Tunable in situ near-UV pulses by transient plasmonic resonance in nanocomposites.

We propose a concept for generation of ultrashort pulses based on transient field-induced plasmonic resonance in nanoparticle composites. Photoionization and free-carrier plasma generation change the susceptibility of nanoparticles on a few-femtosecond scale under the action of the pump pulse. This opens a narrow time window when the system is in plasmonic resonance, which is accompanied by a short burst of the local field.

Photonic molecule state transition by collision.

We investigate the impact of collisions with two-frequency photonic molecules aiming to observe internal dynamic behavior and challenge their strong robustness. Versatile interaction scenarios show intriguing state changes expressed through modifications of the resulting state such as temporal compression and unknown collision-induced spectral tunneling. These processes show potential for efficient coherent supercontinuum generation and all-optical manipulation.

Third and fifth order nonlinear susceptibilities in thin HfO layers.

Third harmonic generation (THG) from dielectric layers is investigated. By forming a thin gradient of HfO with continuously increasing thickness, we are able to study this process in detail. This technique allows us to elucidate the influence of the substrate and to quantify the layered materials third χ(3ω: ω, ω, ω) and even fifth order χ(3ω: ω, ω, ω, ω, - ω) nonlinear susceptibility at the fundamental wavelength of 1030 nm.

Direct time-resolved plasma characterization with broadband terahertz light pulses.

We report here the results of comprehensive plasma characterization and diagnostics by analyzing time-resolved absorption spectra of short ultrabroadband (0.1-50 THz) pulses propagated through the test plasma. Spectral analysis of plasma-induced absorption of such THz pulses provides very direct, in situ, high dynamical range, potentially single-shot access to the plasma density, plasma decay time, electron temperature, and ballistic dynamics of the plasma expansion.

Onset of Bloch oscillations in the almost-strong-field regime.

In the field of high-order harmonic generation from solids, the electron motion typically exceeds the edge of the first Brillouin zone. In conventional nonlinear optics, on the other hand, the excursion of band electrons is negligible. Here, we investigate the transition from conventional nonlinear optics to the regime where the crystal electrons begin to explore the first Brillouin zone.

Self-Stopping of Light.

Here, we show that light can bring itself to a complete standstill (self-stop) via self-interaction mediated by the resonant nonlinearity in a fully homogeneous medium. An intense few-cycle pulse, entering the medium, may reshape to form a strongly coupled light-matter bundle, in which the energy is transferred from light to the medium and back periodically on the single-cycle scale. Such oscillating structure can decelerate, alter its propagation direction, and even completely stop, depending on the state of its internal degrees of freedom.

Role of frequency dependence of the nonlinearity on a soliton's evolution in photonic crystal fibers.

We reveal the crucial role played by the frequency dependence of the nonlinear parameter on the evolution of femtosecond solitons inside photonic crystal fibers (PCFs). We show that the conventional approach based on the self-steepening effect is not appropriate when such fibers have two zero-dispersion wavelengths, and several higher-order nonlinear terms must be included for realistic modeling of the nonlinear phenomena in PCFs. These terms affect not only the Raman-induced wavelength shift of a soliton but also impact its shedding of dispersive radiation.

Single-cycle pulse compression in dense resonant media.

We propose here a new approach for compression and frequency up-conversion of short optical pulses in the regime of extreme nonlinear optics in optically dense absorbing media, providing an alternative route to attosecond-scale pulses at high frequencies. This method is based on dynamics of self-induced transparency (SIT) pulses of nearly single cycle duration, leading to single-cycle-scale Rabi oscillations in the medium. The sub-cycle components of an incident pulse behave as separate SIT-pulses, approaching each other and self-compressing, resulting in the threefold compression in time and frequency up-conversion by the same factor.

Stable coherent mode-locking based on [Formula: see text] pulse formation in single-section lasers.

Here we consider coherent mode-locking (CML) regimes in single-section cavity lasers, taking place for pulse durations less than atomic population and phase relaxation times, which arise due to coherent Rabi oscillations of the atomic inversion. Typically, CML is introduced for lasers with two sections, the gain and absorber ones. Here we show that, for certain combination of the cavity length and relaxation parameters, a very stable CML in a laser, containing only gain section, may arise.

Higher-order dispersion and the spectral behavior in a doubly resonant optical parametric oscillator.

In doubly resonant optical parametric oscillators (DROPOs), it is possible to generate, enhance, and phase lock two frequencies at once. Following intracavity phase conditions, a complex tuning behavior of the signal and idler spectra takes place in DROPOs, cumulating into degeneracy with phase self-locking and coherent wavelength doubling. In this work, we identify group delay matching as the important parameter determining the global tuning behavior and demonstrate the key role of higher-order dispersion in the spectral dependencies.

Selective ultrafast control of multi-level quantum systems by subcycle and unipolar pulses.

The most typical way to optically control population of atomic and molecular systems is to illuminate them with radiation, resonant to the relevant transitions. Here we consider a possibility to control populations with the subcycle and even unipolar pulses, containing less than one oscillation of electric field. Despite the spectrum of such pulses covers several levels at once, we show that it is possible to selectively excite the levels of our choice by varying the driving pulse shape, duration or time delay between consecutive pulses.

Soliton Molecules with Two Frequencies.

We demonstrate a peculiar mechanism for the formation of bound states of light pulses of substantially different optical frequencies, in which pulses are strongly bound across a vast frequency gap. This is enabled by a propagation constant with two separate regions of anomalous dispersion. The resulting soliton compound exhibits moleculelike binding energy, vibration, and radiation and can be understood as a mutual trapping providing a striking analogy to quantum mechanics.

Generating Ultrabroadband Deep-UV Radiation and Sub-10 nm Gap by Hybrid-Morphology Gold Antennas.

We experimentally investigate the interaction between hybrid-morphology gold optical antennas and a few-cycle Ti:sapphire laser up to ablative intensities, demonstrating rich nonlinear plasmonic effects and promising applications in coherent frequency upconversion and nanofabrication technology. The two-dimensional array of hybrid antennas consists of elliptical apertures combined with bowties in its minor axis. The plasmonic resonance frequency of the bowties is red-shifted with respect to the laser central frequency and thus mainly enhances the third harmonic spectrum at long wavelengths.

Regularizing Aperiodic Cycles of Resonant Radiation in Filament Light Bullets.

We demonstrate an up to now unrecognized and very effective mechanism which prevents filament collapse and allows persistent self-guiding propagation retaining a large portion of the optical energy on axis over unexpected long distances. The key ingredient is the possibility of continuously leaking energy into the normal dispersion regime via the emission of resonant radiation. The frequency of the radiation is determined by the dispersion dynamically modified by photogenerated plasma, thus allowing us to excite new frequencies in spectral ranges which are otherwise difficult to access.

Simple route toward efficient frequency conversion for generation of fully coherent supercontinua in the mid-IR and UV range.

Fiber supercontinua represent light sources of pivotal importance for a wide range of applications, ranging from optical communications to frequency metrology. Although spectra encompassing more than three octaves can be produced, the applicability of such spectra is strongly hampered due to coherence degradation during spectral broadening. Assuming pulse parameters at the cutting edge of currently available laser technology, we demonstrate the possibility of strongly coherent supercontinuum generation.

Controlling formation and suppression of fiber-optical rogue waves.

Fiber-optical rogue waves appear as rare but extreme events during optical supercontinuum generation in photonic crystal fibers. This process is typically initiated by the decay of a high-order fundamental soliton into fundamental solitons. Collisions between these solitons as well as with dispersive radiation affect the soliton trajectory in frequency and time upon further propagation.

3D numerical simulations of THz generation by two-color laser filaments.

Terahertz (THz) radiation produced by the filamentation of two-color pulses over long distances in argon is numerically investigated using a comprehensive model in full space-time-resolved geometry. We show that the dominant physical mechanism for THz generation in the filamentation regime at clamping intensity is based on quasi-dc plasma currents. The calculated THz spectra for different pump pulse energies and pulse durations are in agreement with previously reported experimental observations.

Accelerated rogue waves generated by soliton fusion at the advanced stage of supercontinuum formation in photonic-crystal fibers.

Soliton fusion is a fascinating and delicate phenomenon that manifests itself in optical fibers in case of interaction between copropagating solitons with small temporal and wavelength separation. We show that the mechanism of acceleration of a trailing soliton by dispersive waves radiated from the preceding one provides necessary conditions for soliton fusion at the advanced stage of supercontinuum generation in photonic-crystal fibers. As a result of fusion, large-intensity robust light structures arise and propagate over significant distances.

High-power fifth-harmonic generation of femtosecond pulses in the vacuum ultraviolet using a Ti:sapphire laser.

We demonstrate the generation of fifth-harmonic pulses at 161 nm, with an energy of up to 600 nJ and 160 fs pulse duration from a Ti:sapphire laser at 1 kHz repetition rate by four-wave difference-frequency mixing in argon-filled waveguides. The efficiency is greatly improved by coupling to higher-order transverse modes, as well as by coating the inner surface of the waveguide. A numerical model of the process yields an understanding of the main effects influencing the harmonic generation.