J Phys Chem Lett
January 2024
The human brain efficiently processes only a fraction of visual information, a phenomenon termed attentional control, resulting in energy savings and heightened adaptability. Translating this mechanism into artificial visual neurons holds promise for constructing energy-efficient, bioinspired visual systems. Here, we propose a self-rectifying artificial visual neuron (SEVN) based on a NiO/GaO bipolar heterojunction with attentional control on patterns with a target color.
View Article and Find Full Text PDFThe cone photoreceptors in our eyes selectively transduce the natural light into spiking representations, which endows the brain with high energy-efficiency color vision. However, the cone-like device with color-selectivity and spike-encoding capability remains challenging. Here, we propose a metal oxide-based vertically integrated spiking cone photoreceptor array, which can directly transduce persistent lights into spike trains at a certain rate according to the input wavelengths.
View Article and Find Full Text PDFThe biological visual system encodes optical information into spikes and processes them by the neural network, which enables the perception with high throughput of visual processing with ultralow energy budget. This has inspired a wide spectrum of devices to imitate such neural process, while precise mimicking such procedure is still highly required. Here, a highly bio-realistic photoelectric spiking neuron for visual depth perception is presented.
View Article and Find Full Text PDFEmerging memory devices, that can provide programmable information recording with tunable resistive switching under external stimuli, hold great potential for applications in data storage, logic circuits, and artificial synapses. Realization of multifunctional manipulation within individual memory devices is particularly important in the More-than-Moore era, yet remains a challenge. Here, both rewritable and nonerasable memory are demonstrated in a single stimuli-responsive polymer diode, based on a nanohole-nanowrinkle bi-interfacial structure.
View Article and Find Full Text PDFCarbon dots (C-dots) are promising and widely applied carbon fluorescent materials for next-generation white light-emitting diodes (WLEDs). However, nonnegligible thermal quenching issues induced by high working temperature of high-power WLEDs severely limit the further development of C-dot phosphors. In this paper, we report an efficient strategy to improve thermal dissipation within C-dot phosphors to solve the thermal quenching problem.
View Article and Find Full Text PDFWe report the design and preparation of hierarchical hollow-pore nanostructure bilayer conjugated polymer films for high-performance resistive memory devices. By taking the merits of chemical and structural stabilities of a two-dimensional conjugated microporous polymer (2D CMP), a poly[2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] (MEH-PPV) film with a hollow surface was spin-coated onto 2D CMP nanofilm directly, constructing a bilayer heterojunction. A two-terminal diode with a configuration of indium tin oxide/2D CMP/hollow MEH-PPV/Al was fabricated by employing the prepared bilayer heterojunction.
View Article and Find Full Text PDFMXenes, an emerging class of two-dimensional (2D) transition-metal carbide materials, have received increasing attention for their interesting physiochemical properties. For not only MXenes but also other 2D materials, delamination is a requisite step for the exploitation of their unique properties. In this work, a facile method for exfoliating TiCT MXene to nanosheets of small size with the aid of poly(vinylpyrrolidone) (PVP) is designed, which has never been reported to our knowledge.
View Article and Find Full Text PDFMulticolor carbon phosphors as emerging light conversion materials, with full recyclability and stable color convertibility, are poised to accelerate the sustainable development of environment-friendly optoelectronics. Herein, we firstly report a facile strategy, combining single-step hydrothermal and differential washing methods, for the preparation of multicolor carbon emitters with nano-dot/micro-belt structures. The as-prepared hybrids exhibit excellent film-forming ability and demonstrate controllable multicolor solid-state luminescence ranging from white and green to blue light emission, by utilizing the synergistic effect between nano-dot and micro-belt structures.
View Article and Find Full Text PDFBuilding stretchable memory is an effective strategy for developing next-generation memory technologies toward stretchable and wearable electronics. Here we demonstrate a universal strategy for the fabrication of high performance stretchable polymer memory via tailoring surface morphology, in which common conjugated polymers and sharp reduced graphene oxide (r-rGO) films are used as active memristive layers and conductive electrodes, respectively. The fabricated devices feature write-once-read-many-times (WORM) memory, with a low switching voltage of 1.
View Article and Find Full Text PDFTwo-dimensional carbon semiconductors have aroused great attention due to their unique structures and novel properties, showing potential applications in emerging electronic and optoelectronic devices. In this work, we reported an effective strategy to controllable prepare ultrathin carbon nanofilms (CNFs) by combining -growth and stepwise thermal annealing, with the features of large-area, tunable properties and nanoscale thickness. The structures, morphologies and electrical properties of these as-prepared CNFs were characterized systematically.
View Article and Find Full Text PDFBuilding transient and flexible memristors is a promising strategy for developing emerging memory technologies. Here, a transient and flexible memristor based on a polymer nanocomposite, with a configuration of silver nanowire (AgNW)/citric acid quantum dot (CA QD)-polyvinyl pyrrolidone (PVP)/AgNW, is fabricated using a full-solution process method. The obtained device exhibits reversible resistive switching behavior and a dynamic random access memory (DRAM) storage feature, with the significant merits of a high ON/OFF ratio, low switching voltage, excellent reproducibility and desirable high flexibility, indicating outstanding memory characteristics such as low misreading, low power operation and low cost potential.
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