Spectral control of nonclassical light pulses using an integrated thin-film lithium niobate modulator.

Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator.

Surface Plasmon Enhanced Upconversion Fluorescence in Short-Wave Infrared for In Vivo Imaging of Ovarian Cancer.

Short-wave infrared (SWIR; 850-1700 nm) upconversion fluorescence enables "autofluorescence-free" imaging with minimal tissue scattering, yet it is rarely explored due to the lack of strongly emissive SWIR upconversion fluorophores. In this work, we apply SWIR upconversion fluorescence for in vivo imaging with exceptional image contrast. Gold nanorods (AuNRs) are used to enhance the SWIR upconversion emission of small organic dyes, forming a AuNR-dye nanocomposite (NC).

Spectrally separable photon-pair generation in dispersion engineered thin-film lithium niobate.

Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band.

Experimental Demonstration of Conjugate-Franson Interferometry.

Franson interferometry is a well-known quantum measurement technique for probing photon-pair frequency correlations that is often used to certify time-energy entanglement. We demonstrate, for the first time, the complementary technique in the time basis called conjugate-Franson interferometry. It measures photon-pair arrival-time correlations, thus providing a valuable addition to the quantum toolbox.

Single-photon frequency shifting with a quadrature phase-shift keying modulator.

Deterministic frequency manipulation of single photons is an essential tool for quantum communications and quantum networks. We demonstrate a 15.65 GHz frequency shift for classical and nonclassical light using a commercially available quadrature phase-shift keying modulator.

Seeing around corners with edge-resolved transient imaging.

Non-line-of-sight (NLOS) imaging is a rapidly growing field seeking to form images of objects outside the field of view, with potential applications in autonomous navigation, reconnaissance, and even medical imaging. The critical challenge of NLOS imaging is that diffuse reflections scatter light in all directions, resulting in weak signals and a loss of directional information. To address this problem, we propose a method for seeing around corners that derives angular resolution from vertical edges and longitudinal resolution from the temporal response to a pulsed light source.

Resolving Photon Numbers Using a Superconducting Nanowire with Impedance-Matching Taper.

Time- and number-resolved photon detection is crucial for quantum information processing. Existing photon-number-resolving (PNR) detectors usually suffer from limited timing and dark-count performance or require complex fabrication and operation. Here, we demonstrate a PNR detector at telecommunication wavelengths based on a single superconducting nanowire with an integrated impedance-matching taper.

Large-alphabet encoding for higher-rate quantum key distribution.

The manipulation of high-dimensional degrees of freedom provides new opportunities for more efficient quantum information processing. It has recently been shown that high-dimensional encoded states can provide significant advantages over binary quantum states in applications of quantum computation and quantum communication. In particular, high-dimensional quantum key distribution enables higher secret-key generation rates under practical limitations of detectors or light sources, as well as greater error tolerance.

Indistinguishable single-mode photons from spectrally engineered biphotons.

We use pulsed spontaneous parametric down-conversion in KTiOPO , with a Gaussian phase-matching function and a transform-limited Gaussian pump, to achieve near-unity spectral purity in heralded single photons at telecommunication wavelength. Theory shows that these phase-matching and pump conditions are sufficient to ensure that a biphoton state with a circularly symmetric joint spectral intensity profile is transform limited and factorable. We verify the heralded-state spectral purity in a four-fold coincidence measurement by performing Hong-Ou-Mandel interference between two independently generated heralded photons.

Revealing hidden scenes by photon-efficient occlusion-based opportunistic active imaging.

The ability to see around corners, i.e., recover details of a hidden scene from its reflections in the surrounding environment, is of considerable interest in a wide range of applications.

Unity-Efficiency Parametric Down-Conversion via Amplitude Amplification.

We propose an optical scheme, employing optical parametric down-converters interlaced with nonlinear sign gates (NSGs), that completely converts an n-photon Fock-state pump to n signal-idler photon pairs when the down-converters' crystal lengths are chosen appropriately. The proof of this assertion relies on amplitude amplification, analogous to that employed in Grover search, applied to the full quantum dynamics of single-mode parametric down-conversion. When we require that all Grover iterations use the same crystal, and account for potential experimental limitations on crystal-length precision, our optimized conversion efficiencies reach unity for 1≤n≤5, after which they decrease monotonically for n values up to 50, which is the upper limit of our numerical dynamics evaluations.

Efficient generation and characterization of spectrally factorable biphotons.

Spectrally unentangled biphotons with high single-spatiotemporal-mode purity are highly desirable for many quantum information processing tasks. We generate biphotons with an inferred heralded-state spectral purity of 99%, the highest to date without any spectral filtering, by pulsed spontaneous parametric downconversion in a custom-fabricated periodically-poled KTiOPO crystal under extended Gaussian phase-matching conditions. To efficiently characterize the joint spectral intensity of the generated biphotons at high spectral resolution, we employ a commercially available dispersion compensation module (DCM) with a dispersion equivalent to 100 km of standard optical fiber and with an insertion loss of only 2.

Photon-efficient imaging with a single-photon camera.

Reconstructing a scene's 3D structure and reflectivity accurately with an active imaging system operating in low-light-level conditions has wide-ranging applications, spanning biological imaging to remote sensing. Here we propose and experimentally demonstrate a depth and reflectivity imaging system with a single-photon camera that generates high-quality images from ∼1 detected signal photon per pixel. Previous achievements of similar photon efficiency have been with conventional raster-scanning data collection using single-pixel photon counters capable of ∼10-ps time tagging.

Computational multi-depth single-photon imaging.

We present an imaging framework that is able to accurately reconstruct multiple depths at individual pixels from single-photon observations. Our active imaging method models the single-photon detection statistics from multiple reflectors within a pixel, and it also exploits the fact that a multi-depth profile at each pixel can be expressed as a sparse signal. We interpret the multi-depth reconstruction problem as a sparse deconvolution problem using single-photon observations, create a convex problem through discretization and relaxation, and use a modified iterative shrinkage-thresholding algorithm to efficiently solve for the optimal multi-depth solution.

Classical imaging with undetected photons.

Barreto Lemos et al. [Nature 512, 409-412 (2014)] reported an experiment in which a non-degenerate parametric downconverter and a non-degenerate optical parametric amplifier--used as a wavelength-converting phase conjugator--were employed to image object transparencies in a manner akin to ghost imaging. Their experiment, however, relied on single-photon detection, rather than the photon-coincidence measurements employed in ghost imaging with a parametric downconverter source.

Entanglement-enhanced sensing in a lossy and noisy environment.

Nonclassical states are essential for optics-based quantum information processing, but their fragility limits their utility for practical scenarios in which loss and noise inevitably degrade, if not destroy, nonclassicality. Exploiting nonclassical states in quantum metrology yields sensitivity advantages over all classical schemes delivering the same energy per measurement interval to the sample being probed. These enhancements, almost without exception, are severely diminished by quantum decoherence.

Unconditional security of time-energy entanglement quantum key distribution using dual-basis interferometry.

High-dimensional quantum key distribution (HDQKD) offers the possibility of high secure-key rate with high photon-information efficiency. We consider HDQKD based on the time-energy entanglement produced by spontaneous parametric down-conversion and show that it is secure against collective attacks. Its security rests upon visibility data-obtained from Franson and conjugate-Franson interferometers-that probe photon-pair frequency correlations and arrival-time correlations.

First-photon imaging.

Imagers that use their own illumination can capture three-dimensional (3D) structure and reflectivity information. With photon-counting detectors, images can be acquired at extremely low photon fluxes. To suppress the Poisson noise inherent in low-flux operation, such imagers typically require hundreds of detected photons per pixel for accurate range and reflectivity determination.

Entanglement's benefit survives an entanglement-breaking channel.

Entanglement is essential to many quantum information applications, but it is easily destroyed by quantum decoherence arising from interaction with the environment. We report the first experimental demonstration of an entanglement-based protocol that is resilient to loss and noise which destroy entanglement. Specifically, despite channel noise 8.

Ghost imaging without discord.

Ragy and Adesso argue that quantum discord is involved in the formation of a pseudothermal ghost image. We show that quantum discord plays no role in spatial light modulator ghost imaging, i.e.

Spectral engineering by Gaussian phase-matching for quantum photonics.

We demonstrate Gaussian-shaped phase matching of a periodically-poled potassium titanyl phosphate (PPKTP) crystal by imposing a custom duty-cycle pattern on its grating structure while keeping the grating period fixed. The PPKTP's phase-matching characteristics are verified through optical difference-frequency generation measurements, showing good agreement with expected values based on our design parameters. Our theoretical analysis predicts that under extended phase-matching conditions the custom-poled PPKTP crystal is capable of generating heralded single photons with a spectral purity of 97%, and can reach as high as 99.

Near-infrared Hong-Ou-Mandel interference on a silicon quantum photonic chip.

Near-infrared Hong-Ou-Mandel quantum interference is observed in silicon nanophotonic directional couplers with raw visibilities on-chip at 90.5%. Spectrally-bright 1557-nm two-photon states are generated in a periodically-poled KTiOPO₄ waveguide chip, serving as the entangled photon source and pumped with a self-injection locked laser, for the photon statistical measurements.

Efficient single-spatial-mode periodically-poled KTiOPO4 waveguide source for high-dimensional entanglement-based quantum key distribution.

We demonstrate generation of high-purity photon pairs at 1560 nm in a single spatial mode from a periodically-poled KTiOPO4 (PPKTP) waveguide. With nearly lossless spectral filtering, the PPKTP waveguide source shows approximately 80 % single-mode fiber coupling efficiency and is well suited for high-dimensional time-energy entanglement-based quantum key distribution. Using high-count-rate self-differencing InGaAs single-photon avalanche photodiodes configured with either square or sinusoidal gating, we achieve > 1 Mbit/s raw key generation with 3 bits-per-photon encoding, and, to the best of our knowledge, the highest reported Franson quantum-interference visibility of 98.

Exploiting sparsity in time-of-flight range acquisition using a single time-resolved sensor.

Range acquisition systems such as light detection and ranging (LIDAR) and time-of-flight (TOF) cameras operate by measuring the time difference of arrival between a transmitted pulse and the scene reflection. We introduce the design of a range acquisition system for acquiring depth maps of piecewise-planar scenes with high spatial resolution using a single, omnidirectional, time-resolved photodetector and no scanning components. In our experiment, we reconstructed 64 × 64-pixel depth maps of scenes comprising two to four planar shapes using only 205 spatially-patterned, femtosecond illuminations of the scene.

Classical far-field phase-sensitive ghost imaging.

We report the first (to our knowledge) far-field ghost images formed with phase-sensitive classical-state light and compare them with ghost images of the same object formed with conventional phase-insensitive classical-state light. To generate signal and reference beams with phase-sensitive cross correlation, we used a pair of synchronized spatial light modulators that imposed random, spatially varying, anticorrelated phase modulation on the outputs from 50-50 beam splitting of a laser beam. In agreement with theory, we found the phase-sensitive image to be inverted, whereas the phase-insensitive image is erect, with both having comparable spatial resolutions and signal-to-noise ratios.