Publications by authors named "Fulizi Xiong"

Background: Low-cost sensor networks for monitoring air pollution are an effective tool for expanding spatial resolution beyond the capabilities of existing state and federal reference monitoring stations. However, low-cost sensor data commonly exhibit non-linear biases with respect to environmental conditions that cannot be captured by linear models, therefore requiring extensive lab calibration. Further, these calibration models traditionally produce point estimates or uniform variance predictions which limits their downstream in exposure assessment.

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As part of our low-cost sensor network, we colocated multipollutant monitors containing sensors for particulate matter, carbon monoxide, ozone, nitrogen dioxide, and nitrogen monoxide at a reference field site in Baltimore, MD, for 1 year. The first 6 months were used for training multiple regression models, and the second 6 months were used to evaluate the models. The models produced accurate hourly concentrations for all sensors except ozone, which likely requires nonlinear methods to capture peak summer concentrations.

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The distribution and dynamics of atmospheric pollutants are spatiotemporally heterogeneous due to variability in emissions, transport, chemistry, and deposition. To understand these processes at high spatiotemporal resolution and their implications for air quality and personal exposure, we present custom, low-cost air quality monitors that measure concentrations of contaminants relevant to human health and climate, including gases (e.g.

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Low-cost air pollution monitors are increasingly being deployed to enrich knowledge about ambient air-pollution at high spatial and temporal resolutions. However, unlike regulatory-grade (FEM or FRM) instruments, universal quality standards for low-cost sensors are yet to be established and their data quality varies widely. This mandates thorough evaluation and calibration before any responsible use of such data.

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The identification and quantification of gas-phase organic compounds, such as volatile organic compounds (VOCs), frequently use gas chromatography (GC), which typically requires high-purity compressed gases. We have developed a new instrument for trace-concentration measurements of VOCs and intermediate-volatility compounds of up to 14 carbon atoms in a fully automated (computer-free), independent, low-cost, compact GC-based system for the quantitative analysis of complex mixtures without the need for compressed, high-purity gases or expensive detectors. Through adsorptive analyte preconcentration, vacuum GC, photoionization detectors, and need-based water-vapor control, we enable sensitive and selective measurements with picogram-level limits of detection (i.

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Due to the rapid development of low-cost air-quality sensors, a rigorous scientific evaluation has not been conducted for many available sensors. We evaluated three Plantower PMS A003 sensors when exposed to eight particulate matter (PM) sources (i.e.

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