Diffractive Imaging of C_{60} Structural Deformations Induced by Intense Femtosecond Midinfrared Laser Fields.

Theoretical studies indicated that C_{60} exposed to linearly polarized intense infrared pulses undergoes periodic cage structural distortions with typical periods around 100 fs (1  fs=10^{-15}  s). Here, we use the laser-driven self-imaging electron diffraction technique, previously developed for atoms and small molecules, to measure laser-induced deformation of C_{60} in an intense 3.6  μm laser field.

10 W CEP-stable few-cycle source at 2 µm with 100 kHz repetition rate.

We developed a high repetition rate optical parametric chirped-pulse amplification (OPCPA) laser system based on fiber-laser-seeded Innoslab to generate few-cycle pulses around 2 µm with passively stable carrier-envelope phase (CEP) by difference frequency generation (DFG). Incorporating a piezo mirror before the DFG stage permits rapid CEP control. The OPCPA system is seeded by a stable supercontinuum generated in bulk material with the picosecond Innoslab pulses.

Discrete dispersion scanning as a simple method for broadband femtosecond pulse characterization.

A simple and easy to implement technique for femtosecond pulse characterization is proposed and experimentally verified. It is based on the introduction of a known amount of dispersion (by controlling the number of passes through dispersive material) and subsequent recording of the spectral positions of second harmonic peaks obtained in a non-linear crystal. Such dependence allows for direct retrieval of the pulse spectral phase.