Publications by authors named "Haijie Cai"

High sensitivity, low concentration, and excellent selectivity are pronounced primary challenges for semiconductor gas sensors to monitor acetone from exhaled breath. In this study, nitrogen-doped carbon quantum dots (N-CQDs) with high reactivity were used to activate dandelion-like hierarchical tungsten oxide (WO) microspheres to construct an efficient and stable acetone gas sensor. Benefiting from the synergistic effect of both the abundant active sites provided by the unique dandelion-like hierarchical structure and the high reaction potential generated by the sensitization of the N-CQDs, the resulting 16 wt % N-CQDs/WO sensor shows an ultrahigh response value (/ = 74@1 ppm acetone), low detection limit (0.

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Formaldehyde, a common illegal additive in aquatic products, poses a threat to people's health and lives. In this study, a novel metal oxide semiconductor gas sensor based on AuPd-modified WO nanosheets (NSs) had been developed for the highly efficient detection of formaldehyde. WO NS modified with 2.

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Palladium (Pd)-modified metal oxide semiconductors (MOSs) gas sensors often exhibit unexpected hydrogen (H ) sensing activity through a spillover effect. However, sluggish kinetics over a limited Pd-MOS surface seriously restrict the sensing process. Here, a hollow Pd-NiO/SnO buffered nanocavity is engineered to kinetically drive the H spillover over dual yolk-shell surface for the ultrasensitive H sensing.

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Amorphous/crystalline heterophase engineering is emerging as an attractive strategy to adjust the properties and functions of nanomaterials. Here, we reveal a heterophase interface role by precisely tailoring the crystalline Pt coverage density on an amorphous Ru surface (cPt/aRu) for ultrasensitive HS detection. We found that when the atomic ratio of Pt/Ru increased from 10 to 50%, the loading modes of Pt changed from island coverage (1cPt/aRu) to cross-linkable coverage (3cPt/aRu) and further to dense coverage (5cPt/aRu).

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The unsaturated coordination and abundant active sites endow amorphous metals with tremendous potential in improving metal oxide semiconductors' gas-sensing properties. However, the amorphous materials maintain the metastable status and easily transfer into the lower-active crystals during the gas-sensing process at high working temperatures, significantly limiting their further applications. Here, a bimetal amorphous PtRu catalyst is developed by accurately regulating the introduction of Pt species into amorphous RuO supports to realize the highly active and stable H S gas-sensing detection.

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Low-cost and real-time formaldehyde (HCHO) monitoring is of great importance due to its volatility, extreme toxicity, and ready accessibility. In this work, a low-cost and integrated microelectromechanical system (MEMS) HCHO sensor is developed based on SnO multishell hollow microspheres loaded with a bimetallic PdPt (PdPt/SnO-M) sensitizer. The MEMS sensor exhibits a high sensitivity to HCHO ((/ - 1) % = 83.

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Microorganisms with high tetracycline (TC) degradation efficiencies are required for biological processes for TC-containing wastewater treatment. With multiple enrichment cultures, a TC-degrading strain TR5 was isolated from chicken manure mixture in a large broiler farm, which was identified as Klebsiella pneumoniae by 16S rRNA gene sequencing and biochemical properties. Strain TR5 could degrade TC quickly (∼90% within 36 h) with the initial TC concentration of 200 mg/L under optimized conditions via single-factor experiment coupled with RSM.

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As a foodborne bacterium, () can cause serious diseases and even death to weak people. 3-Hydroxy-2-butanone (3H-2B) has been proven to be a biomarker for exhalation of LM. Detection of 3H-2B is a fast and effective method for determining whether the food is infected.

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has been recognized as one of the extremely hazardous and potentially life-threatening food-borne pathogens, its real-time monitoring is of great importance to human health. Herein, a simple and effective method based on platinum sensitized tin dioxide semiconductor gas sensors has been proposed for selective and rapid detection of . Pt doped SnO nanospheres with particular mesoporous hollow structure have been synthesized successfully through a robust and template-free approach and used for the detection of 3-hydroxy-2-butanone biomarker of .

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