Particular frost patterns on natural leaves had prompted Yao et al. [Y. Yao .
View Article and Find Full Text PDFPrimary biological aerosol particles (PBAP) play an important role in the climate system, facilitating the formation of ice within clouds, consequently PBAP may be important in understanding the rapidly changing Arctic. Within this work, we use single-particle fluorescence spectroscopy to identify and quantify PBAP at an Arctic mountain site, with transmission electronic microscopy analysis supporting the presence of PBAP. We find that PBAP concentrations range between 10-10 L and peak in summer.
View Article and Find Full Text PDFWe examined ice-nucleating particles (INPs) in the plumes of the Tocantins and Amazon rivers, which drain watersheds with different proportions of degraded land. The concentration of INPs active at -15°C (INP) was an order of magnitude lower in the Tocantins (mean = 13.2 ml; s.
View Article and Find Full Text PDFIce nucleating particles (INP) active at a few degrees below 0°C are produced by a range of organisms and released into the environment. They may affect cloud properties and precipitation when becoming airborne. So far, our knowledge about sources of biological INP is based on grab samples of vegetation, soil or water studied in the laboratory.
View Article and Find Full Text PDFIce nucleation in cold clouds is a decisive step in the formation of rain and snow. Observations and modelling suggest that variations in the concentrations of ice nucleating particles (INPs) affect timing, location and amount of precipitation. A quantitative description of the abundance and variability of INPs is crucial to assess and predict their influence on precipitation.
View Article and Find Full Text PDFLandscapes influence precipitation via the water vapor and energy fluxes they generate. Biologically active landscapes also generate aerosols containing microorganisms, some being capable of catalyzing ice formation and crystal growth in clouds at temperatures near 0 °C. The resulting precipitation is beneficial for the growth of plants and microorganisms.
View Article and Find Full Text PDFRapid Commun Mass Spectrom
May 2013
Rationale: Natural abundance δ(15) N values in soil samples analysed by isotope ratio mass spectrometry (IRMS) are often used to confirm a perturbation after it has been indicated by other parameters. We propose a concept of how δ(15)N values may a priori indicate a perturbation.
Methods: We analysed the δ(15)N values and C:N ratios of 102 soil samples from five regions in northern Eurasia by using an elemental analyser coupled to an isotope ratio mass spectrometer.
Rapid Commun Mass Spectrom
March 2011
The impact of fire on the nitrogen (N) cycle of natural ecosystems is arguable. Here we report and interpret an observation from boreal ecosystems in the Lena River basin, Sakha Republic (Yakutia), Russian Federation. Different types of permafrost soil (0-30 cm depth) were sampled along transects (60-150 m length) from the forest edge towards the centre of four separate thermokarst depressions under grassland.
View Article and Find Full Text PDFNitrous oxide (N(2)O) is a major greenhouse gas that is mainly produced but also reduced by microorganisms in soils. We determined factors for N and O isotope fractionation during the reduction of N(2)O to N(2) in soil in a flow-through incubation experiment. The absolute value of the fractionation factors decreased with increasing reaction rate constant.
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