Sustainable leather alternatives: High-performance and dyeable bio-based materials from fungal chitin and tannic acid.

Leather alternatives (LAs) offer a promising solution to address the environmental and ethical concerns associated with traditional leather production relying animal hides and chemical tanning agents. However, synthetic polymer-based LAs, such as polyurethane and polyvinyl chloride, have limited broader applications due to their complex manufacture process, high emission of volatile organic compounds, and poor biodegradability. Herein, we present the development of biomass-based LAs fabricated by combining two low-cost natural components - fungal chitin and plant polyphenols (i.