Optical evidence of the chiral magnetic anomaly in the Weyl semimetal TaAs.

Chiral pumping from optical electric fields oscillating at terahertz frequencies is observed in the Weyl material TaAs with electric and magnetic fields aligned along both the and axes. Free-carrier spectral weight enhancement is measured directly, confirming theoretical expectations of chiral pumping. A departure from linear field dependence of the Drude weight is observed at the highest fields in the quantum limit, providing evidence of field-dependent Fermi velocity of the chiral Landau level.

Terahertz photoresponse of black phosphorus.

Two-dimensional black phosphorus is a new material that has gained widespread interest as an active material for optoelectronic applications. It features high carrier mobility that allows for efficient free-carrier absorption of terahertz radiation, even though the photon energy is far below the bandgap energy. Here we present an efficient and ultrafast terahertz detector, based on exfoliated multilayer flakes of black phosphorus.

Tunable Ultrafast Thermal Relaxation in Graphene Measured by Continuous-Wave Photomixing.

Hot electron effects in graphene are significant because of graphene's small electronic heat capacity and weak electron-phonon coupling, yet the dynamics and cooling mechanisms of hot electrons in graphene are not completely understood. We describe a novel photocurrent spectroscopy method that uses the mixing of continuous-wave lasers in a graphene photothermal detector to measure the frequency dependence and nonlinearity of hot-electron cooling in graphene as a function of the carrier concentration and temperature. The method offers unparalleled sensitivity to the nonlinearity, and probes the ultrafast cooling of hot carriers with an optical fluence that is orders of magnitude smaller than in conventional time-domain methods, allowing for accurate characterization of electron-phonon cooling near charge neutrality.

Infrared phonons as a probe of spin-liquid states in herbertsmithite ZnCu(OH)Cl.

We report on temperature dependence of the infrared reflectivity spectra of a single crystalline herbertsmithite in two polarizations-parallel and perpendicular to the kagome plane of Cu atoms. We observe anomalous broadening of the low frequency phonons possibly caused by fluctuations in the exotic dynamical magnetic order of the spin liquid.

Nonlinear Terahertz Absorption of Graphene Plasmons.

Subwavelength graphene structures support localized plasmonic resonances in the terahertz and mid-infrared spectral regimes. The strong field confinement at the resonant frequency is predicted to significantly enhance the light-graphene interaction, which could enable nonlinear optics at low intensity in atomically thin, subwavelength devices. To date, the nonlinear response of graphene plasmons and their energy loss dynamics have not been experimentally studied.

Pulsed Near-IR Photoresponse in a Bi-metal Contacted Graphene Photodetector.

We use an ultra-fast near-infrared pulse coincidence technique to study the time, temperature, and power dependence of the photoresponse of a bi-metal contacted graphene photodetector. We observe two components of the photovoltage signal. One component is gate-voltage dependent, linear in power at room temperature and sub-linear at low temperature-consistent with the hot-electron photothermoelectric effect due to absorption in the graphene.

Tunable Terahertz Hybrid Metal-Graphene Plasmons.

We report here a new type of plasmon resonance that occurs when graphene is connected to a metal. These new plasmon modes offer the potential to incorporate a tunable plasmonic channel into a device with electrical contacts, a critical step toward practical graphene terahertz optoelectronics. Through theory and experiments, we demonstrate, for example, anomalously high resonant absorption or transmission when subwavelength graphene-filled apertures are introduced into an otherwise conductive layer.

Plasmon-Enhanced Terahertz Photodetection in Graphene.

We report a large area terahertz detector utilizing a tunable plasmonic resonance in subwavelength graphene microribbons on SiC(0001) to increase the absorption efficiency. By tailoring the orientation of the graphene ribbons with respect to an array of subwavelength bimetallic electrodes, we achieve a condition in which the plasmonic mode can be efficiently excited by an incident wave polarized perpendicular to the electrode array, while the resulting photothermal voltage can be observed between the outermost electrodes.

Sensitive room-temperature terahertz detection via the photothermoelectric effect in graphene.

Terahertz radiation has uses in applications ranging from security to medicine. However, sensitive room-temperature detection of terahertz radiation is notoriously difficult. The hot-electron photothermoelectric effect in graphene is a promising detection mechanism; photoexcited carriers rapidly thermalize due to strong electron-electron interactions, but lose energy to the lattice more slowly.

Approaching the limits of transparency and conductivity in graphitic materials through lithium intercalation.

Various band structure engineering methods have been studied to improve the performance of graphitic transparent conductors; however, none has demonstrated an increase of optical transmittance in the visible range. Here we measure in situ optical transmittance spectra and electrical transport properties of ultrathin graphite (3-60 graphene layers) simultaneously during electrochemical lithiation/delithiation. On intercalation, we observe an increase of both optical transmittance (up to twofold) and electrical conductivity (up to two orders of magnitude), strikingly different from other materials.

Impact of interface roughness on the performance of broadband blackbody absorber based on dielectric-metal film multilayers.

We report on factors affecting the performance of a broadband, mid-IR absorber based on multiple, alternating dielectric / metal layers. In particular, we investigate the effect of interface roughness. Atomic layer deposition produces both a dramatic suppression of the interface roughness and a significant increase in the optical absorption as compared to devices fabricated using a conventional thermal evaporation source.

Photothermal response in dual-gated bilayer graphene.

The photovoltaic and bolometric photoresponse in gapped bilayer graphene was investigated by optical and transport measurements. A pulse coincidence technique at 1.5 μm was used to measure the response times as a function of temperature.

Dual-gated bilayer graphene hot-electron bolometer.

Graphene is an attractive material for use in optical detectors because it absorbs light from mid-infrared to ultraviolet wavelengths with nearly equal strength. Graphene is particularly well suited for bolometers-devices that detect temperature-induced changes in electrical conductivity caused by the absorption of light-because its small electron heat capacity and weak electron-phonon coupling lead to large light-induced changes in electron temperature. Here, we demonstrate a hot-electron bolometer made of bilayer graphene that is dual-gated to create a tunable bandgap and electron-temperature-dependent conductivity.

Carbon nanotube quantum dots as highly sensitive terahertz-cooled spectrometers.

Terahertz technology has recently emerged as a highly sought-after and versatile scientific tool in many fields, including medical imaging, security screening, and wireless communication. However, scientific progress has been hindered by the lack of sources and detectors in this frequency range, thereby known as the terahertz gap. Here, we show that carbon nanotube quantum dots coupled to antennas are extremely sensitive, broad-band, terahertz quantum detectors with spectral resolution.

Broadband and mid-infrared absorber based on dielectric-thin metal film multilayers.

We propose a periodic multilayer structure of dielectric and metal interlayers to achieve a near-perfect broadband absorber of mid-infrared radiation. We examine the influence of four factors on its performance: (1) the interlayer metal conductance, (2) the number of dielectric layers, (3) a nanopatterned antireflective layer, and (4) a reflective metallic bottom layer for backreflection. Absorption characteristics greater than 99% of the 300 K and 500 K blackbody spectra are found for the optimized structures.

Suppression of long-range collective effects in meta-surfaces formed by plasmonic antenna pairs.

The collective effects in a periodic array of plasmonic double-antenna meta-molecules are studied. We experimentally observe that the collective behavior in this structure substantially differs from the one observed in their single-antenna counterparts. This behavior is explained using an analytical dipole model.

Topological quantization in units of the fine structure constant.

Fundamental topological phenomena in condensed matter physics are associated with a quantized electromagnetic response in units of fundamental constants. Recently, it has been predicted theoretically that the time-reversal invariant topological insulator in three dimensions exhibits a topological magnetoelectric effect quantized in units of the fine structure constant α=e²/ℏc. In this Letter, we propose an optical experiment to directly measure this topological quantization phenomenon, independent of material details.

Bianisotropy and spatial dispersion in highly anisotropic near-infrared resonator arrays.

We measure, simulate, and analyze the optical transmission through arrays of Ag nanorod pairs and U-shaped nanostructures as a function of polarization and angle of incidence. The bianisotropic nature of the metamaterials is exhibited in data and in simulations, and we argue that the electric field rather than the magnetic field excites the low frequency "magnetic" mode. We also observe spatial dispersion in the form of frequency shifts as a function of incident angle which we attribute to coupling effects between neighboring structures.

Simultaneous measurement of circular dichroism and Faraday rotation at terahertz frequencies utilizing electric field sensitive detection via polarization modulation.

A far-infrared system measures the full complex Faraday angle, the rotation as well as the ellipticity, with an unprecedented accuracy of 10 microrad/T. The system operates on several far-infrared laser lines in the spectral range from 0.3 to 6 THz and produces results as a continuous function of temperature from 10 to 310 K and applied fields between +/-8 T.

Origin of electromagnon excitations in multiferroic RMnO3.

Electromagnon excitations in multiferroic orthorhombic RMnO3 are shown to result from the Heisenberg coupling between spins despite the fact that the static polarization arises from the much weaker Dzyaloshinskii-Moriya exchange interaction. We present a model incorporating the structural characteristics of this family of manganites that is confirmed by far infrared transmission data as a function of temperature and magnetic field and inelastic neutron scattering results. A deep connection is found between the magnetoelectric dynamics of the spiral phase and the static magnetoelectric coupling in the collinear E phase of this family of manganites.

Optical plasmonic resonances in split-ring resonator structures: an improved LC model.

We systematically investigate the resonant behavior of arrays of Ag nano-structures ranging from isolated simple rods, to U-shapes, to single split ring structures. We show that the lowest order plasmonic resonance associated with a rod red shifts as we create a U and SRR into the position normally associated with a simple LC mode. A second mode red shifts and grows in intensity as we extend the arms of the U-shape, and a third mode appears in the spectra as we close the arms and form a split ring structure.

Effective masses in a strongly anisotropic fermi liquid.

Motivated by the recent experimental observation of quantum oscillations in the underdoped cuprates, we study the cyclotron and infrared Hall effective masses in an anisotropic Fermi liquid characterized by an angle-dependent quasiparticle residue Z_{q}. Our primary motivation is to explain the relatively large value of the cyclotron mass observed experimentally and its relation with the effective Hall mass. Using a phenomenological model of an anisotropic Fermi liquid, we find that the cyclotron mass is enhanced by a factor 1/Z_{q}, while the effective Hall mass is proportional to Z_{q}/Z_{q};{2}, where cdots, three dots, centered implies an averaging over the Fermi surface.

Near-field evidence for ferromagnetic "nanoneedles" in Nd1/2Sr1/2MnO3.

We report on the near-field optical microscopic (NSOM) imaging of single-crystal Nd1/2Sr1/2MnO3 near the first-order phase transition from the CE-type charge-ordered insulator (COI) to the ferromagnetic metal (FMM) at 165 K. Using polarized light, the measurements are sensitive to twin domains through optical anisotropy and to hysteretic inhomogeneous strain associated with the phase transition. Optical evidence for strain relaxation and multiphase coexistence is observed through the transition from 150 to 165 K.

Electromagnons in multiferroic YMn2O5 and TbMn2O5.

Based on temperature dependent far infrared transmission spectra of YMn2O5 and TbMn2O5 single crystals, we report the observation of electric dipole-active magnetic excitations, or electromagnons, in these multiferroics. Electromagnons are found to be directly responsible for the steplike anomaly of the static dielectric constant at the commensurate--incommensurate magnetic transition and are the origin of the colossal magneto-dielectric effect reported in these multiferroics.