Digital Light 3D Printing of Double Thermoplastics with Customizable Mechanical Properties and Versatile Reprocessability.

Digital light processing (DLP) is a 3D printing technology offering high resolution and speed. Printable materials are commonly based on multifunctional monomers, resulting in the formation of thermosets that usually cannot be reprocessed or recycled. Some efforts are made in DLP 3D printing of thermoplastic materials.

Photonic Crystal-Integrated Optoelectronic Devices with Naked-Eye Visualization and Digital Readout for High-Resolution Detection of Ultratrace Analytes.

The detection of ultratrace analytes is highly desirable for the non-invasive monitoring of human diseases. However, a major challenge is fast, naked-eye, high-resolution ultratrace detection. Herein, a rectangular 3D composite photonic crystal (PC)-based optoelectronic device is first designed that combines the sensitivity-enhancing effects of PCs and optoelectronic devices with fast and real-time digital monitoring.

Multicomponent and multifunctional integrated miniature soft robots.

Miniature soft robots with elaborate structures and programmable physical properties could conduct micromanipulation with high precision as well as access confined and tortuous spaces, which promise benefits in medical tasks and environmental monitoring. To improve the functionalities and adaptability of miniature soft robots, a variety of integrated design and fabrication strategies have been proposed for the development of miniaturized soft robotic systems integrated with multicomponents and multifunctionalities. Combining the latest advancement in fabrication technologies, intelligent materials and active control methods enable these integrated robotic systems to adapt to increasingly complex application scenarios including precision medicine, intelligent electronics, and environmental and proprioceptive sensing.

Electrochemical CO reduction to ethylene by ultrathin CuO nanoplate arrays.

Electrochemical reduction of CO to multi-carbon fuels and chemical feedstocks is an appealing approach to mitigate excessive CO emissions. However, the reported catalysts always show either a low Faradaic efficiency of the C product or poor long-term stability. Herein, we report a facile and scalable anodic corrosion method to synthesize oxygen-rich ultrathin CuO nanoplate arrays, which form Cu/CuO heterogeneous interfaces through self-evolution during electrocatalysis.

Digital Light Processing 3D Printing of Enhanced Polymers via Interlayer Welding.

Digital light processing (DLP) 3D printing is advantageous in high printing efficiency and printing resolution for fabricating complex structures across various applications. However, the layer-by-layer curing manner of DLP leads to weak interlayer adhesion and the anisotropic mechanical properties of printed objects. Here, linear polymers are introduced into commercial resins to weld the interlayer by the diffusion and entanglement of linear polymers after DLP printing via heat treatment.

Superior Hard but Quickly Reversible Si-O-Si Network Enables Scalable Fabrication of Transparent, Self-Healing, Robust, and Programmable Multifunctional Nanocomposite Coatings.

A coating with programmable multifunctionality based on application requirements is desirable. However, it is still a challenge to prepare a hard and flexible coating with a quick self-healing ability. Here, a hard but reversible Si-O-Si network enabled by aminopropyl-functionalized poly(silsesquioxane) and triethylamine (TEA) was developed.

Digital Light Processing 3D Printing of Healable and Recyclable Polymers with Tailorable Mechanical Properties.

Three-dimensional (3D) printing is becoming a revolutionary technique across various fields. Especially, digital light processing (DLP) 3D printing shows advantages of high resolution and high efficiency. However, multifunctional monomers are commonly used to meet the rapid liquid-to-solid transformation during DLP printing, and the extensive production of unreprocessable thermosets will lead to resource waste and environmental problems.

Construction of a Different Polymer Chain Structure to Study π-π Interaction between Polymer and Reduced Graphene Oxide.

In this work, a different polymer chain structure was synthesized to study π-π interactions between polymer and reduced graphene oxide (RGO). Polymers with different chain structures were obtained from free radical copolymerization of styrene with 4-cyanostyrene (containing substituted phenyl rings) and 2-vinylnaphthalene (containing naphthalene rings). In this work, the polystyrene, poly(styrene--4-cyanostyrene) and poly(styrene--2-vinylnaphthalene) were named as PS, PSCN and PSNP, respectively.