The strong metal-support interaction (SMSI) in supported catalysts plays a dominant role in catalytic degradation, upgrading, and remanufacturing of environmental pollutants. Previous studies have shown that SMSI is crucial in supported catalysts' activity and stability. However, for redox reactions catalyzed in environmental catalysis, the enhancement mechanism of SMSI-induced oxygen vacancy and electron transfer needs to be clarified.
View Article and Find Full Text PDFThis study comprehensively investigated the impact of dust storms (DSs) on downstream cities, by selecting representative DS events. In this paper, we discussed the characteristics of meteorological conditions, air pollutants, PM components, and their influence on sulfate formation mechanisms. During DSs, strong winds, reaching speeds of up to 10 m/s, led to significant increases in PM and PM, with maximum concentrations of 2684.
View Article and Find Full Text PDFThe arbitrary disposal of used brake pads from motor vehicles has resulted in severe heavy metal pollution and resource wastage, highlighting the urgent need to explore the significant untapped potential of these discarded materials. In this study, The in-situ growth of highly dispersed FeO nanocrystals was achieved by simple oxidation annealing of brake pad debris(BPD). Interestingly, Cu remained unoxidized and acted as a "valence state transformation bridge of FeO" to construct the "triple Fe-C-Cu sites".
View Article and Find Full Text PDFWe report a novel graphene oxide quantum dot (GOQD)-sensitized porous TiO microsphere for efficient photoelectric conversion. Electro-chemical analysis along with the Mott-Schottky equation reveals conductivity type and energy band structure of the two semiconductors. Based on their energy band structures, visible light-induced electrons can transfer from the p-type GOQD to the n-type TiO.
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