Publications by authors named "Haiqiang Qi"

This study aimed to further improve the degradation efficiency of pollutants by electrochemical oxidation system and reduce the consumption of electric energy. A simple method of electrochemical exfoliation was used to modify graphite felt (GF) to prepare an anode material (Ee-GF) with high degradation performance. An anode and cathode cooperative oxidation system was constructed with Ee-GF as the anode and CuFeO/CuO/Cu@EGF as the cathode to efficiently degrade sulfamethoxazole (SMX).

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In this paper, a CuCo-O@CNTs/NF electrode was successfully prepared and used for in-situ degradation of sulfamethoxazole (SMX) in an electro-Fenton-like system. Carbon nanotubes (CNTs) and coral-like copper-cobalt oxides were successively loaded on nickel foam (NF). CNTs contributed to improving the dispersibility and stability of copper-cobalt oxides, and the coral-like copper-cobalt oxide catalyst was anchored on CNTs without any adhesive.

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An iron-copper graphite felt (Fe-Cu/HGF) electrode was successfully prepared by heat treatment and impregnation of graphite felt as the support followed by calcination, and an electro-activated peroxydisulfate (E-PDS) system with Fe-Cu/HGF as the cathode was constructed to degrade Diuron. This system synergistically activated PDS through electrochemical processes and transition metal catalysis. High-valence metal ions could be converted into low-valence metal ions by reduction at the cathode, and low-valence metal ions continuously activated PDS to generate more sulfate radicals (SO) and hydroxyl radicals (OH) to accelerate Diuron degradation.

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Bifunctional cathodes have attracted widespread interest in the heterogeneous electro-Fenton (hetero-EF) process. In this study, the bifunctional composite cathode co-modified with N-doped carbon CoFe alloy (CoFe@NC) and carbon nanotubes (CNTs), designated as CoFe@NC-CNTs/CNTs/NF, integrating hydrogen peroxide (HO) synthesis and catalysis, was prepared for efficient degradation of atrazine (ATZ) under the near-neutral condition (pH = 5.9).

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In this paper, nanoscale CuO particles was successfully anchored at defect sites of carbon nanotubes (CNTs), which doped on three-dimensional copper foam (CF) electrode (CuO@CNTs/CF). The compound as cathode was synthesized via dip-coating and rapid electrodeposition followed by annealing procedure, and conducted in heterogeneous electro-Fenton (EF) system. The CuO@CNTs/CF composites electrode enabled activate O to generate HO in situ and further Cu/CuO synergistic catalysis to produce reactive oxygen species for a broad pH-range via the heterogeneous EF process.

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