Mid-infrared edge-enhanced imaging via angle-selective nonlinear filtering.

We propose a novel, to the best of our knowledge, scheme for mid-infrared upconversion imaging with high tunability between bright-field and edge-enhanced modalities. The involved engineering of the nonlinear process favors shaping the optical transfer function of the imaging system. Consequently, a nonlinear angle-selective filter can be configured to perform an all-optical Fourier processing of the image, which highly depends on phase-matching parameters.

NO precipitation and valorization driven by photocatalysis and adsorption over red soil.

Nitrogen oxides (NO) emissions can cause air pollution that is harmful to human health, even producing serious ecological problems. Whether it is diluted in the air or not, the management and valorization of NO from industrial emissions have been constrained by technology and finance. This study shows that red soil can be used as a photocatalyst to convert NO into soil nitrate nitrogen (NO-N) in the soil.

Wide-field mid-infrared hyperspectral imaging beyond video rate.

Mid-infrared hyperspectral imaging has become an indispensable tool to spatially resolve chemical information in a wide variety of samples. However, acquiring three-dimensional data cubes is typically time-consuming due to the limited speed of raster scanning or wavelength tuning, which impedes real-time visualization with high spatial definition across broad spectral bands. Here, we devise and implement a high-speed, wide-field mid-infrared hyperspectral imaging system relying on broadband parametric upconversion of high-brightness supercontinuum illumination at the Fourier plane.

Giant enhancement of fluorescence resonance energy transfer based on nanoporous gold with small amount of residual silver.

Fluorescence resonance energy transfer (FRET) was found strongly enhanced by plasmon resonance. In this work, Nanoporous Gold with small amount of residual silver was used to form nanoporous gold/organic molecular layer compound with PSS and PAH. The ratio of its specific gold and silver content is achieved by controlling the time of its dealloying.

Synchronization, Desynchronization, and Intermediate Regime of Breathing Solitons and Soliton Molecules in a Laser Cavity.

We report on the experimental and numerical observations of synchronization and desynchronization of bound states of multiple breathing solitons (breathing soliton molecules) in an ultrafast fiber laser. In the desynchronization regime, although the breather molecules as wholes are not synchronized to the cavity, the individual breathers within a molecule are synchronized to each other with a delay (lag synchronization). An intermediate regime between the synchronization and desynchronization phases is also observed, featuring self-modulation of the synchronized state.

Enhanced sequestration of CO from simulated electrolytic aluminum flue gas by modified red mud.

The aluminum industry is facing severe economic and environmental problems due to increasing carbon emissions and growing stockpiles of red mud (RM). RM is a strongly alkaline, high-emission solid waste from the alumina industry with potential for CO sequestration. However, the effectiveness of RM carbon sequestration is poor, and the mechanism behind it is not well understood.

Dual-comb optomechanical spectroscopy.

Optical cavities are essential for enhancing the sensitivity of molecular absorption spectroscopy, which finds widespread high-sensitivity gas sensing applications. However, the use of high-finesse cavities confines the wavelength range of operation and prevents broader applications. Here, we take a different approach to ultrasensitive molecular spectroscopy, namely dual-comb optomechanical spectroscopy (DCOS), by integrating the high-resolution multiplexing capabilities of dual-comb spectroscopy with cavity optomechanics through photoacoustic coupling.

Mid-infrared single-photon 3D imaging.

Active mid-infrared (MIR) imagers capable of retrieving three-dimensional (3D) structure and reflectivity information are highly attractive in a wide range of biomedical and industrial applications. However, infrared 3D imaging at low-light levels is still challenging due to the deficiency of sensitive and fast MIR sensors. Here we propose and implement a MIR time-of-flight imaging system that operates at single-photon sensitivity and femtosecond timing resolution.

Volume plasma grating by noncollinear interaction of femtosecond filament arrays.

Stable propagation of multifilament arrays in transparent bulk media with adjustable separation distances between adjacent child filaments has always been desired for advanced manufacturing. Here, we report on the generation of an ionization-induced volume plasma grating (VPG) by the interaction of two batches of noncollinearly propagating arrays of multiple filaments (AMF). The VPG can externally arrange the propagation of the pulses along regular plasma waveguides via spatial reconstruction of electrical fields, which is compared with the self-formation of randomly distributed multiple filamentation originated from noises.

Mid-infrared single-pixel imaging at the single-photon level.

Single-pixel cameras have recently emerged as promising alternatives to multi-pixel sensors due to reduced costs and superior durability, which are particularly attractive for mid-infrared (MIR) imaging pertinent to applications including industry inspection and biomedical diagnosis. To date, MIR single-pixel photon-sparse imaging has yet been realized, which urgently calls for high-sensitivity optical detectors and high-fidelity spatial modulators. Here, we demonstrate a MIR single-photon computational imaging with a single-element silicon detector.

Free-Running Single-Photon Detection via GHz Gated InGaAs/InP APD for High Time Resolution and Count Rate up to 500 Mcount/s.

Free-running InGaAs/InP single-photon avalanche photodiodes (SPADs) typically operate in the active-quenching mode, facing the problems of long dead time and large timing jitter. In this paper, we demonstrate a 1-GHz gated InGaAs/InP SPAD with the sinusoidal gating signals asynchronous to the incident pulsed laser, enabling free-running single-photon detection. The photon-induced avalanche signals are quenched within 1 ns, efficiently reducing the SPAD's dead time and achieving a count rate of up to 500 Mcount/s.

Terahertz Time-of-Flight Ranging with Adaptive Clock Asynchronous Optical Sampling.

We propose and implement a terahertz time-of-flight ranging system based on adaptive clock asynchronous optical sampling, where the timing jitter is corrected in real time to recover the depth information in the acquired interferograms after compensating for laser instabilities using electronic signal processing. Consequently, the involved measurement uncertainties caused by the timing jitter during the terahertz sampling process and the noise intensity of the terahertz electric field have been reduced by the utilization of the adaptive clock. The achieved uncertainty range is about 2.

Silicon Nanowire-Assisted High Uniform Arrayed Waveguide Grating.

Determining how to improve the non-uniformity of arrayed waveguide grating (AWG) is of great significance for dense wavelength division multiplexing (DWDM) systems. In this work, a silicon nanowire-assisted AWG structure is proposed, which can achieve high uniformity with a low insertion loss. The article compares the effect of nanowire number and shape on uniformity and insertion loss, finding that double nanowires provide the best performance.

Ultra-rapid dual-comb ranging with an extended non-ambiguity range.

In this Letter, we report a scheme that combines time-of-flight (ToF) ranging detection of multi-repetition-rate pulses with asymmetric dual-comb ranging (DCR) measurement. Notably, this combination extends the non-ambiguity range (NAR) of the DCR method without sacrificing its refresh rate and distance precision. With this scheme, we demonstrate absolute distance measurement of moving targets with an NAR of 1.

Farey tree and devil's staircase of frequency-locked breathers in ultrafast lasers.

Nonlinear systems with two competing frequencies show locking or resonances. In lasers, the two interacting frequencies can be the cavity repetition rate and a frequency externally applied to the system. Conversely, the excitation of breather oscillations in lasers naturally triggers a second characteristic frequency in the system, therefore showing competition between the cavity repetition rate and the breathing frequency.

Dual-comb quartz-enhanced photoacoustic spectroscopy.

Photoacoustic spectroscopy (PAS) using two optical combs is a new-born technique, offering appealing features, including broad optical bandwidths, high resolutions, fast acquisition speeds, and wavelength-independent photoacoustic detection, for chemical sensing. However, its further application to, e.g.

Optical Bistability in a Tunable Gourd-Shaped Silicon Ring Resonator.

In this study, a tunable gourd-shaped ring resonator is demonstrated to generate optical bistability. The system consists of two sub-rings for a gourd shape configuration with a U-shaped wave guiding pathway. The transfer matrix method and FDTD simulation are used to acquire the spectral characteristics of the system.

Special Issue: State-of-the-Art Nanophotonic and Optical Nanomaterials in China.

In recent years, the fields of nanophotonics and nano-optics have been greatly fueled by rapid advancements in photonic science and technology, especially by the emergence of novel optical nanomaterials and new functional nanostructures [...

Carbon-Assistant Nanoporous Gold for Surface-Enhanced Raman Scattering.

Surface-enhanced Raman scattering (SERS) technology can amplify the Raman signal due to excited localized surface plasmon (LSP) from SERS substrates, and the properties of the substrate play a decisive role for SERS sensing. Several methods have been developed to improve the performance of the substrate by surface modification. Here, we reported a surface modification method to construct carbon-coated nanoporous gold (C@NPG) SERS substrate.

Generation of broadband parabolic pulses based on a pre-chirper free, core-pumped nonlinear fiber amplifier for coherent anti-Stokes Raman imaging.

We report the generation of parabolic pulses with broadband spectrum from a core-pumped Yb-doped fiber amplifier seeded by a dispersion managed fiber oscillator. The net cavity dispersion of Yb-doped oscillator was continuously changed from 0.074 to -0.

High-speed photon-number-resolving detection via a GHz-gated SiPM.

Silicon photomultipliers (SiPMs) constitute a promising candidate for photon-number-resolving (PNR) detection via spatial multiplexing, which offer advantages like high integration and low cost. Up to date, there has been continuous endeavor in boosting the PNR performances, particularly on the resolved photon numbers and operation speed. Here, we demonstrate a GHz-gated SiPM in the Geiger mode, which allows to quench the photon-induced avalanche signal within 1 ns.

Hydrogenated Amorphous Titania with Engineered Surface Oxygen Vacancy for Efficient Formaldehyde and Dye Removals under Visible-Light Irradiation.

Hydrogenated crystalized TiO with oxygen vacant (O) doping has attracted considerable attraction, owing to its impressive photoactivity. However, amorphous TiO, as a common allotrope of titania, is ignored as a hydrogenated templet. In this work, hydrogenated amorphous TiO (HAm-TiO) with engineered surface O and high surface area (176.

Passive repetition-rate stabilization for a mode-locked fiber laser by electro-optic modulation.

We report a passive stabilization of the repetition rate for a mode-locked fiber laser by using an electro-optic modulator in a phase-biased nonlinear amplifying loop mirror. The underlying mechanism, in contrast to active feedback operations, lies in the cross-phase modulation between electrical and optical pulses within an electro-optic crystal. The resulting spectral shift can automatically compensate for the cavity-length drift via the group velocity dispersion.

Wide-field mid-infrared single-photon upconversion imaging.

Frequency upconversion technique, where the infrared signal is nonlinearly translated into the visible band to leverage the silicon sensors, offers a promising alternation for the mid-infrared (MIR) imaging. However, the intrinsic field of view (FOV) is typically limited by the phase-matching condition, thus imposing a remaining challenge to promote subsequent applications. Here, we demonstrate a wide-field upconversion imaging based on the aperiodic quasi-phase-matching configuration.