Publications by authors named "Georg Von Freymann"

Article Synopsis
  • Spintronic terahertz emitters (STEs) are powerful terahertz sources that can operate across a wide range of pumping frequencies, yet their performance is ultimately limited by their optical damage threshold.
  • Recent advancements in technology require STEs to pump at higher megahertz rates rather than the traditional kilohertz rates, highlighting a gap in research on this topic.
  • The study introduces a new classification of the optical damage threshold based on repetition rates and identifies temperature-driven inter-layer diffusion as the main failure cause, offering insights for improving STE performance in future applications.
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Electric field induced second harmonic (EFISH) measurements are performed on thin films of arsenic sulfide deposited on chromium coated fused silica substrates by thermal evaporation of amorphous AsS bulk material. EFISH allows to widely tune the second-order optical susceptibility (χ). An observed shift of the minimum of the second harmonic generation (SHG) intensity away from 0 V reveals a non-EFISH bulk χ, which is unexpected for amorphous materials.

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The remagnetization process after ultrafast demagnetization can be described by relaxation mechanisms between the spin, electron, and lattice reservoirs. Thereby, collective spin excitations in form of spin waves and their angular momentum transfer play an important role on the longer timescales. In this work, we address the question whether the magnitude of demagnetization-the so-called quenching-affects the coherency and the phase of the excited spin waves.

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Resistivity is one of the most important characteristics in the semiconductor industry. The most common way to measure resistivity is the four-point probe method, which requires physical contact with the material under test. Terahertz time domain spectroscopy, a fast and non-destructive measurement method, is already well established in the characterization of dielectrics.

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Terahertz tomography is a promising method among non-destructive inspection techniques to detect faults and defects in dielectric samples. Recently, image quality was improved significantly through the incorporation of information and off-axis data. However, this improvement has come at the cost of increased measurement time.

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Considering light transport in disordered media, the medium is often treated as an effective medium requiring accurate evaluation of an effective refractive index. Because of its simplicity, the Maxwell-Garnett (MG) mixing rule is widely used, although its restriction to particles much smaller than the wavelength is rarely satisfied. Using 3D finite-difference time-domain simulations, we show that the MG theory indeed fails for large particles.

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Spintronic terahertz emitters promise terahertz sources with an unmatched broad frequency bandwidth that are easy to fabricate and operate, and therefore easy to scale at low cost. However, current experiments and proofs of concept rely on free-space ultrafast pump lasers and rather complex benchtop setups. This contrasts with the requirements of widespread industrial applications, where robust, compact, and safe designs are needed.

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Since temperature and its spatial, and temporal variations affect a wide range of physical properties of material systems, they can be used to create reconfigurable spatial structures of various types in physical and biological objects. This paper presents an experimental optical setup for creating tunable two-dimensional temperature patterns on a micrometer scale. As an example of its practical application, we have produced temperature-induced magnetization landscapes in ferrimagnetic yttrium iron garnet films and investigated them using micro-focused Brillouin light scattering spectroscopy.

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Terahertz time-domain spectroscopy systems based on resonator-internal repetition-rate modulation, such as SLAPCOPS and ECOPS, rely on electronic phase detectors which are typically prone to exhibit both a non-negligible random and systematic timing error. This limits the quality of the recorded information significantly. Here, we present the results of our recent attempt to reduce these errors in our own electronic phase detection systems.

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A method for direct fabrication of 3D silver microstructures with high fabrication throughput on virtually any substrate is presented. The method is based on laser-induced photoreduction of silver ions to silver atoms, supported by nucleation, substrate functionalization and a multiple exposure fabrication process. The combination of the novel photosensitive suspension and the novel fabrication scheme enables effective fabrication speeds of up to 1 cm per second, with a minimum structure size of less than 1 μm, a resolution of more than 750 lines/mm and a resistivity of 3.

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Sensing with undetected photons allows access to spectral regions with simultaneous detection of photons of another region and is based on nonlinear interferometry. To obtain the full information of a sample, the corresponding interferogram has to be analyzed in terms of amplitude and phase, which has been realized so far by multiple measurements followed by phase variation. Here, we present a polarization-optics-based phase-quadrature implementation in a nonlinear interferometer for imaging with undetected photons in the infrared region.

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The rich physical properties of multiatomic crystals are determined, to a significant extent, by the underlying geometry and connectivity of atomic orbitals. The mixing of orbitals with distinct parity representations, such as s and p orbitals, has been shown to be useful for generating systems that require alternating phase patterns, as with the sign of couplings within a lattice. Here we show that by breaking the symmetries of such mixed-orbital lattices, it is possible to generate synthetic magnetic flux threading the lattice.

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Microscale 3D printing technologies have been of increasing interest in industry and research for several years. Unfortunately, the fabricated structures always deviate from the respective expectations, often caused by the physico-chemical properties during and after the printing process. Here, we show first steps towards a simple, fast and easy to implement algorithm to predict the final structure topography for multi-photon lithography - also known as Direct Laser Writing (DLW).

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Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the light, represented by the number of photons, their phase provides important information and enables a plethora of applications. We present a phase-sensitive measurement method in the terahertz spectral range by only detecting visible light.

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We present a robust, fiber-based endoscope with a silver direct-laser-written structure for radio frequency (RF) emission next to the optical fiber facet. Thereby, we are able to excite and probe a sample, such as nitrogen-vacancy (NV) centers in diamond, with RF and optical signals simultaneously and specifically measure the fluorescence of the sample fully through the fiber. At our targeted frequency range of around 2.

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In the past decade, symmetry-protected bound states in the continuum (BICs) have proven to be an important design principle for creating and enhancing devices reliant upon states with high-quality () factors, such as sensors, lasers, and those for harmonic generation. However, as we show, current implementations of symmetry-protected BICs in photonic crystal slabs can only be found at the center of the Brillouin zone and below the Bragg diffraction limit, which fundamentally restricts their use to single-frequency applications. By microprinting a three-dimensional (3D) photonic crystal structure using two-photon polymerization, we demonstrate that this limitation can be overcome by altering the radiative environment surrounding the slab to be a 3D photonic crystal.

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Weyl points are robust point degeneracies in the band structure of a periodic material, which act as monopoles of Berry curvature. They have been at the forefront of research in three-dimensional topological materials as they are associated with novel behavior both in the bulk and on the surface. Here, we present the experimental observation of a charge-2 photonic Weyl point in a low-index-contrast photonic crystal fabricated by two-photon polymerization.

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Artificial gauge fields the control over the dynamics of uncharged particles by engineering the potential landscape such that the particles behave as if effective external fields are acting on them. Recent years have witnessed a growing interest in artificial gauge fields generated either by the geometry or by time-dependent modulation, as they have been enablers of topological phenomena and synthetic dimensions in many physical settings, e.g.

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The detection of terahertz photons by using silicon-based devices enabled by visible photons is one of the fundamental ideas of quantum optics. Here, we present a classical detection principle using optical upconversion of terahertz photons to the near-infrared spectral range in the picosecond pulse regime, which finally enables the detection with a conventional sCMOS camera. By superimposing terahertz and optical pump pulses in a periodically poled lithium-niobate crystal, terahertz photons at 0.

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The discovery of artificial gauge fields controlling the dynamics of uncharged particles that otherwise elude the influence of standard electromagnetic fields has revolutionised the field of quantum simulation. Hence, developing new techniques to induce these fields is essential to boost quantum simulation of photonic structures. Here, we experimentally demonstrate the generation of an artificial gauge field in a photonic lattice by modifying the topological charge of a light beam, overcoming the need to modify the geometry along the evolution or impose external fields.

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Quantum sensing is highly attractive for accessing spectral regions in which the detection of photons is technically challenging: Sample information is gained in the spectral region of interest and transferred via biphoton correlations into another spectral range, for which highly sensitive detectors are available. This is especially beneficial for terahertz radiation, where no semiconductor detectors are available and coherent detection schemes or cryogenically cooled bolometers have to be used. Here, we report on the first demonstration of quantum sensing in the terahertz frequency range in which the terahertz photons interact with a sample in free space and information about the sample thickness is obtained by the detection of visible photons.

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We present an overview of functional metallic microstructures fabricated via direct laser writing out of the liquid phase. Metallic microstructures often are key components in diverse applications such as, e.g.

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