Spectro-temporal behavior of dye-based solid-state random lasers under a picosecond pumping regime: Part III.

In two recent works, the authors have investigated the spectro-temporal properties of the random laser emission from solid state dye-doped powders in picosecond pumping regime. Each emission pulse consists, both above and below threshold, in a collection of narrow peaks of a spectro-temporal width at the theoretical limit (ΔωΔt≅1). The distribution of path lengths traveled inside the diffusive active medium by photons that can be amplified by stimulated emission explains this behavior, as demonstrated by a simple theoretical model developed by the authors.

Spectro-temporal behavior of dye-based solid-state random lasers under picosecond pumping regime: part II.

In a very recent work the spectral and temporal properties of the random laser emission from solid state dye-doped powders have been investigated by the authors in picosecond pumping regime. The emission shows within each pulse, peaks of more intensity than background, and of a spectro-temporal width at the theoretical limit (ΔωΔt≅1), even in conditions well below the threshold. The relationship between the distribution of paths lengths traveled by photons inside the active medium, and the amplification by stimulated emission explains this behavior.

Spectro-temporal behavior of dye-based solid-state random lasers under picosecond pumping regime.

In this work, the spectral and temporal properties of the random laser emission from dye-doped solid state powders are investigated in picosecond pumping regime. Ultrafast time-resolved spectroscopy achieved with a streak-camera has been used to perform a detailed study of the temporal evolution of the spectrum of their single pulses. Under conditions of low population inversion density, it is observed that the detected radiation occurs as isolated peaks with a very narrow spectro-temporally spread (ΔωΔt≅1).

Input/output energy in solid state dye random lasers.

A new approach to the problem of energy in solid state dye random lasers is presented. The measurements performed in terms of absolute energy show that the slope efficiency depends on the measurement conditions. In particular, in lasers with pumping in the picoseconds range, the result is really different if measured by recording the emission in the same time range or in a longer one (nanoseconds range).

Random laser model for Nd-doped powders and its application to stimulated emission cross-section calculations.

A new theoretical approach for random lasing of Nddoped powders is presented. The model's singularity lies in the fact that it proposes a probability distribution of the stimulated photon paths lengths in the sample, as well as a population inversion shared by different photon paths. The model's predictions satisfactorily compare with the results of laser threshold and absolute input/output energy slope of a real Random Laser.