Alkaline anaerobic fermentation (AAF) of waste activated sludge (WAS) has been demonstrated to be promising for short-chain fatty acids (SCFAs) recovery. However, high-strength metals and EPSs in the landfill leachate-derived WAS (LL-WAS) would stabilize its structure, suppressing AAF performance. To improve sludge solubilization and SCFAs production, AAF was coupled with EDTA addition for LL-WAS treatment.
View Article and Find Full Text PDFAnaerobic ammonium oxidation (anammox) coupled with hydroxyapatite (HAP) crystallization not only achieves simultaneous nitrogen removal and phosphorus recovery, but also cultivates excellent anammox granules. However, a floatation and wash-out of anammox-HAP granules was occurred at low phosphate concentrations. In this study, a reactor inoculated with mature anammox-HAP granules and fed with low phosphate (5 mg P/L) was added with granular activated carbon (GAC) to maintain sludge granulation and nitrogen-removing stability.
View Article and Find Full Text PDFPartial nitrification-anammox process is promising in leachate treatment, but the 11% residue nitrate limits the total nitrogen removal efficiency. Denitrification or partial denitrification and anammox are both practical polishing processes of anammox effluent, requiring extra electron donors. Fortunately, there are organic matter, sulfide and methane in leachate or produced by leachate treatment, which can serve as onsite electron donors.
View Article and Find Full Text PDFPhosphorus recovery from municipal sewage sludge is a promising way to alleviate the shortage of phosphorus resources. However, the recovery efficiency and cost depend greatly on phosphorus species and fractions in different sewage sludges, i.e.
View Article and Find Full Text PDFWastewater treatment plants face the problem of a shortage of carbon source for denitrification. Acidogenic fermentation is an effective method for recovering short-chain fatty acids (SCFAs) as a carbon source from sewage sludge. Herein, the most recent advances in SCFAs production from primary sludge and waste activated sludge are systematically summarised and discussed.
View Article and Find Full Text PDFAlkaline fermentation of waste activated sludge (WAS) to produce short-chain fatty acids (SCFAs) has been proved to be promising to develop internal carbon source for denitrifying processes in municipal wastewater treatment plants. However, a large amount of ammoniacal nitrogen also releases during fermentation, resulting in inhibition of acidogenic process and reduction of carbon source availability. Alkaline fermentation of WAS combined with in-situ ammonia stripping was proposed to improve SCFAs production and carbon source availability simultaneously.
View Article and Find Full Text PDFGiven our vast methane reserves and the forecasted shortage of crude oil in the not too distant future, the conversion of methane into value-added liquid chemicals or fuels would be beneficial. The generated chemicals or fuels could augment the petroleum-dominated chemical market, and also satisfy the increasing demand for transportation fuels. While methane bioconversion to liquid chemicals has just been reported recently, there is limited understanding of the process.
View Article and Find Full Text PDFIt has been reported that microbial reduction of sulfate, nitrite/nitrate and iron/manganese could be coupled with anaerobic oxidation of methane (AOM), which plays a significant role in controlling methane emission from anoxic niches. However, little is known about microbial chromate (Cr(VI)) reduction coupling with AOM. In this study, a microbial consortium was enriched via switching nitrate dosing to chromate feeding as the sole electron acceptor under anaerobic condition in a membrane biofilm reactor (MBfR), in which methane was continuously provided as the electron donor through bubble-less hollow fiber membranes.
View Article and Find Full Text PDFPerchlorate has been widely detected in various water environments and could cause serious health problems. Methane has been proposed as a promising electron donor to remove perchlorate from contaminated water, yet it is unclear whether and how microbial methane oxidation couples with perchlorate reduction, in particular under anoxic conditions. Here, the feasibility and performance of perchlorate reduction driven by methane in the presence and absence of oxygen were investigated and compared in a lab-scale methane-based membrane biofilm reactor.
View Article and Find Full Text PDFEnviron Sci Technol
April 2018
Anaerobic oxidation of methane (AOM) plays a crucial role in controlling the flux of methane from anoxic environments. Sulfate-, nitrite-, nitrate-, and iron-dependent methane oxidation processes have been considered to be responsible for the AOM activities in anoxic niches. We report that nitrate-reducing AOM microorganisms, enriched in a membrane biofilm bioreactor, are able to couple selenate reduction to AOM.
View Article and Find Full Text PDFThe discovery of denitrifying anaerobic methane oxidation (DAMO) has not only improved our understanding of global methane and nitrogen cycles, but also provided new technology options for removal of nitrate from nitrate-contaminated water. Previous studies have demonstrated DAMO organisms could remove nitrate and nitrite from wastewater under strictly anaerobically conditions. In the study, we investigate the feasibility of nitrate removal from groundwater, which contains dissolved oxygen in addition to nitrate.
View Article and Find Full Text PDFWaste activated sludge (WAS) was pretreated by acid or alkali to enhance the anaerobic fermentation (AF) for phosphorus (P) and short-chain fatty acids (SCFAs) release into the liquid simultaneously. With acid pretreatment, the released total P concentration achieved 120mg/L, which was 71.4% higher than that with alkali pretreatment.
View Article and Find Full Text PDFThe performance of a granule-based partial nitritation-anammox process is expected to be affected by the granule size distribution, but little is known about the impact of granule size on microbial community structure and diversity. To reveal how the microbial composition and diversity vary with granule size, granules from a partial nitritation-anammox reactor were size-fractionated into five classes (<0.2, 0.
View Article and Find Full Text PDFBiogas, generated from an expanded granular sludge bed (EGSB) reactor treating municipal solid waste (MSW) leachate, was recirculated for calcium removal from the leachate via a carbonation process with simultaneous biogas purification. Batch trials were performed to optimize the solution pH and imported biogas (CO2) for CaCO3 precipitation. With applicable pH of 10-11 obtained, continuous trials achieved final calcium concentrations of 181-375 mg/L (removal efficiencies≈92.
View Article and Find Full Text PDFNitrate reduction by zero-valent iron (Fe(0)) powder always works well only at controlled pH lower than 4 due to the formation of iron (hydr)oxides on its surface. Fe(0) powder combined with activated carbon (AC), i.e.
View Article and Find Full Text PDFA novel integrated internal and external circulation (IIEC) reactor was developed for anaerobic biodegradation of municipal solid waste (MSW) fresh leachate with chemical oxygen demand (COD) between 40,000 and 60,000mg/l. The pilot-scale IIEC reactor was inoculated with two kinds of granular sludge from paper mill (SPM) and from citric acid factory (SCF), respectively. The bio-treating capacity in contaminant removal and biogas production performed much superior to others' results, principally attributed to appropriate configuration modification.
View Article and Find Full Text PDFThe inhibitory effect of high-strength NH(3)-N on anaerobic biodegradation of landfill leachates in an EGSB bioreactor has been investigated. The research compared start-up performance of the reactor treating the landfill leachate with NH(3)-N in 242-1200 mg/l to that treating the compost leachate with NH(3)-N in 38-410 mg/l. The observations showed that the performance of the reactor treating the landfill leachate was only marginally worse than that treating the compost leachate at the mesophilic temperature when NH(3)-N concentration was under 1500 mg/l.
View Article and Find Full Text PDFThis research investigated the calcium effect on the anaerobic treatment of fresh leachate in an expanded granular sludge bed (EGSB) bioreactor under mesophilic conditions. The observations show that the bioreactor, inoculated with anaerobic granular sludge, can be started up only in about 40 days for the treatment of calcium-containing fresh leachate with chemical oxygen demand (COD) removal efficiency above 90% and organic loading rate up to 72.84 kg COD/m(3) day.
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