The structure of a nanocatalyst during electrocatalytic reactions often deviates from its pristine structure due to intrinsic properties, or physical and chemical adsorption at the catalytic surfaces. Taking Cu-based catalysts for CO electroreduction reactions (CORR) as an example, they often experience segregation, leaching, and alloying during reactions. With the recent breakthrough development of high-resolution polymer electrochemical liquid cells, electrochemical liquid cell transmission electron microscopy (EC-TEM) alongside other advanced microscopy techniques, has become a powerful platform for revealing electrocatalysts restructuring at the atomic level.
View Article and Find Full Text PDFACS Appl Mater Interfaces
August 2024
In this work, a superhydrophobic surface loaded with elliptical superhydrophilic patterns in a V-shaped arrangement has been fabricated with the help of shape memory membranes with uniform vertically penetrative channels (i.e., SMEUVs, as a mask).
View Article and Find Full Text PDFDeveloping efficient and economical electrocatalysts for acidic oxygen evolution reaction (OER) is essential for proton exchange membrane water electrolyzers (PEMWE). Cobalt oxides are considered promising non-precious OER catalysts due to their high activities. However, the severe dissolution of Co atoms in acid media leads to the collapse of crystal structure, which impedes their application in PEMWE.
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