Water energy-converting techniques that focus on interfacial charge separation and transfer have aroused significant attention. However, the water-repelling nature leads to a less dense liquid layer and a sharp gradient of liquid velocity, which limits its output performance. Here, a water sliding generator (WSG) based on a smooth liquid-like/semiconductor surface (SLSS) is developed that harnesses the full advantage of liquid sliding friction.
View Article and Find Full Text PDFPolymer synthesis via multicomponent reactions (MCRs) has opened avenues in polymer chemistry and led to the development of various types of functional polymers. Herein, we developed a strategy to prepare multifunctional polymers via the successive modification of dihydropyrimidin-2(1)-thione (DHPMT), which can be generated by the tricomponent Biginelli reaction. Four hydrophobic polymers were efficiently prepared by using DHPMT derivatives.
View Article and Find Full Text PDFSmart superwetting membranes with finely tunable properties have attracted increased attention recently. However, they mostly focus on controllable wettability rather than controllable permeability. Also, the oil/water separation performance is usually tested with laboratory-simulated samples, making it hard for the materials to meet practical applications.
View Article and Find Full Text PDFSolar-driven interfacial evaporation is a potential water purification solution. Here, a novel regenerable hydrogel interfacial evaporator is designed with tunable water production. Such an evaporator is fabricated by readily mixing hydroxypropyl chitosan (HPCS) and dibenzaldehyde-functional poly(ethylene glycol) (DF-PEG) at ambient conditions.
View Article and Find Full Text PDFEngineering anti-adhesion coatings always focuses on a specific hierarchy and surface free energy, which passively endures water scouring to wash away the loosely attached foulants. Certain foulants, however, especially those that are highly adhesive or covalently attached on the coatings, cannot be removed off the designed surfaces easily. Inspired by the active self-hunting behavior of the filter-feeding animal Daphnia, herein, we propose a universal antifouling strategy with both passive and active adhesion repellency capabilities.
View Article and Find Full Text PDFShortage of freshwater and deterioration of the marine environment have a serious effect on the human body and ecological environment. Here, we demonstrated a facile way to prepare a multiple-target superwetting porous material to obtain available water without cumbersome steps. Through the facile immersion and hydrothermal method, a charge-enhanced membrane material combining superwettability, electrostatic interaction, and the steric effect is prepared.
View Article and Find Full Text PDFSuperwetting porous membranes with tunable liquid repellency are highly desirable in broad domains including scientific research, chemical industry, and environmental protection. Such membranes should allow for controllable droplet bouncing or spreading, which is difficult to achieve for low surface energy organic liquids (OLs). Here we develop an interfacial physical parameter to regulate the OL wettability of nanoparticle-embedded membranes by structuring synergistic layers with reconfigurable surface energy components.
View Article and Find Full Text PDFSuperwetting membranes with responsive properties have attracted heightened attention because of their fine-tunable surface wettability. However, their functional diversity is severely limited by the "black-or-white" wettability transition. Herein, we describe a coating strategy to fabricate multifunctional responsive superwetting membranes with SiO /octadecylamine patterns.
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