We utilize cavity-enhanced extinction spectroscopy to directly quantify the optical absorption of defects in MoS generated by helium ion bombardment. We achieve hyperspectral imaging of specific defect patterns with a detection limit below 0.01% extinction, corresponding to a detectable defect density below 1 × 10 cm.
View Article and Find Full Text PDFOwing to its low excitation energy and long radiative lifetime, the first excited isomeric state of thorium-229, Th, can be optically controlled by a laser and is an ideal candidate for the creation of a nuclear optical clock, which is expected to complement and outperform current electronic-shell-based atomic clocks. A nuclear clock will have various applications-such as in relativistic geodesy, dark matter research and the observation of potential temporal variations of fundamental constants-but its development has so far been impeded by the imprecise knowledge of the energy of Th. Here we report a direct measurement of the transition energy of this isomeric state to the ground state with an uncertainty of 0.
View Article and Find Full Text PDFA methodology is described to generate an isotopically pure Th ion beam in the 2+ and 3+ charge states. This ion beam enables one to investigate the low-lying isomeric first excited state of Th at an excitation energy of about 7.8(5) eV and a radiative lifetime of up to 10 seconds.
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