Publications by authors named "Hongjun Han"

The combination of intermittently weak ultrasound and sequencing batch reactor was thoroughly investigated to elucidate the relationship between enhanced contaminants removal and activated sludge characteristics, microbial composition, and regulation of differentially expressed genes (DEGs). At 12 °C, irradiation with an ultrasound intensity of 9.68 W/L, an irradiation time of 10 min, and an interval time of 24 h led to significant increases in COD, NH-N, and TP removals with the rates of 93.

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Effectively treating phenolic substances is a crucial task in environmental protection. This study aims to determine whether bacterial-algae biofilm reactors offer superior treatment efficacy compared to traditional activated sludge and biofilm reactors. The average degradation ratios of 2,4-dimethylphenol (40, 70, 150, 300, and 230 mg/L) were found to be 98 %, 99 %, 92.

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The Escherichia coli (E.coli) degrading glucose irradiated by ultrasound irradiation (20 W, 14 min) was investigated as the model system, the glucose degradation increased by 13 % while the E.coli proliferation decreased by 10 % after culture for 18 h.

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It is particularly important to comprehensively assess the biotoxicity variation of industrial wastewater along the treatment process for ensuring the water environment security. However, intensive studies on the biotoxicity reduction of industrial wastewater are still limited. In this study, the toxic organics removal and biotoxicity reduction of coal chemical wastewater (CCW) along a novel full-scale treatment process based on the pretreatment process-anaerobic process-biological enhanced (BE) process-anoxic/oxic (A/O) process-advanced treatment process was evaluated.

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Industrial waste as novel conductive mediator was applied for wastewater treatment as a novel strategy for both waste recycling and sustainable development of wastewater treatment. In this study, nanoscale zero valent iron-loaded fly ash-based activated carbon (nZVI@FABAC) was prepared and applied to enhancing activated sludge (AS) process for coal chemical wastewater (CCW) treatment. The results demonstrated that the removal efficiencies of COD and total phenols (TPh) in nZVI@FABAC/AS process reached about 83.

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Coal chemical wastewater (CCW) is a type of refractory industrial wastewater, and its treatment has become the main bottleneck restricting the sustainable development of novel coal chemical industry. Biological treatment is considered as an economical, effective and environmentally friendly technology for CCW treatment. However, conventional biological process is difficult to achieve the efficient removal of refractory organics because of CCW with the characteristics of composition complexity and high toxicity.

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Anaerobic digestion (AD) of waste activated sludge (WAS) is commonly limited to poor synergistic cooperation of four stages including hydrolysis, acidogenesis, acetogenesis and methanogenesis. Dissimilatory metal reduction that induced by metal-based conductive materials is promising strategy to regulate anaerobic metabolism with the higher metabolic driving force. In this study, MnO as inducer of dissimilatory manganese reduction (DMnR) was added into WAS-feeding AD system for mediating complicated anaerobic metabolism.

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To better promote environment friendly development of the coal chemical industry, this study investigated effects of methanol, sodium citrate, and chlorella powder (a type of microalgae) as co-metabolic substances on enhanced anaerobic treatment of coal pyrolysis wastewater with anaerobic sludge. The anaerobic sludge was loaded into four 2 L anaerobic reactors for co-metabolism enhanced anaerobic experiments. Anaerobic reactor 1 (R1) as control group did not add a co-metabolic substance; anaerobic reactor 2 (R2) added methanol; anaerobic reactor 3 (R3) added sodium citrate; and anaerobic reactor 4 (R4) added chlorella powder.

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Mainstream anaerobic wastewater treatment has received increasing attention for the recovery of methane-rich biogas from biodegradable organics, but subsequent mainstream nitrogen and dissolved methane removal at low temperatures remains a critical challenge in practical applications. In this study, granular sludge coupling n-DAMO with Anammox was employed for mainstream nitrogen removal, and the dissolved methane removal potential of granular sludge at low temperatures was investigated. A stable nitrogen removal rate (0.

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Article Synopsis
  • * Key microbial players like iron-oxidizing (Thiobacillus and Acidovorax) and iron-reducing bacteria (Geothrix and Ignavibacterium) were found to thrive under optimal conditions, aiding the iron cycling process crucial for denitrification efficiency.
  • * The research highlighted enhanced microbial electron transfer activities and enzyme gene abundance during den
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Article Synopsis
  • The study examined the use of a nano-FeO@activated coke enhanced bio-system (FEBS) to effectively treat aromatic organics in coal pyrolysis wastewater under low-oxygen conditions, achieving an average organic removal rate of 92.29%.
  • Metagenomic analysis revealed that the biodegradation processes relied on FeO redox reactions and microbial biofilms, with the main degradation pathways involving bacteria that preferentially cleaved the benzene ring using aerobic methods.
  • Key functional species identified, such as Comamonas, Azotobacter, Alicycliphilus, and Acidovorax, were crucial in breaking down both benzene and nitrogen-heterocyclic compounds through aerobic
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The coal pyrolysis wastewater (CPW) contributed to aquatic environment contamination with amount of aromatic pollutants, and the research on joint toxicity of the mixture of aromatic compounds was vital for environmental protection. By using Tetrahymena thermophile as non-target organism, the joint toxicity of typical nonpolar narcotics and polar narcotics in CPW was investigated. The results demonstrated that the nonpolar narcotics exerted chronic and reversible toxicity by hydrophobicity-based membrane perturbation, while polar narcotics performed acute toxicity by irreversible damage of cells.

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Combining nitrate/nitrite dependent anaerobic methane oxidation (n-DAMO) and anaerobic ammonium oxidation (Anammox) is a promising sustainable wastewater treatment technology, which simultaneously achieve nitrogen removal and methane emission mitigation. However, the practical application of n-DAMO has been greatly limited by its extremely slow growth-rate and low reaction rate. This work proposes an innovative Membrane BioTrickling Filter (MBTF), which consist of hollow fiber membrane for effective methane supplementation and polyurethane sponge as support media for the attachment and growth of biofilm coupling n-DAMO with Anammox.

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Partial nitritation-anammox (PNA) is a promising and energy-efficient process for the sustainable nitrogen removal. However, its wide applications are still limited by the long start-up period and instability of long-term operation. Quorum sensing (QS), as a way of cell-to-cell communication generally regulating various microbial behaviors, has been increasingly investigated in PNA process, because QS may substantially manipulate the metabolism of microorganisms and overcome the limitations of PNA process.

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The integration of nitrate/nitrite dependent anaerobic methane oxidation (n-DAMO) and anaerobic ammonium oxidation (Anammox) provides sustainable solution to simultaneously remove nitrate, nitrite and ammonium. This study demonstrated the sludge granulation process coupling n-DAMO and Anammox from mixed inoculum including river sediment, return activated sludge and crushed anaerobic granule sludge in a novel membrane granular sludge reactor (MGSR). Flocculent biomass gradually turned into compact aggregates and retained as granular sludge with an average diameter of 2.

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The application of Water-Sediment Regulation Project provides abundant freshwater for the Yellow River Delta, changes water and sediment condition, as well as brings lots of exogenous substances. Using orthogonal test with three factors and four levels, we examined the effects of water condition, sediment burial depth and exogenous nitrogen input on the growth of wetland plant, Suaeda salsa. The results showed that sediment burial had great effect on protein content and SOD activity.

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Denitrifying anaerobic methane oxidation (DAMO) coupled to anaerobic ammonium oxidation (anammox) is a promising technology for complete nitrogen removal with economic and environmental benefit. In this work, a model framework integrating DAMO and anammox process was constructed based on suspended-growth systems. The proposed model was calibrated and validated using experimental data from a sequencing batch reactor and a membrane aerated membrane bioreactor (MAMBR).

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To investigate the role of electroactive biofilms for enhanced phenolic degradation, lignite activated coke (LAC) and MAC were used as carriers in moving-bed biofilm reactor (MBBR) for CPW treatment. In contrast to activated sludge (AS) reactor, the carriers improved degradation performance of MBBR. Although two MBBRs exerted similar degradation capacity with over 92% of COD and 93% phenols removal under the highest phenolics concentration (500 mg/L), the effluent of MAC-based MBBR remained higher biodegradability (BOD/COD = 0.

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Powdered activated carbon (PAC), lignite activated coke (LAC) and Fe-C carriers were applied to enhance CBFBRs to degrade targeted phenolics. In start-up stage, PAC and LAC equipped CBFBRs with higher environment adaptability and phenolic degradation capacity for phenol (>96%), p-cresol (>91%) and 3, 5-dimethylphenol (>84%) in comparison to Fe-C carrier. In recovery stage, the superior performance was also identified for CBFBRs in basis of PAC and LAC than Fe-C-based reactor.

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Nitrate/nitrite-dependent anaerobic methane oxidation (n-DAMO) coupling to Anaerobic ammonium oxidation (Anammox) provides an opportunity for simultaneous nitrogen removal and methane emissions mitigation from wastewater. However, to achieve high nitrogen removal rate in such a process remains a critical challenge in practical application. This work investigated the interactions between n-DAMO and Anammox in membrane biofilm reactor (MBfR) and then developed operational strategies of MBfR for high rate nitrogen removal from landfill leachate.

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Article Synopsis
  • * Four different reactor setups were tested over 120 days, with R4 (biofilm + sodium citrate) showing the highest degradation rates of over 98% for quinoline and 95% for indole.
  • * Bacterial and archaea colony analysis revealed that anaerobic conditions in both sludge and biofilm reactors promote different pathways for methane production, highlighting their potential in treating nitrogen heterocyclic wastewater.
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Mixotrophic nitrate removal in wastewater from coal pyrolysis was achieved in microbial electrolysis cell with iron anode (iron-MEC). The effect of voltage, iron anode and conductivity were investigated. The effluent TN concentration was 8.

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A simultaneous nitrification and denitrification (SND) bioaugmention system with Pseudomonas sp. HJ3 inoculated was established to explore the potential of simultaneous phenol and nitrogen removal in coal gasification wastewater (CGW). When the concentration of influent chemical oxygen demand (COD) and total phenols (TPh) was 1,765.

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The purpose of the research was to explore the feasibility of anaerobic hydrolysis in the recycling of chemical wastewater. From the case study of utilization of coal pyrolysis wastewater (CPW), the concept of anaerobic hydrolysis to produce clean and stable energy was proposed. Compared with anaerobic methane production and hydrogen production, anaerobic hydrolysis was more suitable to realize the resource utilization of chemical wastewater.

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