Characterization of Pt-coated twin paraboloidal laboratory capillary high energy X-ray optics.

Novel focusing optics composed of twin paraboloidal capillaries coated with Pt, for laboratory X-ray sources are presented and characterized. The optics are designed to focus the X-rays, resulting in an achromatic focused beam with photon energies up to 40 keV. The performance of the optics under different operational conditions is studied by comparing the energy-photon count spectra of the direct and focused beams.

Single-shot, omni-directional x-ray scattering imaging with a laboratory source and single-photon localization.

Omni-directional, ultra-small-angle x-ray scattering imaging provides a method to measure the orientation of micro-structures without having to resolve them. In this letter, we use single-photon localization with the Timepix3 chip to demonstrate, to the best of our knowledge, the first laboratory-based implementation of single-shot, omni-directional x-ray scattering imaging using the beam-tracking technique. The setup allows a fast and accurate retrieval of the scattering signal using a simple absorption mask.

Evolution of intermetallic GaPd/SiO catalyst and optimization for methanol synthesis at ambient pressure.

The CO hydrogenation to methanol is efficiently catalyzed at ambient pressure by nanodispersed intermetallic GaPd/SiO catalysts prepared by incipient wetness impregnation. Here we optimize the catalyst in terms of metal content and reduction temperature in relation to its catalytic activity. We find that the intrinsic activity is higher for the GaPd/SiO catalyst with a metal loading of 13 wt.

Subpixel resolution in CdTe Timepix3 pixel detectors.

Timepix3 (256 × 256 pixels with a pitch of 55 µm) is a hybrid-pixel-detector readout chip that implements a data-driven architecture and is capable of simultaneous time-of-arrival (ToA) and energy (ToT: time-over-threshold) measurements. The ToA information allows the unambiguous identification of pixel clusters belonging to the same X-ray interaction, which allows for full one-by-one detection of photons. The weighted mean of the pixel clusters can be used to measure the subpixel position of an X-ray interaction.

Novel micro-reactor flow cell for investigation of model catalysts using in situ grazing-incidence X-ray scattering.

The design, fabrication and performance of a novel and highly sensitive micro-reactor device for performing in situ grazing-incidence X-ray scattering experiments of model catalyst systems is presented. The design of the reaction chamber, etched in silicon on insulator (SIO), permits grazing-incidence small-angle X-ray scattering (GISAXS) in transmission through 10 µm-thick entrance and exit windows by using micro-focused beams. An additional thinning of the Pyrex glass reactor lid allows simultaneous acquisition of the grazing-incidence wide-angle X-ray scattering (GIWAXS).