature. The intercorrelated programming of ferroelectric order along out-of-plane (OOP) and in-plane (IP) directions enables a tunable bulk photovoltaic (BPV) effect through multidirectional electrical control.

View Article and Find Full Text PDF

BiOSe has attracted intensive attention due to its potential in electronics, optoelectronics, and ferroelectric applications. Despite that, there have only been a handful of experimental studies based on ultrafast spectroscopy to elucidate the carrier dynamics in BiOSe thin films. Besides, different groups have reported various ultrafast timescales and associated mechanisms across films of different thicknesses.

View Article and Find Full Text PDF

A promising and efficacious approach to manage diabetes is inhibiting α-glucosidase and α-amylase activity. Therefore, the inhibitory activities of five natural sweeteners (mogrosides (Mog), stevioside (Ste), glycyrrhizinic acid (GA), crude trilobatin (CT), and crude rubusoside (CR)) against α-glucosidase and α-amylase and their interactions were evaluated using enzyme kinetics, fluorescence spectroscopy, Fourier infrared spectroscopy, and molecular docking. The inhibitor sequence was CT > GA > Ste, as GA competitively inhibited α-glycosidase activity while CT and Ste exhibited mixed inhibitory effects.

View Article and Find Full Text PDF

Neuro-inspired vision systems hold great promise to address the growing demands of mass data processing for edge computing, a distributed framework that brings computation and data storage closer to the sources of data. In addition to the capability of static image sensing and processing, the hardware implementation of a neuro-inspired vision system also requires the fulfilment of detecting and recognizing moving targets. Here, we demonstrated a neuro-inspired optical sensor based on two-dimensional NbS/MoS hybrid films, which featured remarkable photo-induced conductance plasticity and low electrical energy consumption.

View Article and Find Full Text PDF

Memristive devices operating analogous to biology synapses demonstrate great potential for neuromorphic applications. Here, we reported the space-confined vapor synthesis of ultrathin titanium trisulfide (TiS) nanosheets, and subsequent laser manufacturing of a TiS-TiO-TiS in-plane heterojunction for memristor applications. Due to the flux-controlled migration and aggregation of oxygen vacancies, the two-terminal memristor demonstrates reliable "analog" switching behaviors, in which the channel conductance can be incrementally adjusted by tuning the duration and sequence of programming voltage.

View Article and Find Full Text PDF

Two-dimensional (2D) layered semiconductors with nonlinear optical (NLO) properties hold great promise to address the growing demand of multifunction integration in electronic-photonic integrated circuits (EPICs). However, electronic-photonic co-design with 2D NLO semiconductors for on-chip telecommunication is limited by their essential shortcomings in terms of unsatisfactory optoelectronic properties, odd-even layer-dependent NLO activity and low NLO susceptibility in telecom band. Here we report the synthesis of 2D SnPSe, a van der Waals NLO semiconductor exhibiting strong odd-even layer-independent second harmonic generation (SHG) activity at 1550 nm and pronounced photosensitivity under visible light.

View Article and Find Full Text PDF

Mixed-dimensional van der Waals (vdW) integration has been demonstrated to be effective for the modulation of the physical properties of homogeneous materials. Herein, we reported the enhancement of photothermal conversion and decrease of thermal conductivity in metallic single-walled carbon nanotube (SWCNT) films with the integration of chemical vapor deposition-grown monolayer MoS films. The induced temperature gradient in SWCNT-MoS hybrid films drives carrier diffusion to generate photocurrent the photothermoelectric (PTE) effect, and a self-powered photodetector working in the visible band range from 405 to 785 nm was demonstrated.

View Article and Find Full Text PDF
Article Synopsis
  • * The research introduces a new material, LiNiMnO, which maintains structural stability through a medium-entropy spinel phase and utilizes improved lithium ion movement and charge compensation mechanisms after initial delithiation.
  • * Testing of LiNiMnO shows promising results in a coin cell configuration, achieving a discharge capacity of 314.1 mA h g and an initial specific energy of 999.3 Wh kg at a voltage of about 3.2 V, indicating potential for better performance in lithium batteries.
View Article and Find Full Text PDF

2D van der Waals (vdW) semiconductors hold great potentials for more-than-Moore field-effect transistors (FETs), and the efficient utilization of their theoretical performance requires compatible high-k dielectrics to guarantee the high gate coupling efficiency. The deposition of traditional high-k dielectric oxide films on 2D materials usually generates interface concerns, thereby causing the carrier scattering and degeneration of device performance. Here, utilizing a space-confined epitaxy growth approach, the authors successfully obtained air-stable ultrathin indium phosphorus sulfide (In P S ) nanosheets, the thickness of which can be scaled down to monolayer limit (≈0.

View Article and Find Full Text PDF

Two-dimensional (2D) trigonal selenium (-Se) has become a new member in 2D semiconducting nanomaterial families. It is composed of well-aligned one-dimensional Se atomic chains bonded via van der Waals (vdW) interaction. The contribution of this unique anisotropic nanostructure to its mechanical properties has not been explored.

View Article and Find Full Text PDF
Article Synopsis
  • Two-dimensional (2D) materials are widely researched for their diverse functionalities, and integrating one-dimensional (1D) atomic crystals with these 2D materials leads to mixed-dimensional heterostructures with unique physical properties.
  • The review covers methods for fabricating these heterostructures and highlights their exciting physical phenomena, such as high optical absorption and efficient charge transfer, which enhance their performance in various applications.
  • Potential uses discussed include electronic devices, optoelectronic devices, photonic devices, spintronic devices, and gas sensors, along with an outlook on future opportunities and challenges in this field.
View Article and Find Full Text PDF

2D organic crystals exhibit efficient charge transport and field-effect characteristics, making them promising candidates for high-performance nanoelectronics. However, the strong Fermi level pinning (FLP) effect and large Schottky barrier between organic semiconductors and metals largely limit device performance. Herein, by carrying out temperature-dependent transport and Kelvin probe force microscopy measurements, it is demonstrated that the introducing of 2D metallic 1T-TaSe with matched band-alignment as electrodes for F CuPc nanoflake filed-effect transistors leads to enhanced field-effect characteristics, especially lowered Schottky barrier height and contact resistance at the contact and highly efficient charge transport within the channel, which are attributed to the significantly suppressed FLP effect and appropriate band alignment at the nonbonding van der Waals (vdW) hetero-interface.

View Article and Find Full Text PDF

Hardware implementation of an artificial neural network requires neuromorphic devices to process information with low energy consumption and high heterogeneity. Here we demonstrate an electrolyte-gated synaptic transistor (EGT) based on a trigonal selenium (-Se) nanosheet. Due to the intrinsic low conductivity of the Se channel, the -Se synaptic transistor exhibits ultralow energy consumption, less than 0.

View Article and Find Full Text PDF

Red-spotted grouper (Epinephelus akaara) is one of the high economic value grouper species, however, the knowledge regarding its growth is limited. In this study, full-length cDNAs of growth hormone (gh) and its receptors (ghr1 and ghr2) were cloned from the pituitary and liver of red-spotted grouper, respectively. Tissue distribution analysis showed that gh mRNA was predominantly expressed in the pituitary.

View Article and Find Full Text PDF

Deteriorating water quality, especially from high concentrations of nitrite, is currently largely blamed for disease outbreaks in farmed tilapia (Oreochromis niloticus). In this study, the underlying mechanism of nitrite on the susceptibility of tilapia leucocytes to Streptococcus agalactiae (S. agalactiae) was studied.

View Article and Find Full Text PDF

Growth hormone is a hormone secreted from the pituitary and is involved in the regulation of most major physiological processes such as growth, development and metabolism. Therefore, an accurate and sensitive detection method is needed for the detection of tilapia serum Gh level. Phage display technology is widely used in the expression of antibody fragments, in which fragments of antibodies are expressed as a fusion with phage proteins and are displayed on the phage surface for easy screening.

View Article and Find Full Text PDF

Background: Compensatory growth refers to the phenomenon in which organisms grow faster after the improvement of an adverse environment and is thought to be an adaptive evolution to cope with the alleviation of the hostile environment. Many fish have the capacity for compensatory growth, but the underlying cellular mechanisms remain unclear. In the present study, microarray and nontargeted metabolomics were performed to characterize the transcriptome and metabolome of zebrafish liver during compensatory growth.

View Article and Find Full Text PDF

A material with reversible temperature change capability under an external electric field, known as the electrocaloric effect (ECE), has long been considered as a promising solid-state cooling solution. However, electrocaloric (EC) performance of EC materials generally is not sufficiently high for real cooling applications. As a result, exploring EC materials with high performance is of great interest and importance.

View Article and Find Full Text PDF

The insulin-like growth factor (IGF) system plays a pivotal role in the regulation of growth, and IGF binding proteins (IGFBPs) are important regulatory factors in the IGF system. Generally, IGFBPs inhibit IGF actions by preventing its binding to receptors. Under some conditions, the IGFBPs can also enhance IGF actions.

View Article and Find Full Text PDF

As the close paralog of adiponectin, C1q/TNF-Related Protein 9 (CTRP9) has been reported to be involved in the regulation of glucose and fat metabolism, immunization and endothelial cell functions. However, information regarding the actions of Ctrp9 on reproduction is extremely limited in fish. As a first step, Ctrp9, adiponectin receptor 1 (Adipor1) and Adipor2 were identified from Nile tilapia.

View Article and Find Full Text PDF

Gonadotropin-inhibitory hormone (GnIH), a novel hypothalamic neuropeptide, serves as a key player in the regulation of reproduction across vertebrates, acting on the brain and pituitary to modulate reproductive physiology and behavior. However, little information is available in teleosts regarding the intracellular signal transduction pathway in response to GnIH. To this end, we first cloned the gene of LPXRFa (the piscine ortholog of GnIH) receptor in the half-smooth tongue sole (Cynoglossus semilaevis), a representative species of the order Pleuronectiformes.

View Article and Find Full Text PDF