Publications by authors named "Hongling Dai"

Kitchen waste was mainly composed of carbohydrates, lipids, and proteins. Anaerobic digestion (AD) of kitchen waste usually occurred acidification and further deteriorated. In our previous study, alkali pretreatment combined with bentonite (AP/Be) treatment was proved to enhance high solid AD of kitchen waste.

View Article and Find Full Text PDF

In this study, Se@NC-x decorated with Se was successfully prepared via two-step calcination with zeolitic imidazole framework (ZIF) as a precursor. Mechanistic studies show that PMS would be adsorbed onto the surface of Se@NC-900 to form an active complex (Se@NC-900/PMS*), and the active Se@NC-900/PMS* could oxidize phenol by the rapid decomposition of PMS. Specifically, electrons are extracted by Se@NC-900/PMS* and then transferred to the surface of Se@NC-900, which can trigger the degradation of phenol.

View Article and Find Full Text PDF

Mitogen-activated extracellular signal-regulated kinase 1 and 2 (MEK1/2) are the critical components of the mitogen-activated protein kinase/extracellular signal-regulated kinase 1 and 2 (MAPK/ERK1/2) signaling pathway which is one of the well-characterized kinase cascades regulating cell proliferation, differentiation, growth, metabolism, survival and mobility both in normal and cancer cells. The aberrant activation of MAPK/ERK1/2 pathway is a hallmark of numerous human cancers, therefore targeting the components of this pathway to inhibit its dysregulation is a promising strategy for cancer treatment. Enormous efforts have been done in the development of MEK1/2 inhibitors and encouraging advancements have been made, including four inhibitors approved for clinical use.

View Article and Find Full Text PDF

Carbon-based catalysts have the advantages of biological cleaning, eco-friendly and cost-effective in water treatment. While, nitrogen doped biochar promotes the development of non-radical peroxymonosulfate (PMS) activation in environmental remediation. Thus, three-dimensional sponge-like porous Fe and N co-doped biochar (Fe/CN-30) with high catalytic activity for PMS activation was synthesized.

View Article and Find Full Text PDF

In this study, nano-sized CoFeO composites were prepared through co-precipitation process. Then the phosphorus-doped strong magnetic graphitic carbon nitride hybrids composites (P-CoFeO@GCN) was stemmed from the CoFeO composites via the thermal polymerization method. The TEM results show that the CoFeO nanoparticles have been successfully embedded into the graphitic carbon nitride (GCN).

View Article and Find Full Text PDF
Article Synopsis
  • A novel core-shell catalyst (Fe@POCN/CQDs) was synthesized for effectively degrading tetracycline, showing photocatalytic activity about 4.76 times greater than GCN.
  • The enhanced performance is attributed to the effective heterojunction and synergistic effects between POCN, Fe, and CQDs, which help reduce electron-hole recombination while generating more free radicals for oxidation.
  • The optimal removal of tetracycline reached 97.57% in 30 minutes under specific conditions, with reactive oxygen species playing crucial roles in the degradation process.
View Article and Find Full Text PDF

In this work, hierarchical structure TiO/hemp stem biochar carbon (HSBC) and CN-TiO/HSBC were successfully fabricated, which were used as efficient visible-light photocatalyst degradation for ammonia nitrogen from aqueous solution. The as-prepared CN-TiO/HSBC hybrid catalyst showed the higher efficient photocatalytic activity for decomposition of ammonia nitrogen than those of pure TiO and TiO/HSBC, suggesting suppressed recombination of photogenerated charges and promoted mass transfer due to synergistic effect, and thus increased photocatalytic degradation activity. The degradation of ammonia follows a pseudo-first-order kinetics.

View Article and Find Full Text PDF

Hierarchical Cu-AlO/biomass-activated carbon composites were successfully prepared by entrapping a biomass-activated carbon powder derived from green algae in the Cu-AlO frame (H-Cu-Al/BC) for the removal of ammonium nitrogen (NH -N) from aqueous solutions. The as-synthesized samples were characterized XRD, SEM, BET and FTIR spectroscopy. The BET specific surface area of the synthesized H-Cu-Al/BC increased from 175.

View Article and Find Full Text PDF

In this work, a series of flower-like CuAl layered double hydroxides (LDHs) and hierarchical CuAl/carbon fiber-LDH (CuAl/CF-LDH) materials were synthesized, and these materials were used as catalysts for the degradation of ammonia nitrogen from simulated wastewater. The morphologies and structures of the materials were characterized using scanning electron microscopy (SEM), Fourier transform infrared (FTIR) spectroscopy, Raman spectroscopy (RS), X-ray diffraction (XRD), and the Brunauer-Emmett-Teller (BET) technique. The effects of the catalyst and HO loading dosages, reaction temperature, pH, Cu/Al ratio of the samples, and contact time on the degradation process were investigated by degrading ammonia nitrogen under different conditions, and the possible degradation mechanism was discussed.

View Article and Find Full Text PDF

The coagulant dosage of an existing water plant is mainly determined based on the experience of water treatment process and influent/effluent water quality indexes that have time hysteresis effects. To solve this problem, the effect of coagulant dosage on a number of parameters used to evaluate the efficiency of flocculation in a setup was determined by using the micro-vortex flocculation technology in conjunction with the investigation of the relation between the equivalent diameter and the fractal dimension. By means of the machine vision system and computerized analysis, the effects of floc quantity, floc equivalent diameter and fractal dimension can be assessed.

View Article and Find Full Text PDF

Amine-functionalized magnetic bamboo-based activated carbon (AFM-BAC) derived from bamboo products wastes were employed for effective adsorption of fluoroquinolone antibiotics ciprofloxacin (CIP) and norfloxacin (NOR) through batch processing. The effects of factors on the adsorption of both antibiotics were studied. The studies of various factors influencing the adsorption behavior indicated that the maximum adsorption capacities for two antibiotics adsorption were observed in weakly acidic condition and the adsorption amounts of two antibiotics increased with the increase of zwitterionic form, implying the importance of zwitterionic form, and the adsorption process is spontaneous and endothermic.

View Article and Find Full Text PDF

The performances of ordered mesoporous carbon CMK-3 (OMC), bamboo-based carbon (BC), and these two kinds of adsorbents modified by thermal treatment in the ammonia atmosphere at high temperatures were evaluated for the removal fluoroquinolone antibiotic (ciprofloxacin) from aqueous solution. The adsorption behavior of ciprofloxacin (CIP) onto OMC and BC including adsorption isotherms and kinetics were investigated. The effect of various factors (pH, ionic strength and temperature) on the adsorption process was also investigated.

View Article and Find Full Text PDF