Polarization Dependence of Charge Conduction in Conjugated Polymer Films Investigated with Time-Resolved Terahertz Spectroscopy.

Room temperature Time-Domain Terahertz (TDS) and Time-Resolved Terahertz (TRTS) spectroscopic methods are employed to measure carrier mobility and charge generation efficiency in thin-film semiconductor polymers. Interrogation of the dependence on excitation and probe polarizations yields insight into the underlying material properties that guide charge transport. We apply THz polarization anisotropy probes to analyze charge conduction in preparations of the copolymer PCDTPT, consisting of alternating cyclopenta-dithiophene (donor) and thiadiazolo-pyridine (acceptor) units.

Pulse dynamics in mode-locked lasers: relaxation oscillations and frequency pulling.

A theoretical description of the pulse dynamics in a modelocked laser including gain dynamics is developed. Relaxation oscillations and frequency pulling are predicted that influence the pulse parameters. Experimental observations of the response of a mode-locked Ti:sapphire laser to an abrupt change in the pump power confirm that the predicted behavior occurs.

Optical Frequency Metrology of an Iodine-Stabilized He-Ne Laser Using the Frequency Comb of a Quantum-Interference-Stabilized Mode-Locked Laser.

We perform optical frequency metrology of an iodine-stabilized He-Ne laser using a mode-locked Ti:sapphire laser frequency comb that is stabilized using quantum interference of photocurrents in a semiconductor. Using this technique, we demonstrate carrier-envelope offset frequency fluctuations of less than 5 mHz using a 1 s gate time. With the resulting stable frequency comb, we measure the optical frequency of the iodine transition [(127)I2 R(127) 11-5 i component] to be 473 612 214 712.

Impulsive stimulated Raman scattering: comparison between phase-sensitive and spectrally filtered techniques.

Impulsive stimulated Raman scattering is used to generate and control coherent phonons and other low-frequency modes. In transparent materials, pump-probe experiments are usually performed by spectrally resolving the probe beam and measuring the spectral shift as a function of pump-probe time delay. By measuring the optical phase of the probe pulse as a function of time delay, we find that the phonon signal can be increased by a factor alpha(omegadelta)(-1), where omega is the phonon frequency and delta is the pulse duration.