Momentum space separation of quantum path interferences between photons and surface plasmon polaritons in nonlinear photoemission microscopy.

Quantum path interferences occur whenever multiple equivalent and coherent transitions result in a common final state. Such interferences strongly modify the probability of a particle to be found in that final state, a key concept of quantum coherent control. When multiple nonlinear and energy-degenerate transitions occur in a system, the multitude of possible quantum path interferences is hard to disentangle experimentally.

Direct electron beam patterning of electro-optically active PEDOT:PSS.

The optical and electronic tunability of the conductive polymer poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) has enabled emerging applications as diverse as bioelectronics, flexible electronics, and micro- and nano-photonics. High-resolution spatial patterning of PEDOT:PSS opens up opportunities for novel active devices in a range of fields. However, typical lithographic processes require tedious indirect patterning and dry etch processes, while solution-processing methods such as ink-jet printing have limited spatial resolution.

Ultracompact wavefront characterization of femtosecond 3D printed microlenses using double-frequency Ronchi interferometry.

3D printed microoptics have become important tools for miniature endoscopy, novel CMOS-based on-chip sensors, OCT-fibers, among others. Until now, only image quality and spot diagrams were available for optical characterization. Here, we introduce Ronchi interferometry as ultracompact and quick quantitative analysis method for measuring the wavefront aberrations after propagating coherent light through the 3D printed miniature optics.

Limits of the detection of microplastics in fish tissue using stimulated Raman scattering microscopy.

We demonstrate the detection sensitivity of microplastic beads within fish tissue using stimulated Raman scattering (SRS) microscopy. The intrinsically provided chemical contrast distinguishes different types of plastic compounds within fish tissue. We study the size-dependent signal-to-noise ratio of the microplastic beads and determine a lower boundary for the detectable size.

Spectrally resolved ultrafast transient dynamics of a femtosecond fiber-feedback optical parametric oscillator.

We report on spectrotemporal transient dynamics in a femtosecond fiber-feedback optical parametric oscillator (FFOPO) system. Burst modulation of the pump beam in combination with dispersive Fourier transformation sampling allows to record single-pulse signal spectra at 41 MHz sampling rate. Therefore, each individual pulse of the signal transients can be spectrally resolved.

Ultrafast Time Dynamics of Plasmonic Fractional Orbital Angular Momentum.

The creation and manipulation of optical vortices, both in free space and in two-dimensional systems such as surface plasmon polaritons (SPPs), has attracted widespread attention in nano-optics due to their robust topological structure. Coupled with strong spatial confinement in the case of SPPs, these plasmonic vortices and their underlying orbital angular momentum (OAM) have promise in novel light-matter interactions on the nanoscale with applications ranging from on-chip particle manipulation to tailored control of plasmonic quasiparticles. Until now, predominantly integer OAM values have been investigated.

Hybrid fiber-solid-state laser with 3D-printed intracavity lenses.

Microscale 3D-printing has revolutionized micro-optical applications ranging from endoscopy, imaging, to quantum technologies. In all these applications, miniaturization is key, and in combination with the nearly unlimited design space, it is opening novel, to the best of our knowledge, avenues. Here, we push the limits of miniaturization and durability by realizing the first fiber laser system with intra-cavity on-fiber 3D-printed optics.

Micro- and nanofabrication of dynamic hydrogels with multichannel information.

Creating micro/nanostructures containing multi-channel information within responsive hydrogels presents exciting opportunities for dynamically changing functionalities. However, fabricating these structures is immensely challenging due to the soft and dynamic nature of hydrogels, often resulting in unintended structural deformations or destruction. Here, we demonstrate that dehydrated hydrogels, treated by a programmable femtosecond laser, can allow for a robust fabrication of micro/nanostructures.

Laser written mirror profiles for open-access fiber Fabry-Perot microcavities.

We demonstrate laser-written concave hemispherical structures produced on the endfacets of optical fibers that serve as mirror substrates for tunable open-access microcavities. We achieve finesse values of up to 200, and a mostly constant performance across the entire stability range. This enables cavity operation also close to the stability limit, where a peak quality factor of 1.

Spatially Resolved Nonlinear Plasmonics.

Nonlinear optical plasmonics investigates the emission of plasmonic nanoantennas with the aid of nonlinear spectroscopy. Here we introduce nonlinear spatially resolved spectroscopy (NSRS) which is capable of imaging the k-space as well as spatially resolving the THG signal of gold nanoantennas and investigating the emission of individual antennas by wide-field illumination of entire arrays. Hand in hand with theoretical simulations, we demonstrate our ability of imaging various oscillation modes inside the nanostructures and therefore spatial emission hotspots.

Stress-induced birefringence in 3D direct laser written micro-optics.

3D direct laser writing is a widely used technology to create different nano- and micro-optical devices for various purposes. However, one big issue is the shrinking of the structures during polymerization, which results in deviations from the design and in internal stress. While the deviations can be compensated by adapting the design, the internal stress remains and induces birefringence.

Electrically switchable metallic polymer metasurface device with gel polymer electrolyte.

We present an electrically switchable, compact metasurface device based on the metallic polymer PEDOT:PSS in combination with a gel polymer electrolyte. Applying square-wave voltages, we can reversibly switch the PEDOT:PSS from dielectric to metallic. Using this concept, we demonstrate a compact, standalone, and CMOS compatible metadevice.

3D stimulated Raman spectral imaging of water dynamics associated with pectin-glycocalyceal entanglement.

Pectin is a heteropolysaccharide responsible for the structural integrity of the cell walls of terrestrial plants. When applied to the surface of mammalian visceral organs, pectin films form a strong physical bond with the surface glycocalyx. A potential mechanism of pectin adhesion to the glycocalyx is the water-dependent entanglement of pectin polysaccharide chains with the glycocalyx.

Complex aspherical singlet and doublet microoptics by grayscale 3D printing.

We demonstrate 3D printed aspherical singlet and doublet microoptical components by grayscale lithography and characterize and evaluate their excellent shape accuracy and optical performance. The typical two-photon polymerization (2PP) 3D printing process creates steps in the structure which is undesired for optical surfaces. We utilize two-photon grayscale lithography (2GL) to create step-free lenses.

Dielectric Mie voids: confining light in air.

Manipulating light on the nanoscale has become a central challenge in metadevices, resonant surfaces, nanoscale optical sensors, and many more, and it is largely based on resonant light confinement in dispersive and lossy metals and dielectrics. Here, we experimentally implement a novel strategy for dielectric nanophotonics: Resonant subwavelength localized confinement of light in air. We demonstrate that voids created in high-index dielectric host materials support localized resonant modes with exceptional optical properties.

Adjustment-free two-sided 3D direct laser writing for aligned micro-optics on both substrate sides.

3D direct laser writing is a powerful and widely used tool to create complex micro-optics. The fabrication method offers two different writing modes. During the immersion mode, an immersion medium is applied between the objective and the substrate while the photoresist is exposed on its back side.

Electro-active metaobjective from metalenses-on-demand.

Switchable metasurfaces can actively control the functionality of integrated metadevices with high efficiency and on ultra-small length scales. Such metadevices include active lenses, dynamic diffractive optical elements, or switchable holograms. Especially, for applications in emerging technologies such as AR (augmented reality) and VR (virtual reality) devices, sophisticated metaoptics with unique functionalities are crucially important.

Coupling light emission of single-photon sources into single-mode fibers: mode matching, coupling efficiencies, and thermo-optical effects.

We discuss the coupling efficiency of single-photon sources into single-mode fibers using 3D printed micro-optical lens designs. Using the wave propagation method, we optimize lens systems for two different quantum light sources and assess the results in terms of maximum coupling efficiencies, misalignment effects, and thermo-optical influences. Thereby, we compare singlet lens designs with one lens printed onto the fiber with doublet lens designs with an additional lens printed onto the semiconductor substrate.

Numerical optimization of single-mode fiber-coupled single-photon sources based on semiconductor quantum dots.

We perform extended numerical studies to maximize the overall photon coupling efficiency of fiber-coupled quantum dot single-photon sources emitting in the near-infrared and O-band and C-band. Using the finite element method, we optimize the photon extraction and fiber-coupling efficiency of quantum dot single-photon sources based on micromesas, microlenses, circular Bragg grating cavities and micropillars. The numerical simulations which consider the entire system consisting of the quantum dot source itself, the coupling lens, and the single-mode fiber, yield overall photon coupling efficiencies of up to 83%.

Quantitative determination of the electric field strength in a plasmon focus from ponderomotive energy shifts.

Spectroscopic photoemission microscopy is used to detect and quantify a ponderomotive shift in the energy of electrons that are emitted from a surface plasmon polariton focus. The focus is formed on an atomically flat Au(111) surface by an Archimedean spiral and is spatiotemporally separated from the circularly polarized light pulse used to excite the spiral. A spectroscopic analysis of electrons emitted from the focus exhibits a peaked above-threshold electron emission spectrum.

Predicting Concentrations of Mixed Sugar Solutions with a Combination of Resonant Plasmon-Enhanced SEIRA and Principal Component Analysis.

The detection and quantification of glucose concentrations in human blood or in the ocular fluid gain importance due to the increasing number of diabetes patients. A reliable determination of these low concentrations is hindered by the complex aqueous environments in which various biomolecules are present. In this study, we push the detection limit as well as the discriminative power of plasmonic nanoantenna-based sensors towards the physiological limit.

Sub-40 fs optical parametric oscillator beyond the gain bandwidth limit.

We report a compact and passively stable optical parametric oscillator for direct generation of sub-40 fs pulses, five times shorter than the 200 fs pump oscillator. By employing an intracavity all normal dispersion feedback fiber, we achieved low-noise and coherent broadening beyond the parametric gain bandwidth limitation. We demonstrate spectral coverage from 1.

Predicting Laser-Induced Colors of Random Plasmonic Metasurfaces and Optimizing Image Multiplexing Using Deep Learning.

Structural colors of plasmonic metasurfaces have been promised to a strong technological impact thanks to their high brightness, durability, and dichroic properties. However, fabricating metasurfaces whose spatial distribution must be customized at each implementation and over large areas is still a challenge. Since the demonstration of printed image multiplexing on quasi-random plasmonic metasurfaces, laser processing appears as a promising technology to reach the right level of accuracy and versatility.

3D-Printed Micro Lens-in-Lens for In Vivo Multimodal Microendoscopy.

Multimodal microendoscopes enable co-located structural and molecular measurements in vivo, thus providing useful insights into the pathological changes associated with disease. However, different optical imaging modalities often have conflicting optical requirements for optimal lens design. For example, a high numerical aperture (NA) lens is needed to realize high-sensitivity fluorescence measurements.