Realization of ferromagnetism in the two-dimensional (2D) van der Waals (vdW) crystals opens up a vital route to understand the magnetic ordering in the 2D limit and to design novel spintronics. Here, we report enriched layer-number-dependent magnetotransport properties in the vdW ferromagnet FeGeTe. By studying the magnetoresistance and anomalous Hall effect (AHE) in nanoflakes with thicknesses down to monolayer, we demonstrate that while the bulk crystals exhibit soft ferromagnetism with an in-plane magnetic anisotropy, hard ferromagnetism develops upon thinning, and a perpendicular eas-axis anisotropy is realized in bilayer flakes, which is accompanied by a pronounced enhancement of AHE because of extrinsic mechanisms.
View Article and Find Full Text PDFAs an intriguing topological phase, higher-order topological insulators have attracted tremendous attention, but the candidate materials are limited in artificial and inorganic systems. In this work, we propose a universal approach to search for two-dimensional (2D) second-order topological insulators (SOTIs) in covalent organic frameworks (COFs) with symmetric cores. The underlying mechanism is illustrated through tight-binding calculations in a star lattice, showing the 2D SOTI in an overlooked energy window between two Kagome-bands with four types of nontrivial band structures.
View Article and Find Full Text PDFElemental tellurium, conventionally recognized as a narrow bandgap semiconductor, has recently aroused research interests for exploiting Weyl physics. Chirality is a unique feature of Weyl cones and can support helicity-dependent photocurrent generation, known as circular photogalvanic effect. Here, we report circular photogalvanic effect with opposite signs at two different mid-infrared wavelengths which provides evidence of Weyl-related optical responses.
View Article and Find Full Text PDFTopological physics has been extensively studied in different kinds of bosonic and Fermionic systems, but the coexistence of topological phonons and electrons in one single material has seldom been reported. Recently, graphdiyne has been proposed as a two-dimensional (2D) electronic second-order topological insulator (SOTI). In this work, we found that graphdiyne is equivalent to Kekulé lattice, also realizing a 2D phononic SOTI in both out-of-plane and in-plane modes.
View Article and Find Full Text PDFThe two-dimensional (2D) twisted bilayer materials with van der Waals coupling have ignited great research interests, paving a new way to explore the emergent quantum phenomena by twist degree of freedom. Generally, with the decreasing of twist angle, the enhanced interlayer coupling will gradually flatten the low-energy bands and isolate them by two high-energy gaps at zero and full filling, respectively. Although the correlation and topological physics in the low-energy flat bands have been intensively studied, little information is available for these two emerging gaps.
View Article and Find Full Text PDFRecently, the precise folding of flexible graphene is reported experimentally [ , 2019, 365, 1036-1040], demonstrating an efficient approach to manipulate its electronic and optoelectronic properties. Here, we propose a light-induced high-Chern-number Chern insulator (CI) in the folded graphene. Along both armchair and zigzag folding directions, we demonstrate that there are two-handedness-dependent chiral interface states localized at the curved region.
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