Understanding and Mitigating the Degradation of Perovskite Solar Cells Based on a Nickel Oxide Hole Transport Material during Damp Heat Testing.

The development of stable materials, processable on a large area, is a prerequisite for perovskite industrialization. Beyond the perovskite absorber itself, this should also guide the development of all other layers in the solar cell. In this regard, the use of NiO as a hole transport material (HTM) offers several advantages, as it can be deposited with high throughput on large areas and on flat or textured surfaces via sputtering, a well-established industrial method.

Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap.

Polariton lasers are coherent light sources based on the condensation of exciton-polaritons in semiconductor microcavities, which occurs either in the kinetic or thermodynamic (Bose-Einstein) regime. Besides their fundamental interest, polariton lasers have the potential of extremely low operating thresholds. Here, we demonstrate ultra-low threshold polariton lasing at room temperature, using an all-dielectric, GaN membrane-based microcavity, with a spontaneously-formed zero-dimensional trap.

Coupled counterrotating polariton condensates in optically defined annular potentials.

Polariton condensates are macroscopic quantum states formed by half-matter half-light quasiparticles, thus connecting the phenomena of atomic Bose-Einstein condensation, superfluidity, and photon lasing. Here we report the spontaneous formation of such condensates in programmable potential landscapes generated by two concentric circles of light. The imposed geometry supports the emergence of annular states that extend up to 100 μm, yet are fully coherent and exhibit a spatial structure that remains stable for minutes at a time.

Optical superfluid phase transitions and trapping of polariton condensates.

Semiconductor microcavities are used to support freely flowing polariton quantum liquids allowing the direct observation and optical manipulation of macroscopic quantum states. Incoherent optical excitation at a point produces radially expanding condensate clouds within the planar geometry. By using arbitrary configurations of multiple pump spots, we discover a geometrically controlled phase transition, switching from the coherent phase-locking of multiple condensates to the formation of a single trapped condensate.

Geometrically locked vortex lattices in semiconductor quantum fluids.

Macroscopic quantum states can be easily created and manipulated within semiconductor microcavity chips using exciton-photon quasiparticles called polaritons. Besides being a new platform for technology, polaritons have proven to be ideal systems to study out-of-equilibrium condensates. Here we harness the photonic component of such a semiconductor quantum fluid to measure its coherent wavefunction on macroscopic scales.